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Decoherence and Dissipation in Quantum Two-State Systems

M. Grigorescu

Published Jan 1, 1997• 7 citations
OpenAlex

Abstract

: The Brownian dynamics of the density operator for a quantum system interacting with a classical heat bath is described using a stochastic, non-linear Liouville equation obtained from a variational principle. The rate of the noise-induced transitions is expressed as a function of the environmental spectral density, and is discussed for the case of white noise and blackbody radiation. The time-scale of decoherence and dissipation is obtained numerically for a system of two quantum states. These are the ground and first excited state of the center of mass vibrations for a single ion confined in a harmonic trap. PACS numbers: 42.50.Lc,05.40.+j,32.80.Pj 1 Introduction The evolution of a quantum system surrounded by a thermal environment represents a fundamental problem of the quantum theory, increasingly important for applications. In the classical mechanics, a particle interacting with a heat bath has a Brownian evolution towards thermalization, which reduces to a purely dissipative moti...

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: The Brownian dynamics of the density operator for a quantum system interacting with a classical heat bath is described using a stochastic, non-linear Liouville equation obtained from a variational principle. The rate of the noise-induced transitions is expressed as a function of the environmental spectral density, and is discussed for the case of white noise and blackbody radiation. The time-scale of decoherence and dissipation is obtained numerically for a system of two quantum states. These are the ground and first excited state of the center of mass vibrations for a single ion confined in a harmonic trap. PACS numbers: 42.50.Lc,05.40.+j,32.80.Pj 1 Introduction The evolution of a quantum system surrounded by a thermal environment represents a fundamental problem of the quantum theory, increasingly important for applications. In the classical mechanics, a particle interacting with a heat bath has a Brownian evolution towards thermalization, which reduces to a purely dissipative moti...
Classical Brownian motion has well been investigated since the pioneering work of Einstein, which inspired mathematicians to lay the theoretical foundation of stochastic processes. A stochastic formulation for quantum dynamics of dissipative systems described by the system-plus-bath model has been developed and found many applications in chemical dynamics, spectroscopy, quantum transport, and other fields. This article provides a tutorial review of the stochastic formulation for quantum dissipative dynamics. The key idea is to decouple the interaction between the system and the bath by virtue of the Hubbard-Stratonovich transformation or Itô calculus so that the system and the bath are not directly entangled during evolution, rather they are correlated due to the complex white noises introduced. The influence of the bath on the system is thereby defined by an induced stochastic field, which leads to the stochastic Liouville equation for the system. The exact reduced density matrix can be calculated as the stochastic average in the presence of bath-induced fields. In general, the plain implementation of the stochastic formulation is only useful for short-time dynamics, but not efficient for long-time dynamics as the statistical errors go very fast. For linear and other specific systems, the stochastic Liouville equation is a good starting point to derive the master equation. For general systems with decomposable bath-induced processes, the hierarchical approach in the form of a set of deterministic equations of motion is derived based on the stochastic formulation and provides an effective means for simulating the dissipative dynamics. A combination of the stochastic simulation and the hierarchical approach is suggested to solve the zero-temperature dynamics of the spin-boson model. This scheme correctly describes the coherent-incoherent transition (Toulouse limit) at moderate dissipation and predicts a rate dynamics in the overdamped regime. Challenging problems such as the dynamical description of quantum phase transition (local- ization) and the numerical stability of the trace-conserving, nonlinear stochastic Liouville equation are outlined.
For the purpose of understanding the quantum behavior such as quantum decoherence, fluctuations, dissipation, entanglement and teleportation of a mesoscopic or macroscopic object interacting with a general environment, we derive here a set of exact master equations for the reduced density matrix of N interacting harmonic oscillators in a heat bath with arbitrary spectral density and temperature. For the case N = 2, we also give an influence functional treatment of this model and provide explicit expressions for the evolution operator of the reduced density matrix which are useful for the study of decoherence and disentanglement issues. We show a simple application of this master equation by examining the decoherence and disentanglement of two harmonic oscillators due to their interaction with a common environment under Markovian approximation. Two classes of problems of interest to us which these equations can be usefully applied to are that of the quantum dynamics of nanoelectromechanical oscillators and the entanglement evolution of multi-partite macroscopic states such as quantum superposition of mirrors in a high Q cavity. To address a key conceptual issue for macroscopic quantum phenomena we examine the conditions for an assumption often implicitly made in these studies to be valid, namely, that the quantum behavior of a macroscopic object in an environment can be accurately represented by only treating the dynamics of its center-of-mass variable. We also mention how these results can be used to calculate the uncertainty principle governing a macroscopic object at finite temperature.
We derive and analyze the Born-Markov master equation for a quantum harmonic oscillator interacting with a bath of independent two-level systems. This hitherto virtually unexplored model plays a fundamental role as one of the four ``canonical'' system-environment models for decoherence and dissipation. To investigate the influence of further couplings of the environmental spins to a dissipative bath, we also derive the master equation for a harmonic oscillator interacting with a single spin coupled to a bosonic bath. Our models are experimentally motivated by quantum-electromechanical systems and micron-scale ion traps. Decoherence and dissipation rates are found to exhibit temperature dependencies significantly different from those in quantum Brownian motion. In particular, the systematic dissipation rate for the central oscillator decreases with increasing temperature and goes to zero at zero temperature, but there also exists a temperature-independent momentum-diffusion (heating) rate.
In the frames of classical mechanics the generalized Langevin equation is derived for an arbitrary mechanical subsystem coupled to the harmonic bath of a solid. A time-acting temperature operator is introduced for the quantum Klein-Kramers and Smoluchowski equations, accounting for the effect of the quantum thermal bath oscillators. The model of Brownian emitters is theoretically studied and the relevant evolutionary equations for the probability density are derived. The Schrodinger equation is explained via collisions of the target point particles with the quantum force carriers, transmitting the fundamental interactions between the point particles. Thus, electrons and other point particles are no waves and the wavy chapter of quantum mechanics originated for the force carriers. A stochastic Lorentz-Langevin equation is proposed to describe the underlaying Brownian-like motion of the point particles in quantum mechanics. Considering the Brownian dynamics in the frames of the Bohmian mechanics, the density functional Bohm-Langevin equation is proposed, and the relevant Smoluchowski-Bohm equation is derived. A nonlinear master equation is proposed by proper quantization of the classical Klein-Kramers equation. Its equilibrium solution in the exact canonical Gibbs density operator, while the well-known Caldeira-Leggett equation is simply a linearization at high temperature. In the case of a free quantum Brownian particles, a new law for the spreading of the wave packet it discovered, which represents the quantum generalization of the classical Einstein law of Brownian motion. A new projector operator is proposed for the collapse of the wave function of a quantum particle moving in a classical environment. Its application results in dissipative Schrodinger equations, as well as in a new form of dissipative Liouville equation in classical mechanics.
We consider a model of environment-induced dissipationless decoherence of a quantum system where the system is coupled to the bath degrees of freedom via the system Hamiltonian itself. We solve exactly for the reduced density operator of the system for an arbitrary spectral density of the thermal bath and also write down an exact master equation in the Lindblad form. We compare and contrast the above results with those obtained by considering the system frequencies to be randomly modulated as in stochastic models. We observe that a coupling to the bath as above necessarily induces a Kerr-like coherent contribution in the reduced dynamics of the system. This Kerr-like term is a reflection of the quantum nature of the bath and cannot be obtained from stochastic models. For the special case of a harmonic oscillator we consider the influence of decoherence and its relation with phase diffusion. Our numerical results exhibit oscillations in the evolution of system variables which overall is a signature of the quantum nature of the environment.
Quantum systems are unavoidably open to their surrounding degrees of freedom. The theory of open quantum systems is thus crucial to understanding the fluctuations, dissipation, and decoherence of a quantum system of interest. Typically, the bath is modeled as an ensemble of harmonic oscillators, which yields Gaussian statistics of the bath influence on the quantum systems. However, there are also phenomena in which the bath consists of two-state systems, spins, or anharmonic oscillators; therefore, the non-Gaussian properties of the bath become important. Nevertheless, a theoretical framework to describe quantum systems under the influence of such non-Gaussian baths is not well established. Here, we develop a theory to describe quantum dissipative systems affected by Poisson noise properties of the bath, because the Lévi-Itô decomposition theorem asserts that Poisson noise is fundamental in describing arbitrary white noise beyond Gaussian properties. We introduce a quantum bath model that allows for the consistent description of dissipative quantum systems. The obtained master equation reveals non-Gaussian bath effects in the white noise regime, and provides an essential step toward describing open quantum dynamics under the influence of generic baths.