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Physics of Electronic and Atomic Collisions: ICPEAC VIII

Multiphoton Radiative Atomic and Molecular Collisions

B. I. Ermolaev, V. E. Khartsiev

Published Jan 1, 1973• 0 citations
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Multiphoton Ionization of Atomic and Molecular Hydrogen at 0.53 μ

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This work reports multiphoton ionization and dissociation of molecular hydrogen under the influence of laser radiation at 0.53 $\ensuremath{\mu}$. The six-photon ionization probability of hydrogen atoms is derived for laser radiation acting upon atomic hydrogen from a molecular hydrogen beam which is up to 80% dissociated by radio-frequency power. The experimental six-photon ionization probability of atomic hydrogen has been found to be in good agreement with the corresponding probability calculated using time-dependent perturbation theory if the statistical properties of the incident light are taken into account.

Physical Review A•Jan 1, 1973•64 citations
Merging two subfields, collisions and spectroscopy, this book presents the latest research proposals, innovative experiments and fresh ideas. Topics considered include radiative collision induced electron continuum-continuum scattering; models of laser-induced chemical reactions; experimental studies of laser-induced ionizing collisions; laser photodissociation of Na/sub 2/ + ions produced by laser resonant ionization of Na vapor; steady-state electron-atom collision in a laser field; conditions for the observation of the predicted splitting of the laser assisted electron impact of the differential cross section of atoms; transitions between resonances; some proposals for experiments; above-threshold multiphoton ionization; observability of optical collisions in the frequency and the time domain; laser switched collisions - a diagrammatical approach; polarization of atomic fluorescence excited by molecular photodissociation; multiphoton selective excitation; on the role of chaotic dynamics with many basins of attraction; predissociation in a strong electromagnetic field; theory of double resonance; and coherent excitation of polyatomic molecules up to highly excited vibrational states by laser light.
This work reports multiphoton ionization and dissociation of molecular hydrogen under the influence of laser radiation at 0.53 $\ensuremath{\mu}$. The six-photon ionization probability of hydrogen atoms is derived for laser radiation acting upon atomic hydrogen from a molecular hydrogen beam which is up to 80% dissociated by radio-frequency power. The experimental six-photon ionization probability of atomic hydrogen has been found to be in good agreement with the corresponding probability calculated using time-dependent perturbation theory if the statistical properties of the incident light are taken into account.