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Physical Review A

Structural phase transition of the ion crystals embedded in an optical lattice

Zhi-Chao Liu, Liang Chen, Ji Li, Hang Zhang, Chengbin Li, Fei Zhou, Shi‐Lei Su, L.-L. Yan, Mang Feng

Published Sep 30, 2020• 13 citations
Publisher

Abstract

The structural phase transition (SPT) occurring in trapped-ion systems is a typical many-body physics, and the SPT induced by the thermal effect represents a special thermodynamic phenomenon between traditional thermodynamics and quantum thermodynamics. We explore this thermal-effect-induced SPT by embedding trapped $^{40}\mathrm{Ca}^{+}$ ion crystals in an optical lattice, in which the ion crystals are confined by a surface-electrode trap and laser-cooled down to a temperature of several millikelvins. The considered thermal effect, leading to a temperature variation of tens of microkelvins in the SPT, comes completely from the optical lattice, which is independent of the laser irradiation regarding cooling of the ion crystals. In comparison with previous work [J. Li et al., Phys. Rev. A 99, 063402 (2019)], the present investigation helps to further clarify the effect of thermal fluctuation and further explore the positive role of the fluctuation in thermodynamics at the atomic level, even for potentially practical applications.

DOI
10.1103/physreva.102.033116

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The structural phase transition (SPT) occurring in trapped-ion systems is a typical many-body physics, and the SPT induced by the thermal effect represents a special thermodynamic phenomenon between traditional thermodynamics and quantum thermodynamics. We explore this thermal-effect-induced SPT by embedding trapped 40Ca+^{40}\mathrm{Ca}^{+}40Ca+ ion crystals in an optical lattice, in which the ion crystals are confined by a surface-electrode trap and laser-cooled down to a temperature of several millikelvins. The considered thermal effect, leading to a temperature variation of tens of microkelvins in the SPT, comes completely from the optical lattice, which is independent of the laser irradiation regarding cooling of the ion crystals. In comparison with previous work [J. Li et al., Phys. Rev. A 99, 063402 (2019)], the present investigation helps to further clarify the effect of thermal fluctuation and further explore the positive role of the fluctuation in thermodynamics at the atomic level, even for potentially practical applications.
Thermal fluctuation usually damages observations in physical systems. But here we demonstrate a unique contribution made by thermal fluctuation, that is, our observation of linear-zigzag phase transitions induced solely by temperature of the 40Ca+^{40}\mathrm{Ca}^{+}40Ca+ ion crystals in a surface-electrode trap. In contrast to the previously observed counterparts based on change in the mechanical equilibrium conditions of the ions, our presented structural phase transition occurs due to controllable influence of thermal fluctuation. The ions' temperature is well controlled by tuning the cooling laser and the experimental observation could be fully understood by classical Langevin equation in addition to the effects from thermal fluctuation. Our experimental investigation indicates the possibility of the positive role thermal fluctuation played in the thermodynamic process at the atomic level, which might bridge the thermodynamics from the macroscopic domain to the quantum regime.
Phase transitions have been a research focus in many-body physics over past decades. Cold ions, under strong Coulomb repulsion, provide a repealing paradigm of exploring phase transitions in stable confinement by electromagnetic field. We demonstrate various conformations of up to sixteen laser-cooled (40)Ca(+) ion crystals in a home-built surface-electrode trap, where besides the usually mentioned structural phase transition from the linear to the zigzag, two additional phase transitions to more complicated two-dimensional configurations are identified. The experimental observation agrees well with the numerical simulation. Heating due to micromotion of the ions is analysed by comparison of the numerical simulation with the experimental observation. Our investigation implies very rich and complicated many-body behaviour in the trapped-ion systems and provides effective mechanism for further exploring quantum phase transitions and quantum information processing with ultracold trapped ions.
We investigate numerically the structural dynamics of ion Coulomb crystals confined in a three-dimensional harmonic trap when influenced by an additional one-dimensional optically induced periodical potential. We demonstrate that transitions between thermally excited crystal structures, such as body-centered cubic and face-centered cubic, can be suppressed by a proper choice of the potential depth and periodicity. Furthermore, by varying the harmonic trap parameters and/or the optical potential in time, controlled transitions between crystal structures can be obtained with close to unit efficiency.
Coulomb crystallisation of laser-cooled ensembles of ions in harmonic traps has been studied experimentally with many spectacular results in recent years. It is well known that for sufficiently large numbers of ions the ground state of a Coulomb crystal in such a system has a body-centred cubic (bcc) structure. However, in experiments with crystals of up to a few 104 ions, structural transitions between bcc and, for example, face centred cubic (fee) or hexagonal close packed (hep) structures are observed. For constant ion densities, the lattice spacing of the planes of highest density differs only by about 3% between bcc and fee structures and simulations predict very small energy differences, thus thermal effects even at temperatures in the mK regime are sufficient to excite these transitions. Here we study numerically the possibility of controlling and switching the crystal structure with the help of periodic potentials generated by the dipole forces of standing-wave light fields.
We investigate the structural properties and melting behaviors of two-dimensional ion crystals in an RF trap, focusing on the effects of ion temperature and trap potential symmetry. We identify distinct crystal structures that form under varying trapping conditions and temperatures through experimental observations and theoretical analyses. As the temperature increases or the trap potential becomes more symmetric, we observe a transition from a lattice arrangement to elongated ring-like formations aligned along the trap axes. Our experimental and theoretical efforts enhance our understanding of phase transitions in low-dimensional, confined systems, offering insights into the controlled formation of quantum crystals for applications in quantum simulations and many-body physics.
We report the sympathetic cooling and Coulomb crystallization of molecular ions above the surface of an ion-trap chip. N2+{\mathrm{N}}_{2}^{+}N2+​ and CaH+{\mathrm{CaH}}^{+}CaH+ ions were confined in a surface-electrode radio-frequency (rf) ion trap and cooled by the interaction with laser-cooled Ca+{\mathrm{Ca}}^{+}Ca+ ions to secular translational temperatures in the millikelvin range. The configuration of trapping potentials generated by the surface electrodes enabled the formation of planar bicomponent Coulomb crystals and the spatial separation of the molecular from the atomic ions on the chip. The structural and thermal properties of the Coulomb crystals were characterized using molecular dynamics simulations. The present study extends chip-based trapping techniques to cold molecular ions with potential applications in mass spectrometry, chemistry, quantum information science, and spectroscopy.