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Optics Express

Coherent 420 nm light generated by the cavity-enhanced four-wave mixing process in Rb vapor

Jinpeng Yuan, Hao Liu, Lirong Wang, Liantuan Xiao, Suotang Jia

Published Jan 26, 2021• 20 citations
Publisher

Abstract

We have generated a stable and continuously tunable single frequency (420 nm) coherent blue light (CBL) by the cavity-enhanced four-wave mixing process in Rb vapor. With the bow-tie-type ring cavity, the output power was 3.3 mW, two orders of magnitude higher than that of the CBL generated by the single-pass four-wave mixing process. The measured power stabilities of the 420 nm CBL operated at 2.5 mW and 1.5 mW for 1000 s were 2.89% and 1.88%, respectively. Under the scanning pump laser frequency, the continuously tunable range of the generated CBL reached 1.68 GHz without mode hopping. The measured beam qualities of the generated laser were M x 2 = 1.117 and M y 2 = 1.179 . The excellent performance of the 420 nm CBL was characterized by velocity transfer spectroscopy with 780 nm probe laser. This high quality short wavelength coherent light is potentially applicable to photon-atom interactions in quantum optics and fundamental research fields.

DOI
10.1364/oe.416307

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Acta Physica Sinica•Jan 1, 2022•3 citations
We have generated a stable and continuously tunable single frequency (420 nm) coherent blue light (CBL) by the cavity-enhanced four-wave mixing process in Rb vapor. With the bow-tie-type ring cavity, the output power was 3.3 mW, two orders of magnitude higher than that of the CBL generated by the single-pass four-wave mixing process. The measured power stabilities of the 420 nm CBL operated at 2.5 mW and 1.5 mW for 1000 s were 2.89% and 1.88%, respectively. Under the scanning pump laser frequency, the continuously tunable range of the generated CBL reached 1.68 GHz without mode hopping. The measured beam qualities of the generated laser were M x 2 = 1.117 and M y 2 = 1.179 . The excellent performance of the 420 nm CBL was characterized by velocity transfer spectroscopy with 780 nm probe laser. This high quality short wavelength coherent light is potentially applicable to photon-atom interactions in quantum optics and fundamental research fields.
Diode-pumped alkali lasers, possessing high efficiency and narrow linewidth, can provide feasible solutions for wavelength ranges difficult to reach by commercial lasers. In this study, we investigate a generation of coherent blue light (CBL) via four-wave mixing (FWM)-based up-conversion processes in cesium (Cs) vapor. A bichromatic pumping scheme with 852- and 917-nm lasers drives the Cs atoms to the 6 D 5/2 excited level, followed by cascaded decay of 6 D 5/2 → 7 P 3/2 → 6 S 1/2 , producing 456-nm CBL under phase matching conditions. The fluorescence in multiple bands from blue to near- and far-infrared in the FWM process is demonstrated under different experimental conditions. To optimize the experimental parameters, we investigate the dependence of 456-nm CBL on the vapor temperature, frequency, and intensity of the two pump lasers. A maximum power of 2.94 mW is achieved with pump powers of 430 mW (for 852 nm) and 470 mW (for 917 nm). The corresponding conversion efficiency is 1.5%/W, three-fold higher than those in previous studies. Our results can contribute to fundamental research on atom—photon interactions and quantum metrology.
We have investigated the frequency characteristics of the coherent 420 nm beam generated via parametric four-wave mixing (FWM). A single, high-power 778 nm laser is directed through a high-density rubidium cell with a detuning of 1 THz from the intermediate state, generating fields at 420 nm and 5.23 μm through FWM. The frequency of the 420 nm light has been found to shift as the excitation laser is tuned. The measured frequency shift ratio of 1.87±0.04 corresponds with the selection of a different velocity class at each excitation frequency, implying that the 5.23 μm beam frequency is correspondingly shifted. The 420 nm light has been tuned over a range of 1 GHz. This parametric FWM process has potential application as a tunable photon source at novel wavelengths.
We demonstrate the generation of the coherent 420 nm laser via parametric four-wave mixing process in Rb vapor. A single 778 nm laser with circular polarization is directly injected into a high-density atomic vapor, which drives the atoms from the 5S1/2 state to the 5D5/2 state with monochromatic two-photon transition. The frequency up-conversion laser is generated by the parametric four-wave mixing process under the phase matching condition. This coherent laser is firstly certified by the knife-edge method and a narrow range grating spectrometer. Then the generated laser power is investigated in terms of the power and frequency of the incoming beam as well as the density of the atoms. Finally, a 420 nm coherent laser with power of 19 μW and beam quality of M x 2 = 1.32 , M y 2 = 1.37 is obtained with optimal experimental parameters. This novel laser shows potential prospects in the measurement of material properties, information storage, and underwater optical communication.
The frequency evaluation of collimated blue light (CBL) generated by parametric four-wave mixing (FWM) in hot atomic vapor is presented. The cesium ( 133 Cs) atoms are excited from the 6S 1/2 ground state to 8S 1/2 excited state with the 852 and 795 nm pump lasers, producing an optical field at 4.2 µm through an amplified spontaneous emission via population inversion on the 8S 1/2 → 7P 3/2 transition and the 456 nm CBL via FWM on the 7P 3/2 → 6S 1/2 transition. The frequency shift of 456 nm CBL has been measured by velocity-selective optical pumping spectral technique when the frequency of any one of two pumping lasers is tuned. The ratio of the frequency shift of 456 nm CBL to the two-photon frequency detuning of two pumping lasers is 0.8912, implying that the generated 4.2 µm light frequency is also correspondingly shifted.
Abstract We demonstrate 1.37 µ m coherent near-infrared light generation via self-seeded parametric four-wave mixing (FWM) process in Rb atomic vapor. Two lasers (780 nm and 776 nm) in the co-propagating configuration, drive the Rb atoms from the 5S 1/2 ground state to the 5D 5/2 excited state. The parametric FWM around the 5P 3/2 –5D 5/2 –6P 3/2 –6S 1/2 –5P 3/2 transition loop is effectively established under phase matching conditions. The generated coherent light wavelength is confirmed using an optical spectrum analyzer, and the output power is investigated with the input laser frequency, power and atomic density. Consequently, a 1.37 µ m coherent light with the power of 27 µ W and the beam quality of M x 2 = 1.22 and M y 2 = 1.25 is obtained. An additional 795 nm laser is introduced to enhance the output power by 1.5 times through velocity-selective optical hyperfine repumping.
We demonstrate the generation of coherent and collimated blue light (CBL) based on cesium (Cs) 6S1/2(F = 4)→6P3/2(F' = 5)→6D5/2(F'' = 6)→7P3/2(F' = 5)→6S1/2(F = 4) diamond-type atomic system in a heated vapor cell. Two infrared pumping lasers with wavelengths at 852 nm (6S1/2→6P3/2) and 917 nm (6P3/2→6D5/2), provide step-wise excitation to the 6D5/2 excited state, and induce strong two-photon coherence between the 6S1/2 state and 6D5/2 state. The atoms undergo a double cascade accompanied with the amplified spontaneous emission at 15.1 μm via the 7P3/2 intermediate excited state, and produce a beam of 455 nm (7P3/2→6S1/2) CBL with highly spatiotemporal coherence through a parametric four-wave mixing process. We investigate the influence of experimental parameters such as polarization combination of the two pumping lasers, and their power, and the temperature of Cs vapor cell on the CBL. Especially, we add a beam of 894 nm laser operating at the 6S1/2(F = 3) →6P1/2 transition as repumping laser, which can pump atoms back to the 6S1/2(F = 4) state from the 6S1/2(F = 3) state, thus significantly improving the power of CBL. This technique of the CBL enhancement via optical pumping is also useful for the other alkali metal atoms.