Effect of counterintuitive time delays in nonlinear mixing
R. I. Thompson, L. Marmet, Boris Peter Stoicheff
The effect of varying the relative arrival time of the two laser pulses employed in doubly resonant four-wave sum mixing, enhanced by induced transparency, is studied with the aim of optimizing the efficiency of vacuum-ultraviolet generation. With atomic hydrogen as the nonlinear medium, pulsed radiation with wavelengths of 243 and 656 nm and durations of 8 and 14 ns, respectively, is mixed to generate 103-nm coherent radiation. It is shown that by delaying the arrival time of the ground-state pump beam (243 nm) by 2.5-3.5 ns relative to the arrival of the upper-state coupling beam (656 nm), it is possible to enhance the generated intensity by a factor of 2 or more.
Optics Letters•Jan 15, 2000•9 citations