This thesis is devoted to the study of strongly correlated electron systems in two spatial dimensions. The main perspective used in this work is that of scaling, implemented by the renormalization group formalism. This thesis can be divided into three main parts. The first part, comprised of chapters 2-5, investigates various aspects of two dimensional insulating quantum antiferromagnets. In particular, chapters 2-4 deal with the phase transition between an ordered antiferromagnet and a valence bond solid on a square lattice. This transition falls outside the conventional Landau-Ginzburg-Wilson paradigm and is described by a so-called “deconfined ” quantum critical point. In chapter 2, we present an elegant calculation of the scaling dimension of the valence bond solid order parameter at this quantum critical point. Chapters 3 and 4 investigate signatures of deconfined criticality in the response of an antiferromagnet to non-magnetic impurities. Chapter 5 describes the edge response of a conventional ordered square-lattice antiferromagnet. The second part of this thesis, comprised of chapters 6 and 7, studies the subject
This thesis is devoted to the study of strongly correlated electron systems in two spatial dimensions. The main perspective used in this work is that of scaling, implemented by the renormalization group formalism. This thesis can be divided into three main parts. The first part, comprised of chapters 2-5, investigates various aspects of two dimensional insulating quantum antiferromagnets. In particular, chapters 2-4 deal with the phase transition between an ordered antiferromagnet and a valence bond solid on a square lattice. This transition falls outside the conventional Landau-Ginzburg-Wilson paradigm and is described by a so-called “deconfined ” quantum critical point. In chapter 2, we present an elegant calculation of the scaling dimension of the valence bond solid order parameter at this quantum critical point. Chapters 3 and 4 investigate signatures of deconfined criticality in the response of an antiferromagnet to non-magnetic impurities. Chapter 5 describes the edge response of a conventional ordered square-lattice antiferromagnet. The second part of this thesis, comprised of chapters 6 and 7, studies the subject
Strongly correlated low-dimensional quantum spin models provide a well-established frame- \nwork to study magnetic properties of insulators, and are of great theoretical interest and experimental relevance in condensed-matter physics. In this thesis, I use quantum Monte Carlo methods to numerically study quantum critical behavior in low-dimensional quantum spin models and wavefunctions. \n \nFirst, I study spinons &ndash emergent spin-1/2 bosonic excitations &ndash at certain one- and two-dimensional quantum phase transitions (QPTs) in spin models, by characterizing their size and confinement length quantitatively. In particular, I focus on the QPT from an antiferromagnetic (AFM) phase into a valence-bond solid (VBS) phase, which is an example of a violation of the standard Landau-Ginzburg-Wilson paradigm for phase transitions. This transition in two dimensions (2D) is instead likely described by a novel theory called "deconfined quantum criticality" (DQC). According to the theory, spinons should be deconfined. The degree of deconfinement is quantified in my calculations. \n \nSecond, I present a comprehensive study of so-called short-bond resonating-valence-bond (RVB) spin liquids in 2D, which have been suggested as a good starting point for understanding the spin physics of high-temperature cuprates. I find that these RVB states can also be classified as quantum-critical VBS states, which indicates that RVB is less disordered than expected. This work suggests a possible mapping from the quantum RVB states to classical dimer models via a classical continuum field theory--the height model. This map explicitly bridges well-established classical results to future quantum studies. \n \nThird, I consider 1D amplitude product (AP) states, which are generalized versions of RVB states, with different wavefunction weightings of bonds according to their lengths. AP states constitute a good ansatz for certain Hamiltonians and are of broad interest in quantum magnetism. I study phase transitions from AFM-VBS phases in AP states by tuning their amplitudes, and obtain continuously varying critical exponents. In addition, I classify the 1D AP states through entanglement entropy calculations of the central charge in (1+1)D conformal field theory. This new classification could serve as guide for AP states as trial wavefunctions to search for ground states of corresponding quantum spin models.
We study a number of quantum phase transitions, which are exotic in their nature and separates non-trivial phases of matter. Since quantum fluctuations, which drive these phase transitions, are stronger in low-dimensions, we concentrate on low-dimensional systems. We consider two different two-dimensional systems in this thesis and study their phase transition. \n\nFirst, we investigate a phase transition in graphene, one of the most famous two-dimensional systems in condensed matter. For a suspended bilayer graphene in ν = 0 quantum Hall regime, the conductivity data and mean-field analysis suggests a phase transition from an antiferromagnetic (AF) state to a valence bond solid (VBS) state, when perpendicular electric field is increased. This AF to VBS phase transition is reminiscent of deconfined criticality, which is a novel phase transition that cannot be explained by Landau’s theory of symmetry breaking. We show that in the strong coupling regime of bilayer graphene, the AF state is destabilized by the transverse electric field, likely resulting in a VBS state. We also consider monolayer and bilayer graphene in the large cyclotron gap limit and show that the effective action for the AF and VBS order parameters have a topological Wess-Zumino-Witten term, supporting that the phase transition observed in experiments is in the deconfined criticality class. \n\nSecond, we study the model systems of cuprate superconductor, which is effectively a two-dimensionalal system in the CuO_2 plane. The proposal that the pseudogap metal is a fractionalized Fermi liquid described by a quantum dimer model is extended using the density matrix renormalization group. Measuring the Friedel oscillations in the open boundaries reveals that the fermionic dimers have dispersion minima near (π/2,π/2), which is compatible with the Fermi arcs in photoemission. Moreover, investigating the entanglement entropy suggests that the dimer model with low fermion density is similar to the free fermion system above the Lifshitz transition. We also study the phase transition from a metal with SU(2) spin symmetry to an AF metal. By applying the functional renormalization group to the two-band spin-fermion model, we establish the existence of a strongly coupled fixed point and calculate critical exponents of the fixed point.
This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.
Deconfined quantum criticality of two-dimensional SU(2) quantum antiferromagnets featuring a transition from an antiferromagnetically ordered ground state to a so-called valence-bond solid state, is governed by a non-compact CP1 model with a Maxwell term in 2+1 spacetime dimensions. We introduce a new perspective on deconfined quantum criticality within a field-theoretic framework based on an expansion in powers of ε=4−d for fixed number N of complex matter fields. We show that in the allegedly weak first-order transition regime, a so-called conformal phase transition leads to a genuine deconfined quantum critical point. In such a transition, the gap vanishes when the critical point is approached from above and diverges when it is approached from below. We also find that the spin stiffness has a universal jump at the critical point.
In this thesis I investigate several aspects of local quantum criticality, a concept of key importance in a number of physical contexts ranging from critical heavy fermion compounds to quantum dot systems. Quantum critical points are associated with second order phase transitions at zero temperature. In contrast to their finite-temperature counterparts, the zero-point motion cannot be neglected near a quantum critical point. As a result, the incorporation of quantum dynamics leads to an effective dimension larger than the spatial dimension of the system for the order parameter fluctuations within the Ginzburg-Landau-Wilson treatment of criticality. This so-called quantum-to-classical mapping works well for the critical properties in insulating systems but apparently fails in systems containing gapless fermions. This has been experimentally most clearly been demonstrated within a particular class of intermetallic compounds called heavy fermions. A particular way in which the Ginzburg-Landau-Wilson paradigm fails is for critical Kondo destruction that seems to underlie the unconventional quantum criticality seen in the heavy fermions. I focus on studying the properties of critical Kondo destruction and the emergence of energy-over-temperature-scaling in systems without spatial degrees of freedom, i.e., so-called quantum impurity systems. In particular, I employ large-N techniques to address critical properties of this class of quantum phase transitions in and out of equilibrium. As quantum critical systems are characterized by a scale-invariant spectrum with many low-lying excitations, it may appear that any perturbation can lead to a response beyond the linear response regime. Understanding what governs the non-linear response regime near quantum criticality is an interesting area. Here, I first present a path integral version of the Schrieffer-Wolff transformation which relates the functional integral form of the partition function of the Anderson model to that of its effective low-energy model. The equivalence between the low-energy sector of the Anderson model in the Kondo regime and the spin-isotropic Kondo model is usually established via a canonical transformation performed on the Hamiltonian, followed by a projection. The resulting functional integral assumes the form of a spin path integral and includes a geometric phase factor, i.e. a Berry phase. The approach stresses the underlying symmetries of the model and allows for a straightforward generalization of the transformation to more involved models. As an example of the efficiency of the approach I apply it to a single electron transistor attached to ferromagnetic leads and derive the effective low-energy model of such a magnetic transistor. As Kondo screening is a local phenomenon, it and its criticality can be studied using the appropriate impurity model. A general impurity model to study critical Kondo destruction is the pseudogap Bose-Fermi Kondo model. Here, I concentrate on the multi-channel version of the model using the dynamical large-N study. This model allows to study the non-trivial interplay between two different mechanisms of critical Kondo destruction. The interplay of two processes that can each by itself lead to critical Kondo destruction. The zero-temperature residual entropy at various fixed points for the model is also discussed. The two channel Anderson model exhibits several continuous quantum phase transitions between weak- and strong-coupling phases. The non-crossing approximation (NCA) is believed to give reliable results for the standard two-channel Anderson model of a magnetic impurity in a metal. I revisit the reliability of the NCA for the standard two channel Anderson model (constant conduction electron density of states) and investigate its reliability for the two-channel pseudogap Anderson model. This is done by comparing finite-temperature, finite-frequency solutions of the NCA equations and asymptotically exact zero-temperature NCA solutions with numerical renormalization-group calculations. The phase diagram of this model is well established. The focus here will be on the dynamical scaling properties obtained within the NCA. Finally, I study the thermal and non-thermal steady state scaling functions and the steady-state dynamics of the pseudogap Kondo model. This model allows us to study the concept of effective temperatures near fully interacting as well as weak-coupling fixed points and compare the out-of-equilibrium scaling properties of critical Kondo destruction to those of the traditional spin-density wave (SDW) scenario. The differences I identify can be experimentally probed. This may be helpful in identifying the nature of the quantum critical points observed in certain heavy fermion compounds.
Motivated by recent Monte Carlo simulations of H\"oglund and Sandvik (arXiv:0808.0408), we study edge response in square lattice quantum antiferromagnets. We use the O(3) nonlinear $\ensuremath{\sigma}$ model to compute the decay asymptotics of the staggered magnetization, energy density, and local magnetic susceptibility away from the edge. We find that the total edge susceptibility is negative and diverges logarithmically as the temperature $T\ensuremath{\rightarrow}0$. We confirm the predictions of the continuum theory by performing a 1/S expansion of the microscopic Heisenberg model with the edge. We propose a qualitative explanation of the edge dimerization seen in Monte Carlo simulations by a theory of valence-bond-solid correlations in the N\'eel state. We also discuss the extension of the latter theory to the response of a single nonmagnetic impurity, and its connection to the theory of the deconfined critical point.