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Superradiance and Topological Quantum Optics in Atomic Medium and Cavity QED

Han Cai

Published Dec 8, 2017• 0 citations
OpenAlex

Abstract

In this dissertation we focused on two topics: 1. atomic cooperative effect, including superradiance, subradiance and collective Lamb shift in an atomic ensemble; 2. novel topological effect in quantum optics system, such as Haldane model, synthetic magnetic field in superradiance lattice and synthetic spin-orbit interaction in Fock-state lattices. \n\nIn the first part, we start from the Dicke state, an N-particle atomic ensemble excited by a single photon. Due to the interaction of the atoms with a continuum of vacuum modes, the Dicke state has a larger decay rate compared with an isolated atom, termed the single photon superradiance. In the “opposite” case, the single-photon subradiance state does not decay because of the destructive interference of the atomic transitions. We study the protection of subradiant states by the symmetry of the atomic distributions in the Dicke limit, in which collective Lamb shifts cannot be neglected. We find that antisymmetric states are subradiant states for distributions with reflection symmetry. Continuous symmetry can also be used to achieve subradiance in an extended ensemble. This study is relevant to the problem of robust quantum memory with long storage time and fast readout.\n\nIn the second part, we start from introducing the concepts, methods, and models from quantum optics or condensed matter physics. They include the timed-Dicke states, electromagnetically induced transparency, coupled wave equations, tight-binding model, band theory, Floquet theory, superradiance lattice, integer quantum Hall effect, Haldane model, etc.. Based upon these tools, we study three topological quantum optics systems: (i) a Haldane model with in situ tunable topological properties in a two-dimensional momentumspace superradiance lattice composed of timed Dicke states in electromagnetically induced transparency; (ii) a spin-orbit coupled Fock-state lattice, which introduce a novel quantum operation to generate mesoscopic superposition states, e.g., the NOON states and cat states; (iii) a synthetic magnetic field created in a quasi one dimensional superradiance lattice, which is predicted to be observed in thermal vapours of alkali atoms instead of only in cold atoms (as in previous experiments). This study aims to provide a novel, highly tunable platform simulating exotic phenomena in condensed matter physics and offers a basis of topological quantum optics and novel photonic devices.

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In this dissertation we focused on two topics: 1. atomic cooperative effect, including superradiance, subradiance and collective Lamb shift in an atomic ensemble; 2. novel topological effect in quantum optics system, such as Haldane model, synthetic magnetic field in superradiance lattice and synthetic spin-orbit interaction in Fock-state lattices. \n\nIn the first part, we start from the Dicke state, an N-particle atomic ensemble excited by a single photon. Due to the interaction of the atoms with a continuum of vacuum modes, the Dicke state has a larger decay rate compared with an isolated atom, termed the single photon superradiance. In the “opposite” case, the single-photon subradiance state does not decay because of the destructive interference of the atomic transitions. We study the protection of subradiant states by the symmetry of the atomic distributions in the Dicke limit, in which collective Lamb shifts cannot be neglected. We find that antisymmetric states are subradiant states for distributions with reflection symmetry. Continuous symmetry can also be used to achieve subradiance in an extended ensemble. This study is relevant to the problem of robust quantum memory with long storage time and fast readout.\n\nIn the second part, we start from introducing the concepts, methods, and models from quantum optics or condensed matter physics. They include the timed-Dicke states, electromagnetically induced transparency, coupled wave equations, tight-binding model, band theory, Floquet theory, superradiance lattice, integer quantum Hall effect, Haldane model, etc.. Based upon these tools, we study three topological quantum optics systems: (i) a Haldane model with in situ tunable topological properties in a two-dimensional momentumspace superradiance lattice composed of timed Dicke states in electromagnetically induced transparency; (ii) a spin-orbit coupled Fock-state lattice, which introduce a novel quantum operation to generate mesoscopic superposition states, e.g., the NOON states and cat states; (iii) a synthetic magnetic field created in a quasi one dimensional superradiance lattice, which is predicted to be observed in thermal vapours of alkali atoms instead of only in cold atoms (as in previous experiments). This study aims to provide a novel, highly tunable platform simulating exotic phenomena in condensed matter physics and offers a basis of topological quantum optics and novel photonic devices.
Topological phases of matters are of fundamental interest and have promising applications. Fascinating topological properties of light have been unveiled in classical optical materials. However, the manifestation of topological physics in quantum optics has not been discovered. Here we study the topological phases in a two-dimensional momentum-space superradiance lattice composed of timed Dicke states (TDS) in electromagnetically induced transparency (EIT). By periodically modulating the three EIT coupling fields, we can create a Haldane model with in-situ tunable topological properties, which manifest themselves in the contrast between diffraction signals emitted by superradiant TDS. The topological superradiance lattices provide a controllable platform for simulating exotic phenomena in condensed matter physics and offer a basis of topological quantum optics and novel photonic devices.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
We first study effects of collective states (CS) in both superradiant and electromagnetically induced transparent (EIT) systems. For superradiance, we incorporate cooperative effects into a two-atom master equation, which results in a superradiant decay time close to the experimental data. Additionally, we identify the role of collectivity in Raman superradiance in a Bose-Einstein condensate (BEC). As an application of CS to quantum information, we study the feasibility of EIT in semiconductors, a flexible multiple beam splitter for generating entangled single photons, and effect of diffusion of the stored coherence. ^ Second, we show that transverse momentum distribution may improve the phase resolution of an atomic interferometer. The improvement is due to the fact that the transit time for the transverse momentum states is a constant. ^ Third, atom and molecule currents in a Fermi gas in the neighborhood of a Feshbach resonance are studied in a one-dimensional optical ring lattice by directly diagonalizing small models. A rotational analogy of flux quantization is used to show that a fraction of the current is carried by particles with twice the mass of an atom, which suggests pairing and superfluidity of fermions. ^
Superradiance is one of the many fascinating phenomena predicted by quantum electrodynamics that have first been experimentally demonstrated in atomic systems and more recently in condensed matter systems like quantum dots, superconducting q-bits, cyclotron transitions and plasma oscillations in quantum wells (QWs). It occurs when a dense collection of N identical two-level emitters are phased via the exchange of photons, giving rise to enhanced light-matter interaction, hence to a faster emission rate. Of great interest is the regime where the ensemble interacts with one photon only and therefore all of the atoms, but one, are in the ground state. In this case the quantum superposition of all possible configurations produces a symmetric state that decays radiatively with a rate N times larger than that of the individual oscillators. This phenomenon, called single photon superradiance, results from the exchange of real photons among the N emitters. Yet, to single photon superradiance is also associated another collective effect that renormalizes the emission frequency, known as cooperative Lamb shift. In this work, we show that single photon superradiance and cooperative Lamb shift can be engineered in a semiconductor device by coupling spatially separated plasma resonances arising from the collective motion of confined electrons in QWs. These resonances hold a giant dipole along the growth direction z and have no mutual Coulomb coupling. They thus behave as a collection of macro-atoms on different positions along the z axis. Our device is therefore a test bench to simulate the low excitation regime of quantum electrodynamics.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
The interaction of confined atoms with a single mode radiation field is the main subject in the theory of cavity quantum electrodynamics . The constraints imposed by the cavity on matter and radiation fields give rise to collective phenomena. One possible outcome is the enhanced and coherent spontaneous emission of photons by the atoms: the superradiance. As predicted by Dicke, conservation laws are essential in superradiance and are derived from the matter-interaction Hamiltonian . Here, we consider N two-level ultracold atoms interacting with a single mode bosonic field, in the Dicke Hamiltonian, and trapped inside a non-dissipative optical cavity . Numerical and analytical results derived from finite size regime indicate the matter–radiation coupling strength, λ , is insufficient to draw the complete picture of the system. Instead, they support the relevance of U ( 1 ) symmetry, which prompts the study of (i) particle and angular momentum conservation, (ii) the constraints imposed to correlation functions and (iii) the influence of symmetries in the system dynamics . Further exploring the U ( 1 ) and rotational symmetries permits a simple interpretation of antirotating contributions as spin–orbit operators. As application, we show two species of ultracold clouds develop interactions due to antirotating operators.