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Vestiges of quantum oscillations in the open evolution of semiclassical states

Alfredo M. Ozorio de Almeida

Published Dec 20, 2017• 0 citations
OpenAlex

Abstract

A single wave component of a quantum particle can in principle be detected by the way that it interferes with itself, that is, through the local wave function correlation. The interpretation as the expectation of a local translation operator allows this measure of quantum wavyness to be followed through the process of decoherence in open quantum systems. This is here assumed to be Markovian, determined by Lindblad operators that are linear in position and momentum. The limitation of small averaging windows and even smaller correlation lengths simplifies the semiclassical theory for the evolving local correlation. Its spectrum has a peak for each classical momentum, subjected to Gaussian broadening with decoherence. These spectral lines can be clearly resolved even after the Wigner function has become positive: The correlations located far from caustics seem to be the last vestige of quantum oscilations.

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Vestiges of quantum oscillations in the open evolution of semiclassical states

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A single wave component of a quantum particle can in principle be detected by the way that it interferes with itself, that is, through the local wave function correlation. The interpretation as the expectation of a local translation operator allows this measure of quantum wavyness to be followed through the process of decoherence in open quantum systems. This is here assumed to be Markovian, determined by Lindblad operators that are linear in position and momentum. The limitation of small averaging windows and even smaller correlation lengths simplifies the semiclassical theory for the evolving local correlation. Its spectrum has a peak for each classical momentum, subjected to Gaussian broadening with decoherence. These spectral lines can be clearly resolved even after the Wigner function has become positive: The correlations located far from caustics seem to be the last vestige of quantum oscilations.

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Vestiges of quantum oscillations in the open evolution of semiclassical states

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A single wave component of a quantum particle can in principle be detected by the way that it interferes with itself, that is, through the local wave function correlation. The interpretation as the expectation of a local translation operator allows this measure of quantum wavyness to be followed through the process of decoherence in open quantum systems. This is here assumed to be Markovian, determined by Lindblad operators that are linear in position and momentum. The limitation of small averaging windows and even smaller correlation lengths simplifies the semiclassical theory for the evolving local correlation. Its spectrum has a peak for each classical momentum, subjected to Gaussian broadening with decoherence. These spectral lines can be clearly resolved even after the Wigner function has become positive: The correlations located far from caustics seem to be the last vestige of quantum oscilations.
A single wave component of a quantum particle can in principle be detected by the way that it interferes with itself, that is, through the local wave function correlation. The interpretation as the expectation of a local translation operator allows this measure of quantum wavyness to be followed through the process of decoherence in open quantum systems. This is here assumed to be Markovian, determined by Lindblad operators that are linear in position and momentum. The limitation of small averaging windows and even smaller correlation lengths simplifies the semiclassical theory for the evolving local correlation. Its spectrum has a peak for each classical momentum, subjected to Gaussian broadening with decoherence. These spectral lines can be clearly resolved even after the Wigner function has become positive: The correlations located far from caustics seem to be the last vestige of quantum oscilations.
Abstract A single wave component of a quantum particle can in principle be detected by the way that it interferes with itself, that is, through the local wave function correlation. The interpretation as the expectation of a local translation operator allows this measure of quantum wavyness to be followed through the process of decoherence in open quantum systems. This is here assumed to be Markovian, determined by Lindblad operators that are linear in position and momentum. The limitation of small averaging windows and even smaller correlation lengths simplifies the semiclassical theory for the evolving local correlation. Its spectrum has a peak for each classical momentum, subjected to Gaussian broadening with decoherence. These spectral lines can be clearly resolved even after the Wigner function has become positive: the correlations located far from caustics seem to be the last vestige of quantum oscilations.
The Lindblad master equation governs the general Markovian evolution of a density operator for an open quantum system. Semiclassical Wigner functions represent density operators in phase space in terms of chords on a classical manifold, so that the amplitude and phase of each chord contribution is classically defined. Inserting such a Wigner function into a phase space version of the master equation, its explicit evolution is derived in the absence of dissipation. There results a simple extension of the unitary evolution of the semiclassical Wigner function, which does not affect the phase of each chord contribution, while dampening its amplitude exponentially. Projecting the Wigner function on to an orthogonal position or momentum basis, the dampening of long chords emerges as the exponential decay of off-diagonal elements of the density matrix.
ABSTRACT: The concept of open quantum system is very broad and it is related to the ability of measuring only certain degree of freedoms of a particular system. Although this idea is relatively simple, the separation between the system of interest, the degree of freedoms that are accesible experimentally, and the reservoir, the degree of freedoms that are not accesible experimentally, is not always clear. For instance, in molecular systems, electronic spectroscopy has access only to electronic degree of freedoms so that the nuclear and vibrational degree of freedom become the reservoir, this makes its description not trivial. This scenario leads to have non-trivial and structured reservoirs and to develop powerful tools to analyze them. The hallmark of non-trivial and structured reservoirs is the non-Markovian dynamics. By translating the Feynman and Vernon influence functional approach into phase-space representation, we develop two theories of semiclassical evolution of the Wigner function of the system of interest that incorporate non-Markovian dynamics and highly non-trivial quantum effects such as non-locality of quantum mechanics: (i) We translate the Caldeira-Leggett model into phase-space representation of quantum mechanics and (ii) we consider the possibility of having non-linear baths and therefore, truly quantum reservoirs. During the last forty years the study of energy loss and coherence in quantum systems has been based on the Ullersma-Caldeira-Leggett model, a model that describes the environment of quantum systems of interest as a collection of harmonic oscillators with classical evolution. We constructed this model in the Wigner-Weyl representation of quantum mechanics and discuss the classical nature of the evolution of the bath modes and the semiclassical evolution of the central system. As an application of the semiclassical Wigner propagator, the non-Markovian time evolution under the Morse potencial is analyzed. There, it is clear how decohering processes shrink the propagator to smaller regions of phase space implying that the dynamics become more local, i.e., more classical. The current level of experimentation and control of physical systems have called into question the validity of the model in, one hand, molecular systems (e.g. photosynthetic complexes immersed in solvents, chemical systems in liquid phase or gas and manipulated with intense laser pulses) and, in the other hand, solid state systems (e.g. Josephson junctions, spins in quantum dots or "spinning ice"). Given the importance of these systems in the development of new quantum technologies and in the understanding of quantum phenomena in mesoscopic systems, it has become necessary to develop new models of the environment and efficient methodologies with quantitative prediction power. However, some of them are artificial modifications of the Ullersma-Caldeira-Leggett model without solid and clean physical support. Here we formulated a general framework that allows the study of quantum correlations in quantum systems in the presence of non-harmonic thermal baths (e.g. baths formed by strongly coupled diatomic molecules). This formulation will allow a more precise and quantitative description of processes such as the transport of excitons in photosynthetic complexes, the transfer of heat in solid state devices, among others. Results clearly show the non-classical time dynamics of the bath modes. The implementation of this particular theory remains, however, as a challenge.
A proposal for obtaining predictions of correlations between positions and momenta from the peaks of the Wigner function is studied. An implementation of this proposal based on approximate Wigner functions of a special form obtained from semiclassical wave functions is shown to be unreliable because the exact Wigner functions do not have this form. This approach has been used to argue that classical general relativity is predicted from the semiclassical wave function of the Universe, and this must now be reconsidered. A new measure of correlation, involving projection onto coherent states, is proposed for predicting classical correlations from a general Wigner function. In the harmonic oscillator, it predicts a correlation of position and momentum given by the Hamiltonian equated to the classical energy.
We challenge the standard picture of decohering Schrödinger cat states as an ensemble average obeying a Lindblad master equation, brought about locally from an irreversible interaction with an environment. We generate self-consistent collections of pure system states correlated with specific environmental records, corresponding to the function of the wave-particle correlator first introduced in Carmichael et al. [ Phys. Rev. Lett. 85 (2000)]. In the spirit of Carmichael et al. [in Coherent States: Past, Present and Future , World Scientific, 1994], we find that the complementary unravelings evince a pronounced disparity when the “position” and “momentum” of the damped cavity mode — an explicitly open quantum system — are measured. Intensity-field correlations may largely deviate from a monotonic decay, while Wigner functions of the cavity state display contrasting manifestations of quantum interference when conditioned on photon counts sampling a continuous photocurrent. In turn, the conditional photodetection events mark the contextual diffusion of both the net charge generated at the homodyne detector, and the electromagnetic field amplitude in the resonator.