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Frontiers in Optics

Controlling Atomic Qubits with Electromagnetic Vortices

Andrei V. Afanasev

Published Jan 1, 2020• 0 citations
Publisher

Abstract

We predict behavior of atomic qubits in response to electromagnetic vortices, known as twisted photons: They can induce △m=±2 transitions between atomic levels and Zeeman sub-levels, while suppressing △m=±1 transitions only allowed for plane waves.
DOI
10.1364/fio.2020.fw5b.1

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A form of quantum control is proposed by applying twisted light, also known as optical vortex beams, to drive ultranarrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg, and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules, reducing simultaneously probe-induced frequency shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis, which opens the $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{0}$ doubly forbidden clock transition with a high $E1M1$ two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the $M2$ magnetic quadrupole $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{2}$ transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment, significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices merged with composite pulses will ultimately benefit experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approaches to atomic interferometry, and precision tests of fundamental theories in physics and high-accuracy optical metrology.

arXiv:2306.17620•Physical Review A•Oct 23, 2023•14 citations
Polarization dependence of the enhancement and suppression of four-wave mixing (FWM) in a multi-Zeeman level atomic system is investigated both theoretically and experimentally.A dressing field applied to the adjacent transition can cause energy level splitting.Therefore, it can control the enhancement and suppression of the FWM processes in the system due to the effect of electromagnetically induced transparency.The results show that the pumping beams with different polarizations select the transitions between different Zeeman levels that, in turn, affect the enhancement and suppression efficiencies of FWM.
Employing an intense laser field coupling to the degenerate two-level system of cesium 6 2S_ 1/2(F=4)- 6 2P_ 3/2(F′=5) transition in a cesium vapor cell, electromagnetically induced absorption (EIA) has been demonstrated via probe absorption spectra, at the same time, electromagnetically induced transparency (EIT) of V-type three-level scheme has been demonstrated on the F=4-F′=3 and F=4-F′=4 transition frequency. The EIA is affected by the intensity and detuning of the coupling laser. By analyzing the effect of optical pumping between Zeeman sub-levels on the EIA and the coherent interactions between multiple degenerate two-level atoms, it is shown that the optical pumping affects the population of different Zeeman sub-levels and the number of the involved two-level atoms, the coherent time between the sub-levels is then changed and the linewidth and intensity of the EIA are affected accordingly.
A form of quantum control is proposed by applying twisted light, also known as optical vortex beams, to drive ultranarrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg, and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules, reducing simultaneously probe-induced frequency shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis, which opens the $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{0}$ doubly forbidden clock transition with a high E1M1E1M1E1M1 two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the M2M2M2 magnetic quadrupole $^{1}S_{0}\ensuremath{\rightarrow}^{3}P_{2}$ transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment, significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices merged with composite pulses will ultimately benefit experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approaches to atomic interferometry, and precision tests of fundamental theories in physics and high-accuracy optical metrology.