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Journal of Experimental and Theoretical Physics

Radiation from a System of Resonant Molecules with Energy-level Scatter

A. I. Alekseev, Viktor Mikhaĭlovich Galit︠s︡kiĭ

Published Apr 1, 1966• 0 citations
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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Oct 29, 2010•1 citation
A mathematical modeling of the time evolution of the populations of the states of a five-level molecule during transformation of resonant monochromatic irradiation and spontaneous emission from the highest-energy state excited by a short pulse of light is performed. The formalism of the optical Bloch equations and quantum theory of radiation are applied a composite system consisting of a molecule and a quantized radiation field. The results of simulation of the evolution of the population of the states of the molecule in the case of spontaneous emission are similar for both of these two approaches, but differ significantly in the case of conversion by the molecule of monochromatic radiation. These differences are the greater, the higher the intensity of resonance Rayleigh scattering or (and) relaxed fluorescence, as a result of which the molecule returns to the initial ground state. An explanation of the nature of these differences is given.
Resonant scattering of atoms with formation of the Feshbach resonance in the presence of a laser radiation coupling the levels of two bound atoms (a molecule) is considered. The laser field leads to a second resonance in scattering and broadening of resonances, which facilitates the possibility of experimental observation of asymmetry of the total scattering cross-section arising because of interference between resonant and potential scatterings. The effects associated with interference of the two channels of decay of a bound system of two atoms (a molecule) in the laser field are studied. An expression is obtained for the scattering length in collision of two cold atoms in the field of laser radiation.
Collisions of atoms with formation of Feshbach resonances in the presence of laser field are considered. The elastic and inelastic scattering cross sections are calculated. The laser field leads to second resonance in elastic scattering, broadening of resonances, and arising of interference between resonant and potential scattering. The effects associated with interference of the two channels of decay of bound system of two atoms (a molecule) in laser field are studied. It is shown that if the energy equals that of the lower stable Stark-shifted level plus the energy of two photons, the resonance is quenched. It is also shown that with the increase in two-photon effective interaction the pattern of resonance scattering changes essentially.