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Frontiers in Optics

An Integrated Photonic Platform for Rare-Earth Ions in Thin Film Lithium Niobate

Subhojit Dutta, Elizabeth A. Goldschmidt, Sabyasachi Barik, Uday Saha, Edo Waks A

Published Jan 1, 2020• 7 citations
Publisher

Abstract

We present an integrated photonic platform for rare earth ions in thin film lithium niobate. The ions in the thin film presernve bulk-like optical properties. This paves the pathway for exciting integrated optoelectronic devices in both the classical and quantum regimes.
DOI
10.1364/fio.2020.fw1d.7

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Rare-earth ion ensembles doped in single crystals are a promising materials system with widespread applications in optical signal processing, lasing, and quantum information processing. Incorporating rare-earth ions into integrated photonic devices could enable compact lasers and modulators, as well as on-chip optical quantum memories for classical and quantum optical applications. To this end, a thin film single crystalline wafer structure that is compatible with planar fabrication of integrated photonic devices would be highly desirable. However, incorporating rare-earth ions into a thin film form-factor while preserving their optical properties has proven challenging. We demonstrate an integrated photonic platform for rare-earth ions doped in a single crystalline thin film lithium niobate on insulator. The thin film is composed of lithium niobate doped with Tm 3+ . The ions in the thin film exhibit optical lifetimes identical to those measured in bulk crystals. We show narrow spectral holes in a thin film waveguide that require up to 2 orders of magnitude lower power to generate than previously reported bulk waveguides. Our results pave the way for scalable on-chip lasers, optical signal processing devices, and integrated optical quantum memories.
As an active material with favorable linear and nonlinear optical properties, thin-film lithium niobate has demonstrated its potential in integrated photonics. Integration with rare-earth ions, which are promising candidates for quantum memories and transducers, will enrich the system with new applications in quantum information processing. Here, we investigate the optical properties at 1.5 μm wavelengths of rare-earth ions (Er3+) implanted in thin-film lithium niobate waveguides and micro-ring resonators. Optical quality factors near a million after post-annealing show that ion implantation damage can be repaired. The transition linewidth and fluorescence lifetime of erbium ions are characterized. The ion-cavity coupling is observed through a Purcell enhanced fluorescence from which a Purcell factor of 3.8 ± 0.5, compared with waveguide lifetime, is extracted. This platform is compatible with top-down lithography processes and leads to a scalable path for controlling spin-photon interfaces in photonic circuits.
Quantum photonics provides a powerful toolbox with vast applications ranging from quantum simulation, photonic information processing, all optical universal quantum computation, secure quantum internet as well as quantum enhanced sensing. Many of these applications require the integration of several complex optical elements and material systems which pose a challenge to scalability. It is essential to integrate linear and non-linear photonics on a chip to tackle this issue leading to more compact, high bandwidth devices. In this thesis we demonstrate a pathway to achieving several components in the quantum photonic toolbox on the same integrated photonic platform. We focus particularly on two of the more nontrivial components, a single photon source and an integrated quantum light-matter interface. We address the problem of a scalable, chip integrated, fast single photon source, by using atomically thin layers of 2D materials interfaced with plasmonic waveguides. We further embark on the challenge of creating a new material system by integrating rare earth ions with the emerging commercial platform of thin film lithium niobate on insulator. Rare earth ions have found widespread use in classical and quantum information processing. However, these are traditionally doped in bulk crystals which hinder their scalability. We demonstrate an integrated photonic interface for rare earth ions in thin film lithium niobate that preserves the optical and coherence properties of the ions. This combination of rare earth ions with the chip-scale active interface of thin film lithium niobate opens a plethora of opportunities for compact optoelectronic devices. As an immediate application we demonstrate an integrated optical quantum memory with a rare earth atomic ensemble in the thin film. The new light matter interface in thin film lithium niobate acts as a key enabler in an already rich optical platform representing a significant advancement in the field of integrated quantum photonics.