Abstract Progress in the creation of large-scale, artificial quantum coherent structures demands the investigation of their nonequilibrium dynamics when strong interactions, even between remote parts, are non-perturbative. Analysis of multiparticle quantum correlations in a large system in the presence of decoherence and external driving is especially topical. Still, the scaling behavior of dynamics and related emergent phenomena are not yet well understood. We investigate how the dynamics of a driven system of several quantum elements (e.g., qubits or Rydberg atoms) changes with increasing number of elements. Surprisingly, a two-element system exhibits chaotic behaviors. For larger system sizes, a highly stochastic, far from equilibrium, hyperchaotic regime emerges. Its complexity systematically scales with the size of the system, proportionally to the number of elements. Finally, we demonstrate that these chaotic dynamics can be efficiently controlled by a periodic driving field. The insights provided by our results indicate the possibility of a reduced description for the behavior of a large quantum system in terms of the transitions between its qualitatively different dynamical regimes. These transitions are controlled by a relatively small number of parameters, which may prove useful in the design, characterization, and control of large artificial quantum structures.
Abstract Progress in the creation of large-scale, artificial quantum coherent structures demands the investigation of their nonequilibrium dynamics when strong interactions, even between remote parts, are non-perturbative. Analysis of multiparticle quantum correlations in a large system in the presence of decoherence and external driving is especially topical. Still, the scaling behavior of dynamics and related emergent phenomena are not yet well understood. We investigate how the dynamics of a driven system of several quantum elements (e.g., qubits or Rydberg atoms) changes with increasing number of elements. Surprisingly, a two-element system exhibits chaotic behaviors. For larger system sizes, a highly stochastic, far from equilibrium, hyperchaotic regime emerges. Its complexity systematically scales with the size of the system, proportionally to the number of elements. Finally, we demonstrate that these chaotic dynamics can be efficiently controlled by a periodic driving field. The insights provided by our results indicate the possibility of a reduced description for the behavior of a large quantum system in terms of the transitions between its qualitatively different dynamical regimes. These transitions are controlled by a relatively small number of parameters, which may prove useful in the design, characterization, and control of large artificial quantum structures.
Progress in the creation of large scale, artificial quantum coherent structures demands the investigation of their nonequilibrium dynamics when strong interactions, even between remote parts, are non-perturbative. Analysis of multiparticle quantum correlations in a large system in the presence of decoherence and external driving is especially topical. Still, scaling behaviour of dynamics and related emergent phenomena are not yet well understood. We investigate how the dynamics of a driven system of several quantum elements (e.g., qubits or Rydberg atoms) changes with increasing number of elements. Surprisingly, a two-element system exhibits chaotic behaviours. For larger system sizes a highly stochastic, far from equilibrium, {\em hyperchaotic} regime emerges. Its complexity systematically scales with the size of the system, proportionally to the number of elements. Finally, we demonstrate that these chaotic dynamics can be efficiently controlled by a periodic driving field. The insights provided by our results indicate the possibility of a reduced description for the behaviour of a large quantum system in terms of the transitions between its qualitatively different dynamical regimes, which are controlled by a relatively small number of parameters, and may prove useful in the design, characterization and control of large artificial quantum structures.
Due to the variety of tools available to control atomic, molecular, and optical (AMO) systems, they provide a versatile platform for studying many-body physics, quantum simulation, and quantum computation. Although extensive efforts are employed to reduce coupling between the system and the environment, the effects of the environment can never fully be avoided, so it is important to develop a comprehensive understanding of open quantum systems. The system-environment coupling often leads to loss via dissipation, which can be countered by a coherent drive. Open quantum systems subject to dissipation and drive are known as driven-dissipative systems, and they provide an excellent platform for studying many-body nonequilibrium physics. The first part of this dissertation will focus on driven-dissipative phase transitions. Despite the nonequilibrium nature of these systems, the corresponding phase transitions tend to exhibit emergent equilibrium behavior. However, we will show that in the vicinity of a multicritical point where multiple phase transitions intersect, genuinely nonequilibrium criticality can emerge, even though the individual phase transitions on their own exhibit equilibrium criticality. These nonequilibrium multicritical points can exhibit a variety of exotic phenomena not possible for their equilibrium counterparts, including the emergence of complex critical exponents, which lead to discrete scale invariance and spiraling phase boundaries. Furthermore, the Liouvillian gap can take on complex values, and the fluctuation-dissipation theorem is violated, corresponding to an effective temperature which gets "hotter" and "hotter" at longer and longer wavelengths. The second part of this dissertation will focus on Rydberg atoms. In particular, we study how the spontaneous generation of contaminant Rydberg states drastically modifies the behavior of a driven-dissipative Rydberg system due to the resultant dipole-dipole interactions. These interactions lead to a complicated competition of both blockade and anti-blockade effects, leading to strongly enhanced Rydberg populations for far-detuned drive and reduced Rydberg populations for resonant drive.
This thesis presents several experiments investigating the regimes of behaviour of a proto-typical open quantum many-body system far away from equilibrium. The experimental platform is based on ultracold atoms laser-excited to Rydberg states, which we engineer to emulate a strongly interacting, driven-dissipative quantum spin system. The high degree of control over the relevant microscopic processes and their parameters, as well as the ability to widely tune interaction and driving strengths provides the means to address fundamental questions on how different regimes of dynamical behaviour emerge in complex open quantum systems and how they can be characterised. \n \nIn the first part, we discuss how control over the relevant properties of Rydberg spin systems, like temperature, density, long evolution times, strong interactions, tunable driving, and dissipation can be achieved. We introduce the new experimental apparatus developed during this thesis, which combines both single-photon and two-photon Rydberg excitation schemes with high atom densities and long excitation times using an optical dipole trap. Additionally, we investigate theoretically how long coherence times exceeding motional timescales combined with strong many-body interactions can be achieved in such a system. We identify an optimal parameter regime for two-photon excitation where such conditions can be generated with coherence times and interaction strengths comparable to what is achievable for single-photon excitation. \n \nIn the second part we explore the macroscopic non-equilibrium behaviour of our system and devise suitable observables for characterising different regimes of behaviour. We discover that the slow atom loss inherent to our system provides a convenient observable for the many-body state of the system. Focussing on evolution times where the effect of the atom loss on the evolution is small, we discover that the rate of atom loss exhibits powerlaw scaling with the driving strength over several orders of magnitude. The measured scaling exponents reveal the non-equilibrium phase structure of the many-body system and allow us to distinguish dissipation-dominated, paramagnetic and critical regimes, as well as an instability. In the observed critical regime, collectively enhanced driving dominates over dissipation, leading to scaling associated to the critical point of the non-dissipative equilibrium Rydberg spin system. Based on the known microscopic processes of our system, we perform classical many-body rate equation simulations, which agree well with the observed phase structure as well as the position and associated scaling exponents of the individual regimes. These findings open up new means to study and classify out of equilibrium systems based on slow particle loss and powerlaw scaling. \n \nIn the last part of this thesis we reveal a second type of criticality in our system, which is genuinely non-equilibrium in character and arises from an absorbing state phase transition. The critical state of this phase transition dominates the system evolution at late times where particle loss is no longer negligible. We identify self-organisation as the mechanism driving the system to this critical state, which we observe through powerlaw scaling of the non-equilibrium steady-state. These experiments establish Rydberg atoms as a well controlled platform for implementing and exploring models of absorbing state phase transitions and self-organised criticality with unprecedented access to the underlying microscopic properties of the system.
Non-equilibrium quantum dynamics represents an emerging paradigm for condensed matter physics, quantum information science, and statistical mechanics. Strongly interacting Rydberg atoms offer an attractive platform to examine driven-dissipative dynamics of quantum spin models with long-range order. Here, we explore the conditions under which stationary many-body entanglement persists with near-unit fidelity and high scalability. In our approach, coherent many-body dynamics is driven by Rydberg-mediated laser transitions, while atoms at the lattice boundary locally reduce the entropy of the many-body system. Surprisingly, the many-body entanglement is established by continuously evolving a locally dissipative Rydberg system towards the steady state, precisely as with optical pumping. We characterize the dynamics of multipartite entanglement in an one-dimensional lattice by way of quantum uncertainty relations, and demonstrate the long-range behavior of the stationary entanglement with finite-size scaling. Our work opens a route towards dissipative preparation of many-body entanglement with unprecedented scaling behavior.
Reliable processing of quantum information for developing quantum technologies requires precise control of out-of-equilibrium many-body systems. This is a highly challenging task because the fragility of quantum states to external perturbations increases with the system size. Here, we report on a series of experimental quantum simulations that quantify the sensitivity of a controlled Hamiltonian evolution to perturbations that drive the system away from the targeted evolution. Based on out-of-time ordered correlations, we demonstrate that the decay rate of the process fidelity increases with the effective number K of correlated qubits as ${K}^{\ensuremath{\alpha}}$. As a function of the perturbation strength, we observe a decoherence scaling transition of the exponent $\ensuremath{\alpha}$ between two distinct dynamical regimes. In the limiting case below the critical perturbation strength, the exponent $\ensuremath{\alpha}$ drops sharply below 1, and there is no inherent limit to the number of qubits that can be controlled. This resilient quantum feature of the controlled dynamics of quantum information is promising for reliable control of large quantum systems.
The control of nonequilibrium quantum dynamics in many-body systems is challenging because interactions typically lead to thermalization and a chaotic spreading throughout Hilbert space. We investigate nonequilibrium dynamics after rapid quenches in a many-body system composed of 3 to 200 strongly interacting qubits in one and two spatial dimensions. Using a programmable quantum simulator based on Rydberg atom arrays, we show that coherent revivals associated with so-called quantum many-body scars can be stabilized by periodic driving, which generates a robust subharmonic response akin to discrete time-crystalline order. We map Hilbert space dynamics, geometry dependence, phase diagrams, and system-size dependence of this emergent phenomenon, demonstrating new ways to steer complex dynamics in many-body systems and enabling potential applications in quantum information science.