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Optics Express

Quantum-correlated photon-pair generation via cascaded nonlinearity in an ultra-compact lithium-niobate nano-waveguide

Bradley S. Elkus, Kamal Abdelsalam, Sasan Fathpour, Prem Kumar, Gregory S. Kanter

Published Dec 5, 2020• 23 citations
Publisher

Abstract

We generate quantum-correlated photon pairs using cascaded χ ( 2 ) : χ ( 2 ) traveling-wave interactions for second-harmonic generation (SHG) and spontaneous parametric down-conversion (SPDC) in a single periodically-poled thin-film lithium-niobate (TFLN) waveguide. When pulse-pumped at 50 MHz, a 4-mm-long poled region with nearly 300%/Wcm2 SHG peak efficiency yields a generated photon-pair probability of 7±0.2 × 10−4 with corresponding coincidence-to-accidental ratio (CAR) of 13.6±0.7. The CAR is found to be limited by Stokes/anti-Stokes Raman-scattering noise generated primarily in the waveguide. A Raman peak of photon counts at 250 cm−1 Stokes shift from the fundamental-pump wavenumber suggests most of the noise that limits the CAR originates within the lithium niobate material of the waveguide.

DOI
10.1364/oe.411575

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We generate quantum-correlated photon pairs using cascaded χ ( 2 ) : χ ( 2 ) traveling-wave interactions for second-harmonic generation (SHG) and spontaneous parametric down-conversion (SPDC) in a single periodically-poled thin-film lithium-niobate (TFLN) waveguide. When pulse-pumped at 50 MHz, a 4-mm-long poled region with nearly 300%/Wcm2 SHG peak efficiency yields a generated photon-pair probability of 7±0.2 × 10−4 with corresponding coincidence-to-accidental ratio (CAR) of 13.6±0.7. The CAR is found to be limited by Stokes/anti-Stokes Raman-scattering noise generated primarily in the waveguide. A Raman peak of photon counts at 250 cm−1 Stokes shift from the fundamental-pump wavenumber suggests most of the noise that limits the CAR originates within the lithium niobate material of the waveguide.
We report detailed experimental studies in a single wavelength-band system of correlated photon-pair generation in a 1.5 μm telecommunication wavelength-band using cascaded χ(2):χ(2) processes, second-harmonic generation, and the following spontaneous parametric down conversion (c-SHG/SPDC), in a periodically poled LiNbO3 (PPLN) ridge-waveguide device. By using a PPLN module with 600%/W of the SHG efficiency, we achieved a coincidence-to-accidental ratio (CAR) of 2380 at 1.8×10−4 of the mean number of the signal photon per pulse. Detailed investigation on the origin of uncorrelated noise photons was also discussed in this paper. We revealed that the noise photons mainly originated from spontaneous Raman scattering induced in pigtail optical fibers and also that the PPLN device itself had poor contribution to the noise photons. This feature of the c-SHG/SPDC process is promising for the realization of a noise-photon-free, high-purity quantum entangled photon-pair source.
Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.
We report the generation of high-purity correlated photon-pairs and polarization entanglement in a 1.5 μm telecommunication wavelength-band using cascaded χ((2)):χ((2)) processes, second-harmonic generation (SHG) and the following spontaneous parametric down conversion (SPDC), in a periodically poled LiNbO(3) (PPLN) ridge-waveguide device. By using a PPLN module with 600%/W of the SHG efficiency, we have achieved a coincidence-to-accidental ratio (CAR) higher than 4000 at 7.45×10(-5) of the mean number of the photon-pair per pulse. We also demonstrated that the maximum reach of the CAR was truly dark-count-limited by the single-photon detectors used here. This indicates that the fake (noise) photons were negligibly small in this system, even though the photon-pairs, the Raman noise photons, and the pump photons were in the same wavelength band. Polarization entangled photon pairs were also generated by constructing a Sagnac-loop-type interferometer which included the PPLN module and an optical phase-difference compensator to observe maximum entanglement. We achieved two-photon interference visibilities of 99.6% in the H/V basis and 98.7% in the diagonal basis. The peak coincidence count rate was approximately 50 counts per second at 10(-3) of the mean number of the photon-pair per pulse.
We demonstrate the generation of correlated photon pairs in a modal phase-matched lithium niobate nanowaveguide via cascaded second-harmonic generation (SHG) and spontaneous parametric down conversion (SPDC). A pair generation rate (PGR) of1.1×105HzmW−21.1 \times 10^{5} \text{Hz} \text{mW}^{-2}1.1×105HzmW−2and coincidence-toaccidental ratio (CAR) up to 188 are obtained.
A thin-film periodically poled lithium niobate waveguide was designed and fabricated which generates entangled photon pairs at telecommunications wavelengths with high coincidences-to-accidentals counts ratio CAR>67000, two-photon interference visibility V>99%, and heralded single-photon autocorrelation g_{H}^{(2)}(0)<0.025. Nondestructive in situ diagnostics were used to determine the poling quality in 3D. Megahertz rates of photon pairs were generated by less than a milliwatt of pump power, simplifying the pump requirements and dissipation compared to traditional spontaneous parametric down-conversion lithium niobate devices.