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Simultaneous Magneto-Optical Trapping of Lithium and Ytterbium Atoms: Towards Production of Ultracold Polar Molecules

Okano, Masayuki

Published Mar 23, 2010• 13 citations
OpenAlex

Abstract

We have successfully implemented the first simultaneous magneto-optical trapping (MOT) of lithium ($^6$Li) and ytterbium ($^{174}$Yb) atoms, towards production of ultracold polar molecules of LiYb. For this purpose, we developed the dual atomic oven which contains both atomic species as an atom source and successfully observed the spectra of the Li and Yb atoms in the atomic beams from the dual atomic oven. We constructed the vacuum chamber including the glass cell with the windows made of zinc selenium (ZnSe) for the CO$_2$ lasers, which are the useful light sources of optical trapping for evaporative and sympathetic cooling. Typical atom numbers and temperatures in the compressed MOT are 7$\times10^3$ atoms, 640 $\mu$K for $^6$Li, 7$\times10^4$ atoms and 60 $\mu$K for $^{174}$Yb, respectively.

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We have successfully implemented the first simultaneous magneto-optical trapping (MOT) of lithium (6^66Li) and ytterbium (174^{174}174Yb) atoms, towards production of ultracold polar molecules of LiYb. For this purpose, we developed the dual atomic oven which contains both atomic species as an atom source and successfully observed the spectra of the Li and Yb atoms in the atomic beams from the dual atomic oven. We constructed the vacuum chamber including the glass cell with the windows made of zinc selenium (ZnSe) for the CO2_22​ lasers, which are the useful light sources of optical trapping for evaporative and sympathetic cooling. Typical atom numbers and temperatures in the compressed MOT are 7×103\times10^3×103 atoms, 640 μ\muμK for 6^66Li, 7×104\times10^4×104 atoms and 60 μ\muμK for 174^{174}174Yb, respectively.
This thesis presents progress toward the production of ultracold CsYb molecules. To this end, an apparatus capable of producing magneto optical traps of Yb and Cs was designed, built and tested. Both atoms are produced in a dual species oven and both slowed to low speeds by a single Zeeman slower. From the Zeeman slower atoms are captured in a dual-species magneto-optical trap. To cool caesium the 852 nm D2 transition is addressed by two lasers for cooling and repump. For ytterbium the 399 nm 1S0 ⇒ 1P1 transition is addressed for the Zeeman slower and the 556 nm 1S0 ⇒ 3P1 transition is addressed for the magneto-optical trap. The 399 nm light is produced by two homebuilt diode lasers in an injection-seeding setup, which can produce up to 100 mW. The 556 nm light is produced from a commercial frequency doubled fiber laser, which can produce up to 260 mW. The Zeeman slower is characterised experimentally for both Cs and Yb, and the results compared to those of a numerical simulation of the slower for Yb. The velocity distribution exiting the slower is very sensitive to the exact magnetic field profile, the laser power and detuning of the laser light. The number of atoms loaded into the magneto-optical trap was investigated as a function of the magnetic field gradient, the laser power and the laser detuning. The capture velocity of the Yb MOT is small because the linewidth of the MOT transition is narrow, and so we investigated the influence of broadening the laser linewidth by adding multiple finely-spaced sidebands to the laser light. After optimisation the caesium MOT trapped 5.5 ×10^8 atoms at 125 ± 4 μK. The ytterbium MOT trapped 4.7 ×10^9 atoms at 81 ± 2 μK. Lastly we demonstrate that both MOTs can be produced in the same vacuum chamber simultaneously.
Integrating two chemically distinct atomic species into a miniaturized, high-flux cold-atom source is a key challenge for modern experiments with ultracold atomic mixtures and polar molecules. Here, we report a compact setup with in-series two-dimensional magneto-optical traps (2D MOTs) that provides high-flux cold lithium and rubidium atoms. Thanks to the efficient short-distance Zeeman slowing, the maximum 3D MOT loading rate of lithium atoms reaches a record value of 6.6 × 10 9 atoms/s at a moderate lithium-oven temperature of 372 degrees Celsius, which is 44 times higher than that without the Zeeman slowing light. The flux of rubidium is also as high as 2.3 × 10 9 atoms/s with the rubidium oven held at room temperature. Meanwhile, the entire vacuum-chamber system, including an ultra-high-vacuum science cell, is within a small volume of 65 × 55 × 70 cm 3 . Our work represents a substantial improvement over traditional bulky and complex dual-species cold-atom setups. It provides a good starting point for the fast production of a double-degenerate lithium-rubidium atomic mixture and large samples of ultracold lithium-rubidium ground-state molecules.
We present a machine built for experiments with ultracold mixtures of strontium and lithium atoms. The machine includes a science vacuum chamber and the relevant laser systems for cooling and trapping the atoms. With this machine, we realize a D2-line compressed magneto-optical trap (MOT) for 6{^6}6Li and a narrow-linewidth 689-nm MOT for 84^{84}84Sr, obtaining ~10910^9109 6{^6}6Li atoms at 700 μμμK and ~10710^7107 84^{84}84Sr atoms at 1.8 μμμK. Such a dual-species MOT provides an ideal starting point for realizing double degenerate mixtures of 6^66Li and Sr atoms.
Integrating two chemically distinct atomic species into a miniaturized, high-flux cold-atom source is a key challenge for modern experiments with ultracold atomic mixtures and polar molecules.Here, we report a compact setup with in-series two-dimensional magneto-optical traps (2D MOTs) that provides high-flux cold lithium and rubidium atoms.Thanks to the efficient short-distance Zeeman slowing, the maximum 3D MOT loading rate of lithium atoms reaches a record value of 6.6 × 10 9 atoms/s at a moderate lithium-oven temperature of 372 degrees Celsius, which is 44 times higher than that without the Zeeman slowing light.The flux of rubidium is also as high as 2.3 × 10 9 atoms/s with the rubidium oven held at room temperature.Meanwhile, the entire vacuum-chamber system, including an ultra-high-vacuum science cell, is within a small volume of 65 × 55 × 70 cm 3 .Our work represents a substantial improvement over traditional bulky and complex dual-species cold-atom setups.It provides a good starting point for the fast production of a double-degenerate lithium-rubidium atomic mixture and large samples of ultracold lithium-rubidium ground-state molecules.
This thesis describes the design and construction of a new apparatus to laser cool and trap Yb and Cs atoms with the ultimate aim of creating ultracold molecules with both an electric and magnetic dipole moment, which are of great interest in a range of fields. The Yb and Cs atomic beams are first generated and overlapped in a dual species oven. A collimated atomic beam of the two species is formed by the use of an array of capillary tubes at the exit of the oven. At this stage the atoms have an average velocity of 311m/s or 264m/s for Yb and Cs respectively, therefore it is necessary to reduce their velocity before they can be trapped in a magneto-optical trap (MOT). This initial stage of slowing is carried out with a Zeeman slower. Due to their atomic properties, Yb and Cs atoms are unable to be slowed by the same magnetic field profile therefore they cannot be loaded simultaneously, however, the Zeeman slower can load the atoms into a MOT sequentially. Once their velocities have been reduced to approximately 48m/s (10m/s) the Cs (Yb) atoms can be captured in a MOT. The laser systems for cooling Yb and Cs are also presented. Laser cooling of Cs is achieved on the D2 transition at 852.3nm whereas Yb can either be cooled on the 1S0 to 1P1 or 1S0 to 3P1 transitions at 398.9nm or 555.8nm respectively. Due to the relative linewidths of these transitions (2π×28.0MHz and 2π × 182.2kHz), Zeeman slowing is performed for Yb on the 1S0 to 1P1 transition and magneto-optical trapping on the 1S0 to 3P1 transition. A Cs MOT with 1 × 10^8 atoms and an Yb MOT with the order of 10^8 atoms on the narrow 556nm transition are demonstrated. The mixture can be sequentially loaded into a dual species MOT, paving the way for many further experiments exploring this novel mixture.
This thesis describes the advances made towards a dual-species magneto-optical trap (MOT) of Li and Rb for use in photoassociation spectroscopy, Feshbach resonance studies, and, as long-term aspirations, the formation of ultracold heteronuclear polar molecules. The initial discussion will focus on a brief theoretical overview of laser cooling and trapping and the production of ultracold molecules from a cold atom source. Subsequently, details of the experimental system, including those pertaining to the required laser light, the vacuum chamber, and the computer control system will be presented. Finally, preliminary optimization and characterization measurements showing the performance of a single species Li MOT are introduced. These measurements demonstrated the loading of over 8 x 107 Li atoms directly into a MOT without the need for a Zeeman slower.