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Magnetization plateaux in an extended Shastry-Sutherland model

Kai Phillip Schmidt, Julien Dorier, Frédéric Mila

Published Nov 20, 2012• 3 citations
OpenAlex

Abstract

Abstract. We study an extended two-dimensional Shastry-Sutherland model in a magnetic field where besides the usual Heisenberg exchanges of the Shastry-Sutherland model two additional SU(2) invariant couplings are included. Perturbative continous unitary transformations are used to determine the leading order effects of the additional couplings on the pure hopping and on the long-range interactions between the triplons which are the most relevant terms for small magnetization. We then compare the energy of various magnetization plateaux in the classical limit and we discuss the implications for the two-dimensional quantum magnet SrCu2(BO3)2. 1.

Related papers

Magnetization plateaux in an extended Shastry-Sutherland model

Kai Phillip Schmidt, Julien Dorier, Frédéric Mila

We study an extended two-dimensional Shastry-Sutherland model in a magnetic field where besides the usual Heisenberg exchanges of the Shastry-Sutherland model two additional SU(2) invariant couplings are included. Perturbative continous unitary transformations are used to determine the leading order effects of the additional couplings on the pure hopping and on the long-range interactions between the triplons which are the most relevant terms for small magnetization. We then compare the energy of various magnetization plateaux in the classical limit and we discuss the implications for the two-dimensional quantum magnet SrCu 2 (BO 3 ) 2 .

arXiv:0810.1596•Journal of Physics Conference Series•Jan 1, 2009•3 citations

Theory of Magnetization Plateaux in the Shastry-Sutherland Model

Julien Dorier, Kai Phillip Schmidt, Frédéric Mila

Motivated by the remarkable properties of SrCu2(BO3) 2 in a magnetic field, we use perturbative continuous unitary transformations to determine the magnetization plateaux of the Shastry-Sutherland model, unveiling an unexpected sequence of plateaux progressively appearing at 2/9, 1/6, 1/9, and 2/15 upon increasing the interdimer coupling. We predict that a 1/6 plateau should be present in SrCu2(BO3)2, even if residual interactions beyond the Shastry-Sutherland are strong enough to modify the other plateaux below 1/3. The method is extended to calculate the magnetization profile within the plateaux, leading to a local structure around triplons that agrees with NMR results on SrCu2(BO3) 2.

arXiv:0806.3406•Physical Review Letters•Dec 19, 2008•94 citations

Fractional magnetization plateaux of a spin-1/2 Heisenberg model on the Shastry-Sutherland lattice: effect of quantum XY interdimer coupling

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Spin-1/2 Heisenberg model on the Shastry-Sutherland lattice is considered within the many-body perturbation theory developed from the exactly solved spin-1/2 Ising-Heisenberg model with the Heisenberg intradimer and Ising interdimer interactions. The former model is widely used for a description of magnetic properties of the layered compound SrCu _2 2 (BO _3 3 ) _2 2 , which exhibits a series of fractional magnetization plateaux at sufficiently low temperatures. Using the novel type of many-body perturbation theory we have found the effective model of interacting triplet excitations with the extended hard-core repulsion, which accurately recovers 1/8, 1/6 and 1/4 magnetization plateaux for moderate values of the interdimer coupling. A possible existence of a striking quantum phase of bound triplons is also revealed at low enough magnetic fields.

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Local Physics of Magnetization Plateaux in the Shastry-Sutherland Model

Леонид Исаев, Gerardo Ortíz, J. Dukelsky

We address the physical mechanism responsible for the emergence of magnetization plateaux in the Shastry-Sutherland model. By using a hierarchical mean-field approach, we demonstrate that a plateau is stabilized in a certain spin pattern, satisfying local commensurability conditions derived from our formalism. Our results provide evidence in favor of a robust local physics nature of the plateaux states and are in agreement with recent NMR experiments on SrCu2(BO3)2.

arXiv:0906.4991•Physical Review Letters•Oct 21, 2009•22 citations

Exact ground states of a spin- 12 Ising-Heisenberg model on the Shastry-Sutherland lattice in a magnetic field

Taras Verkholyak, Jozef Strečka, Frédéric Mila +1 more

Exact ground states of a spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice with Heisenberg intradimer and Ising interdimer couplings are found by two independent rigorous procedures. The first method uses a unitary transformation to establish a mapping correspondence with an effective classical spin model, while the second method relies on the derivation of an effective hard-core boson model by continuous unitary transformations. Both methods lead to equivalent effective Hamiltonians providing a convincing proof that the spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice exhibits a zero-temperature magnetization curve with just two intermediate plateaus at one-third and one-half of the saturation magnetization, which correspond to stripe and checkerboard orderings of singlets and polarized triplets, respectively. The nature of the remarkable stripe order relevant to the one-third plateau is thoroughly investigated with the help of the corresponding exact eigenvector. The rigorous results for the spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice are compared with the analogous results for the purely classical Ising and fully quantum Heisenberg models. Finally, we discuss to what extent the critical fields of ${\mathrm{SrCu}}_{2}{(\mathrm{BO}}_{3}){}_{2}$ and ${(\mathrm{CuCl})\mathrm{Ca}}_{2}{\mathrm{Nb}}_{3}{\mathrm{O}}_{10}$ can be described within the suggested Ising-Heisenberg model.

arXiv:1407.8229•Physical Review B•Oct 16, 2014•26 citations

Exotic magnetization plateaus in a quasi-two-dimensional Shastry-Sutherland model

G. R. Foltin, Salvatore R. Manmana, Kai Phillip Schmidt

We find unconventional Mott insulators in a quasi-2D version of the Shastry-Sutherland model in a magnetic field. In our realization on a four-leg tube geometry, these are stabilized by correlated hopping of localized magnetic excitations. Using perturbative continuous unitary transformations (pCUTs, plus classical approximation or exact diagonalization) and the density matrix renormalisation group method (DMRG), we identify prominent magnetization plateaus at magnetizations $M=1/8,3/16,1/4$, and $1/2$. While the plateau at $M=1/4$ can be understood in a semiclassical fashion in terms of diagonal stripes, the plateau at $M=1/8$ displays highly entangled wheels in the transverse direction of the tube. Finally, the $M=3/16$ plateau is most likely to be viewed as a classical 1/8 structure on which additional triplets are fully delocalized around the tube. The classical approximation of the effective model fails to describe all these plateau structures which benefit from correlated hopping. We relate our findings to the full 2D system, which is the underlying model for the frustrated quantum magnet $\mathrm{SrCu}{({\mathrm{BO}}_{3})}_{2}$.

arXiv:1405.3260•Physical Review B•Sep 3, 2014•23 citations
Abstract. We study an extended two-dimensional Shastry-Sutherland model in a magnetic field where besides the usual Heisenberg exchanges of the Shastry-Sutherland model two additional SU(2) invariant couplings are included. Perturbative continous unitary transformations are used to determine the leading order effects of the additional couplings on the pure hopping and on the long-range interactions between the triplons which are the most relevant terms for small magnetization. We then compare the energy of various magnetization plateaux in the classical limit and we discuss the implications for the two-dimensional quantum magnet SrCu2(BO3)2. 1.
We study an extended two-dimensional Shastry-Sutherland model in a magnetic field where besides the usual Heisenberg exchanges of the Shastry-Sutherland model two additional SU(2) invariant couplings are included. Perturbative continous unitary transformations are used to determine the leading order effects of the additional couplings on the pure hopping and on the long-range interactions between the triplons which are the most relevant terms for small magnetization. We then compare the energy of various magnetization plateaux in the classical limit and we discuss the implications for the two-dimensional quantum magnet SrCu 2 (BO 3 ) 2 .
Motivated by the remarkable properties of SrCu2(BO3) 2 in a magnetic field, we use perturbative continuous unitary transformations to determine the magnetization plateaux of the Shastry-Sutherland model, unveiling an unexpected sequence of plateaux progressively appearing at 2/9, 1/6, 1/9, and 2/15 upon increasing the interdimer coupling. We predict that a 1/6 plateau should be present in SrCu2(BO3)2, even if residual interactions beyond the Shastry-Sutherland are strong enough to modify the other plateaux below 1/3. The method is extended to calculate the magnetization profile within the plateaux, leading to a local structure around triplons that agrees with NMR results on SrCu2(BO3) 2.
Spin-1/2 Heisenberg model on the Shastry-Sutherland lattice is considered within the many-body perturbation theory developed from the exactly solved spin-1/2 Ising-Heisenberg model with the Heisenberg intradimer and Ising interdimer interactions. The former model is widely used for a description of magnetic properties of the layered compound SrCu _2 2 (BO _3 3 ) _2 2 , which exhibits a series of fractional magnetization plateaux at sufficiently low temperatures. Using the novel type of many-body perturbation theory we have found the effective model of interacting triplet excitations with the extended hard-core repulsion, which accurately recovers 1/8, 1/6 and 1/4 magnetization plateaux for moderate values of the interdimer coupling. A possible existence of a striking quantum phase of bound triplons is also revealed at low enough magnetic fields.
Exact ground states of a spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice with Heisenberg intradimer and Ising interdimer couplings are found by two independent rigorous procedures. The first method uses a unitary transformation to establish a mapping correspondence with an effective classical spin model, while the second method relies on the derivation of an effective hard-core boson model by continuous unitary transformations. Both methods lead to equivalent effective Hamiltonians providing a convincing proof that the spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice exhibits a zero-temperature magnetization curve with just two intermediate plateaus at one-third and one-half of the saturation magnetization, which correspond to stripe and checkerboard orderings of singlets and polarized triplets, respectively. The nature of the remarkable stripe order relevant to the one-third plateau is thoroughly investigated with the help of the corresponding exact eigenvector. The rigorous results for the spin-1/2 Ising-Heisenberg model on the Shastry-Sutherland lattice are compared with the analogous results for the purely classical Ising and fully quantum Heisenberg models. Finally, we discuss to what extent the critical fields of SrCu2(BO3)2{\mathrm{SrCu}}_{2}{(\mathrm{BO}}_{3}){}_{2}SrCu2​(BO3​)2​ and (CuCl)Ca2Nb3O10{(\mathrm{CuCl})\mathrm{Ca}}_{2}{\mathrm{Nb}}_{3}{\mathrm{O}}_{10}(CuCl)Ca2​Nb3​O10​ can be described within the suggested Ising-Heisenberg model.
We find unconventional Mott insulators in a quasi-2D version of the Shastry-Sutherland model in a magnetic field. In our realization on a four-leg tube geometry, these are stabilized by correlated hopping of localized magnetic excitations. Using perturbative continuous unitary transformations (pCUTs, plus classical approximation or exact diagonalization) and the density matrix renormalisation group method (DMRG), we identify prominent magnetization plateaus at magnetizations M=1/8,3/16,1/4M=1/8,3/16,1/4M=1/8,3/16,1/4, and 1/21/21/2. While the plateau at M=1/4M=1/4M=1/4 can be understood in a semiclassical fashion in terms of diagonal stripes, the plateau at M=1/8M=1/8M=1/8 displays highly entangled wheels in the transverse direction of the tube. Finally, the M=3/16M=3/16M=3/16 plateau is most likely to be viewed as a classical 1/8 structure on which additional triplets are fully delocalized around the tube. The classical approximation of the effective model fails to describe all these plateau structures which benefit from correlated hopping. We relate our findings to the full 2D system, which is the underlying model for the frustrated quantum magnet SrCu(BO3)2\mathrm{SrCu}{({\mathrm{BO}}_{3})}_{2}SrCu(BO3​)2​.