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CONTINUOUS-TIME QUANTUM WALKS AND TRAPPING

Elena Agliari, Oliver M Ülken, A. Blumen, Theoretische Polymerphysik, Universität Freiburg

Published Nov 20, 2012• 21 citations
OpenAlex

Abstract

Recent findings suggest that processes such as the electronic energy transfer through the photosynthetic antenna display quantal features, aspects known from the dynamics of charge carriers along polymer backbones. Hence, in modeling energy transfer one has to leave the classical, masterequation-type formalism and advance towards an increasingly quantum-mechanical picture, while still retaining a local description of the complex network of molecules involved in the transport, say through a tight-binding approach. Interestingly, the continuous time random walk (CTRW) picture, widely employed in describing transport in random environments, can be mathematically reformulated to yield a quantummechanical Hamiltonian of tight-binding type; the procedure uses the mathematical analogies between time-evolution operators in statistical and in quantum mechanics: The result are continuoustime quantum walks (CTQWs). However, beyond these formal analogies, CTRWs and CTQWs display vastly different physical properties. In particular, here we focus on trapping processes on a ring and show, both analytically and numerically, that distinct configurations of traps (ranging from periodical to random) yield strongly different behaviours for the quantal mean survival probability, while classically (under ordered conditions) we always find an exponential decay at long times.

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Recent findings suggest that processes such as the electronic energy transfer through the photosynthetic antenna display quantal features, aspects known from the dynamics of charge carriers along polymer backbones. Hence, in modeling energy transfer one has to leave the classical, masterequation-type formalism and advance towards an increasingly quantum-mechanical picture, while still retaining a local description of the complex network of molecules involved in the transport, say through a tight-binding approach. Interestingly, the continuous time random walk (CTRW) picture, widely employed in describing transport in random environments, can be mathematically reformulated to yield a quantummechanical Hamiltonian of tight-binding type; the procedure uses the mathematical analogies between time-evolution operators in statistical and in quantum mechanics: The result are continuoustime quantum walks (CTQWs). However, beyond these formal analogies, CTRWs and CTQWs display vastly different physical properties. In particular, here we focus on trapping processes on a ring and show, both analytically and numerically, that distinct configurations of traps (ranging from periodical to random) yield strongly different behaviours for the quantal mean survival probability, while classically (under ordered conditions) we always find an exponential decay at long times.
Recent findings suggest that processes such as the excitonic energy transfer through the photosynthetic antenna display quantal features, aspects known from the dynamics of charge carriers along polymer backbones. Hence, in modeling energy transfer one has to leave the classical, master-equation-type formalism and advance towards an increasingly quantum-mechanical picture, while still retaining a local description of the complex network of molecules involved in the transport, say through a tight-binding approach. Interestingly, the continuous time random walk (CTRW) picture, widely employed in describing transport in random environments, can be mathematically reformulated to yield a quantum-mechanical Hamiltonian of tight-binding type; the procedure uses the mathematical analogies between time-evolution operators in statistical and in quantum mechanics: The result are continuous-time quantum walks (CTQWs). However, beyond these formal analogies, CTRWs and CTQWs display vastly different physical properties. In particular, here we focus on trapping processes on a ring and show, both analytically and numerically, that distinct configurations of traps (ranging from periodical to random) yield strongly different behaviors for the quantal mean survival probability, while classically (under ordered conditions) we always find an exponential decay at long times.
Continuous time quantum walks (CTQWs) do not necessarily perform better than their classical counterparts, the continuous time random walks (CTRWs). For one special graph, where a recent analysis showed that in a particular direction of propagation the penetration of the graph is faster by CTQWs than by CTRWs, we demonstrate that in another direction of propagation the opposite is true. In this case a CTQW initially localized at one site displays a slow transport. We furthermore show that when the CTQW's initial condition is a totally symmetric superposition of states of equivalent sites, the transport gets to be much more rapid.
We model quantum transport, described by continuous-time quantum walks (CTQWs), on deterministic Sierpinski fractals, differentiating between Sierpinski gaskets and Sierpinski carpets, along with their dual structures. The transport efficiencies are defined in terms of the exact and the average return probabilities, as well as by the mean survival probability when absorbing traps are present. In the case of gaskets, localization can be identified already for small networks (generations). For carpets, our numerical results indicate a trend towards localization, but only for relatively large structures. The comparison of gaskets and carpets further implies that, distinct from the corresponding classical continuous-time random walk, the spectral dimension does not fully determine the evolution of the CTQW.
In the quest for signatures of coherent transport we consider exciton trapping in the continuous-time quantum walk framework. The survival probability displays different decay domains, related to distinct regions of the spectrum of the Hamiltonian. For linear systems and at intermediate times the decay obeys a power law, in contrast with the corresponding exponential decay found in incoherent continuous-time random walk situations. To differentiate between the coherent and incoherent mechanisms, we present an experimental protocol based on a frozen Rydberg gas structured by optical dipole traps.
Abstract What happens when a quantum system undergoing unitary evolution in time is subject to repeated projective measurements to the initial state at random times? A question of general interest is: how does the survival probability S m , namely, the probability that an initial state survives even after m number of measurements, behave as a function of m ? We address these issues in the context of two paradigmatic quantum systems, one, the quantum random walk evolving in discrete time, and the other, the tight-binding model evolving in continuous time, with both defined on a one-dimensional periodic lattice with a finite number of sites N . For these two models, we present several numerical and analytical results that hint at the curious nature of quantum measurement dynamics. In particular, we unveil that when evolution after every projective measurement continues with the projected component of the instantaneous state, the average and the typical survival probability decay as an exponential in m for large m . By contrast, if the evolution continues with the leftover component, namely, what remains of the instantaneous state after a measurement has been performed, the survival probability exhibits two characteristic m values, namely, m 1 ⋆ ( N ) ∼ N and m 2 ⋆ ( N ) ∼ N δ with δ > 1. These scales are such that (i) for m large and satisfying m < m 1 ⋆ ( N ) , the decay of the survival probability is as m −2 , (ii) for m satisfying m 1 ⋆ ( N ) ≪ m < m 2 ⋆ ( N ) , the decay is as m −3/2 , while (iii) for m ≫ m 2 ⋆ ( N ) , the decay is as an exponential. The results for the dynamics with the leftover component, already known for the case of measurements at regular intervals, are being extended here to the case of measurements at random intervals. We find that our results hold independently of the choice of the distribution of times between successive measurements, as have been corroborated by our resu
We study the coherent exciton transport of continuous-time quantum walks (CTQWs) on Erdos-Renyi networks. The Erdos-Renyi network of N nodes is constructed by connecting every pair of nodes with probability ppp. We numerically calculate the ensemble averaged transition probability of quantum transport between two nodes of the networks. For finite networks, we find that the limiting transition probability is reached very quickly. For infinite networks whose spectral density follows the semicircle law, the efficiencies of the classical and quantum-mechanical transport are compared on networks of different average degree. In the long time limiting, we consider the distribution of the ensemble averaged transition probabilities, and show that there is a high probability to find the exciton at the initial node. Such high return probability almost do not alter in a wide range of connection probability p but increases rapidly when the network approaches to be fully connected. For networks whose topology is not extremely connected, the return probability is inversely proportional to the network size N. Furthermore, the transport dynamics are compared with that on a random graph model in which the degree of each node equals to the average degree of the Erdos-Renyi networks.