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Magnetic resonance with squeezed microwaves

Audrey Bienfait, Philippe Campagne-Ibarcq, Alexander Holm Kiilerich, Xin Zhou, Probst, S., Jarryd J. Pla, Thomas Schenkel, D. Vion, Esteve, D., John J. L. Morton, Klaus Mølmer, Patrice Bertet

Published Oct 17, 2017• 63 citations
Publisher

Abstract

Vacuum fluctuations of the electromagnetic field set a fundamental limit to the sensitivity of a variety of measurements, including magnetic resonance spectroscopy. We report the use of squeezed microwave fields, which are engineered quantum states of light for which fluctuations in one field quadrature are reduced below the vacuum level, to enhance the detection sensitivity of an ensemble of electronic spins at millikelvin temperatures. By shining a squeezed vacuum state on the input port of a microwave resonator containing the spins, we obtain a 1.2-dB noise reduction at the spectrometer output compared to the case of a vacuum input. This result constitutes a proof of principle of the application of quantum metrology to magnetic resonance spectroscopy.

DOI
10.6082/aw1at-2pf91

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Vacuum fluctuations of the electromagnetic field set a fundamental limit to the sensitivity of a variety of measurements, including magnetic resonance spectroscopy. We report the use of squeezed microwave fields, which are engineered quantum states of light for which fluctuations in one field quadrature are reduced below the vacuum level, to enhance the detection sensitivity of an ensemble of electronic spins at millikelvin temperatures. By shining a squeezed vacuum state on the input port of a microwave resonator containing the spins, we obtain a 1.2-dB noise reduction at the spectrometer output compared to the case of a vacuum input. This result constitutes a proof of principle of the application of quantum metrology to magnetic resonance spectroscopy.
Vacuum fluctuations of the electromagnetic field set a fundamental limit to the sensitivity of a variety of measurements, including magnetic resonance spectroscopy.We report the use of squeezed microwave fields, which are engineered quantum states of light for which fluctuations in one field quadrature are reduced below the vacuum level, to enhance the detection sensitivity of an ensemble of electronic spins at millikelvin temperatures.By shining a squeezed vacuum state on the input port of a microwave resonator containing the spins, we obtain a 1.2-dB noise reduction at the spectrometer output compared to the case of a vacuum input.This result constitutes a proof of principle of the application of quantum metrology to magnetic resonance spectroscopy.
Squeezed states of the electromagnetic field are characterized by a reduction of fluctuations for one of two quadrature phase amplitudes below the level of fluctuations for the vacuum state. This reduction is a manifestly quantum or nonclassical feature which is of great interest in its own right but also potentially important for precision measurement with sensitivity beyond the shot-noise or vacuum-state limit. We describe three different experiments in which squeezed light has been generated in our laboratory involving parametric downconversion, intracavity frequency doubling, and optical bistability with two-state atoms. By employing the squeezed light produced by a subthreshold optical parametric oscillator, we have achieved improvements in sensitivity beyond the vacuum-state limit for the detection of both phase and amplitude changes of the electromagnetic field. An alternate route to sensitivity beyond the vacuum-state limit is through quantum nondemolition measurement, where we have suggested and are implementing a scheme involving parametric conversion and polarization mixing.
Nonclassical states of light are of increasing interest due to their applications in the emerging field of quantum information processing and communication. Squeezed light is such a state of the electromagnetic field in which the quantum noise properties are altered compared with those of coherent light. Squeezed light and squeezed vacuum states are potentially useful for quantum information protocols as well as optical measurements, where sensitivities can be limited by quantum noise. We experimentally study a source of squeezed vacuum resulting from the interaction of near-resonant light with both cold and hot Rb atoms via the nonlinear polarization self-rotation effect (PSR). We investigate the optimal conditions for noise reduction in the resulting squeezed states, reaching quadrature squeezing levels of up to 2.6 dB below shot noise, as well as observing noise reduction for a broad range of detection frequencies, from tens of kHz to several MHz. We use this source of squeezed vacuum at 795 nm to further study the noise properties of these states and how they are affected by resonant atomic interactions. This includes the use of a squeezed light probe to give a quantum enhancement to an optical magnetometer, as well as studying the propagation of squeezed vacuum in an atomic medium under conditions of electromagnetically induced transparency (EIT). We also investigate the propagation of pulses of quantum squeezed light through a dispersive atomic medium, where we examine the possibilities for quantum noise signals traveling at subluminal and superluminal velocities. The interaction of squeezed light with resonant atomic vapors finds various potential applications in both quantum measurements and continuous variable quantum memories.
Squeezed vacuum states of light show a reduction in quantum noise along one quadrature compared to the vacuum state. This characteristic is the key to improve interferometric measurements beyond their quantum noise limitation. In particular for ground-based gravitational wave detectors [1] the application of squeezed light led to a significant sensitivity improvement of up to 6 dB. Future gravitational wave detectors, like the Einstein Telescope [2] or Cosmic Explorer [3], aim for an even higher enhancement in the range of 10 dB with the injection of squeezed states of light into the dark port of their interferometers.
Squeezed light finds many important applications in quantum information science and quantum metrology, and has been produced in a variety of physical systems involving optical non-linear processes. Here, we show how a non-linear magnetostrictive interaction in a ferrimagnet in cavity magnomechanics can be used to reduce quantum noise of the electromagnetic field. We show optimal parameter regimes where a substantial and stationary squeezing of the microwave output field can be achieved. Realization of the scheme is within reach of current technology in cavity electromagnonics and magnomechanics. Our work provides a new and practicable approach for producing squeezed vacuum states of electromagnetic fields, and may find promising applications in quantum information processing and quantum metrology.
Many experiments that interrogate fundamental theories require detectors whose sensitivities are limited by the laws of quantum mechanics.In cavity-based searches for axionic dark matter, vacuum fluctuations in the two quadratures of the cavity electromagnetic field limit the sensitivity to an axion-induced field.In an apparatus designed to partially mimic existing axion detectors, we demonstrate experimentally that such quantum limits can be overcome through the use of squeezed states.By preparing a microwave cavity in a squeezed state and measuring just the squeezed quadrature, we enhance the spectral scan rate by a factor of 2.12 Æ 0.08.This enhancement is in excellent quantitative agreement with a theoretical model accounting for both imperfect squeezing and measurement.