In this article, we introduce a universal simulation framework covering all regimes of matter-wave light-pulse elastic scattering. Applied to atom interferometry as a study case, this simulator solves the atom-light diffraction problem in the elastic case, i.e., when the internal state of the atoms remains unchanged. Taking this perspective, the light-pulse beam splitting is interpreted as a space and time-dependent external potential. In a shift from the usual approach based on a system of momentum-space ordinary differential equations, our position-space treatment is flexible and scales favourably for realistic cases where the light fields have an arbitrary complex spatial behaviour rather than being mere plane waves. Moreover, the solver architecture we developed is effortlessly extended to the problem class of trapped and interacting geometries, which has no simple formulation in the usual framework of momentum-space ordinary differential equations. We check the validity of our model by revisiting several case studies relevant to the precision atom interferometry community. We retrieve analytical solutions when they exist and extend the analysis to more complex parameter ranges in a cross-regime fashion. The flexibility of the approach, the insight it gives, its numerical scalability and accuracy make it an exquisite tool to design, understand and quantitatively analyse metrology-oriented matter-wave interferometry experiments.
Large-momentum-transfer techniques are instrumental for the next generation of atom interferometers as they significantly improve their sensitivity. State-of-the-art implementations rely on elastic scattering processes from optical lattices such as Bloch oscillations or sequential Bragg diffraction, but their performance is constrained by imperfect pulse efficiencies. Here we develop a Floquet-based theoretical framework that provides a unified description of elastic light-atom scattering across all relevant regimes. Within this formalism, we identify practical regimes that exhibit orders of magnitude reduced losses and improved phase accuracy compared to previous implementations. The model's validity is established through direct comparison with numerical solutions of the Schrödinger equation and through quantitative agreement with recent experimental benchmark results. These findings delineate previously unexplored operating regimes for large momentum transfer beam splitters and open new perspectives for precision atom-interferometric measurements in fundamental physics, gravity gradiometry or gravitational wave detection.
We have used an echo-type atom interferometer that manipulates laser-cooled atoms in a single ground state to investigate the effect of light scattering from pulsed and continuous-wave light. The interferometer uses two off-resonant standing-wave pulses applied at times t=0 and t=T to diffract and recombine momentum states separated by $2\ensuremath{\hbar}k$ at t=2T. Matter wave interference is associated with the formation of a density grating with period $\ensuremath{\lambda}/2$ in the vicinity of this echo time. The grating contrast is measured by recording the intensity of coherently backscattered light. The interferometer is perturbed by an additional pulse applied at $t=2T\ensuremath{-}\ensuremath{\delta}T$ or by continuous-wave background light. If the additional pulse is a standing wave, the momentum states interfering at t=2T are displaced and the grating contrast can be completely recovered due to constructive interference. In this case, the contrast shows a periodic modulation at the atomic recoil frequency as a function of $\ensuremath{\delta}T$. In a recent work, it was shown that the atomic recoil frequency can be measured easily and precisely when using coherence functions to model the signal shape. This paper provides an alternative description of the signal shape through an analytical calculation of echo formation in the presence of an additional standing-wave pulse. Using this treatment, it is possible to model the effects of spontaneous emission and spatial profile of the laser beam on the signal shape. Additionally, the theory predicts scaling laws as a function of the pulse area and the number of additional standing-wave pulses. These scaling laws are investigated experimentally and can be exploited to improve precision measurements of the atomic recoil frequency. We also show that coherence functions can be used to make a direct measurement of the populations of momentum states associated with the ground state under conditions where the Doppler-broadened velocity distribution of the sample is much larger than the recoil velocity. These measurements are consistent with Monte Carlo wave-function simulations. If the additional pulse is a traveling wave, we find that the grating contrast measured as a function of $\ensuremath{\delta}T$ can be modeled by a quasiperiodic coherence function as in previous experiments that utilized atomic beams. In this work, we investigate the dependence of the photon scattering rate on the intensity and detuning of the traveling wave. We also study the effects of perturbing the interferometer with continuous-wave light and find that the dependence of the photon scattering rate on the intensity and detuning of the perturbing field is consistent with expectations.
Light-pulse atom interferometers serve as tools for high-precision metrology and are targeting measurements of relativistic effects. This development is facilitated by extended interrogation times and large-momentum-transfer techniques generating quantum superpositions of both interferometer arms on large distances. Due to the finite speed of light, diffracting light pulses cannot interact simultaneously with both arms, inducing phase perturbations that compromise the accuracy of the sensor -- an effect that becomes progressively important as spatial separations increase. For a consistent framework, we develop a theory for finite-speed-of-light effects in atom interferometers alongside with other relativistic effects such as the mass defect. Our analysis shows that their magnitude depends crucially on the diffraction mechanism and the specific interferometer geometry. We demonstrate that the velocity of the atomic cloud at the mirror pulse of a Mach-Zehnder interferometer is less critical than the precise tuning of the lasers for resonant diffraction. Finally, we propose an experiment to test our predictions based on recoilless transitions and discuss mitigation strategies to reduce the bias in gravimetric applications.
Inertial navigation systems are vital for modern society, be it on airplanes or in the context of autonomous mobility. On the other hand atom interferometers are exquisite measurement devices for inertia in fundamental physics and field applications, but are mostly limited to measuring one inertial observable. By utilizing time averaged optical potentials, the ultra-cold atomic ensemble input to the interferometer can be prepared in nearly arbitrary fashion. This results in a boost of preparation speed and number of atoms in the interferometer by increasing the size of the trap to match the size of the pre-cooled ensemble for optimal loading. Successive fast reduction of the extend of the trap leads to optimal evaporation efficiency and leads to increased sensitivity of the device, due to reduced cycle time of the experiment and increased atom number. Beyond this, the technique allows for new sensor geometries via the creation of multiple single wells, allowing for differential atom interferometry with numerous simultaneous interferometers. In this thesis, the first matter-wave analogue of a classical accelerometer array is implemented via the creation of a 3 × 3 array of Bose-Einstein condensates, consisting of 3 × 105 atoms and spanning a total area of 1.6 mm2 . Successive manipulation of the matter-waves with atom optics, coherently addressing the momentum states of the ensembles, allows for splitting, redirecting and readout pulses, realizing Mach-Zehnder type atom interferometers. Correlation of the nine 1D-acceleration measurements output by the interferometers yields measurements of linear acceleration, Euler- and centrifugal acceleration. The estimated sensitivity limits per shot are 6 × 10−5m s−2 for linear acceleration, 0.19 rad s − 2 for rotational acceleration and 203 mrad s−1 for rotation rate and are mainly limited due to the short free fall time of the ensembles, constrained by the atom optics light field. The correlation also allowed to determine the rotation center, being close to the retro reflection mirror of the atom optics light field. Crucial for the realization of this measurement was the implementation of time averaged potentials as stated above, facilitated through two 2D acousto-optical deflectors and a software defined radio, allowing for generating the required RF-signals. The techniques to simultaneously load and evaporate multiple ensembles into distinct traps from a single cloud of cold atoms and subsequently enlarge the spacing between the ensembles with adiabatic transport ramps are of highest interest for e.g. the Very Long Baseline Atom Interferometer facility in Hannover. Due to the correlated outputs systematic errors, such as wave front abberations, can be nullified. Furthermore the scheme can be extended to 3D matter-wave arrays, fulfilling all requirements necessary for an autonomous inertial measurement unit.
This cumulative thesis consists of four publications [1-4], presented as three contributions (I) - (III), where the second one (II) consists of the joint publications [2,3]. All publications were written during the author's research activities at the Institute of Quantum Physics under the supervision of Prof. Dr. W. P. Schleich. All of the presented publications consider light-matter interactions and their potential application in atom interferometry, a comparatively young and rapidly evolving technique. Atom interferometers find application in high-precision measurements, the determination of physical constants, the testing of fundamental physics, and the provision of gravimeters and gyroscopes. The advancement of technology and science has led to significant improvements in performance and the development of ambitious mobile and space-based devices. The recent success of several experiments has led to the proposal of further experiments with the aim of opening up new frontiers. However, the construction of future devices necessitates a decision regarding the employed diffraction mechanism and geometry, depending on the specific technical and scientific requirements. Furthermore, it is necessary to enhance the sensitivity of future devices. The contributions in this dissertation address these issues. The first contribution (I) focuses on the diffraction of atoms by laser pulses which can be employed to generate atom-optical diffraction elements like beam splitters and mirrors. These diffraction elements can be combined to construct atom interferometers, which have been successfully employed for precision measurements regarding fundamental physics as well as practical applications. The article presents a numerical comparison of two distinct diffraction mechanisms (Bragg and Raman) and diffraction geometries (single and double diffraction) in microgravity. It discusses the fundamental differences between the mechanisms and geometries with respect to the diffraction efficiency, taking into account the width of the initial wave function and the duration of the light pulse. Additionally, it explores the transition between the two diffraction geometries when starting from an atom initially at rest and increasing its momentum. The results may serve as a reference for experimentalists in selecting the most suitable configuration, based on their aims and requirements in the realization of more advanced atom interferometers. The second contribution (II) is a follow-up to the previous one, but focuses exclusively on a single diffraction type in microgravity, namely the so-called double Raman diffraction. In contrast to the previous article, where we only discussed single two-photon processes, we consider in this article a six-photon process, also known as third-order diffraction, as well as three subsequent two-photon processes, which both lead to the same amount of transferred momentum and can both be used to realize large-momentum transfer (LMT). We demonstrate that third-order double Raman diffraction is a viable and advantageous method for the diffraction of small momentum distributions like Bose-Einstein condensates (BECs) compared to a sequence of three two-photon processes. Furthermore, we show that third-order Raman pulses can be successfully applied to create higher-order Raman atom interferometers. Third-order diffraction can be perfectly combined with other LMT techniques and, moreover, allows for a reduction in the overall duration of the diffraction process and the complexity of the experimental set-up, as only two distinct laser frequencies are required. Moreover, we present a third-order Mach-Zehnder interferometer with spurious paths being disregarded. As demonstrated later on in [3], this interferometer generates optimal contrast and a substantial amplitude. The third contribution (III) extends the semi-classical λ-scheme of single Raman diffraction, as discussed in detail in contribution (I), into a fully quantized multi-atom multi-λ configuration with center-of-mass motion inside a cavity. Therefore, the incorporation of an internal structure allows for a more realistic modeling of the atoms, which is relevant for multi-photon interaction or cooling processes. We use for our analysis the framework of second quantization, i.e., we take into account the field-theoretical nature of the multi-particle atomic field as well as of the diffracting light field. We reduce this model with a Hamiltonian averaging theory applied to the atomic field operators and obtain an effective Hamiltonian, which determines the time evolution of the system. We demonstrate the efficiency of our model by the application of a typical initial state. Moreover, for a specific input state, we obtain the Hong-Ou-Mandel effect simultaneously in the atomic and the optical system. Our many-body formalism is perfectly suited to theoretically describe contemporary high-precision atom interferometric experiments based on entanglement between the atoms, that aim to surpass the shot-noise limit.