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Excitation of Nuclei and Atoms Trapping in Optical Fields of High Intensity

Anatoli Andreev

Published Nov 1, 2006• 0 citations
OpenAlex

Abstract

This report results from a contract tasking Moscow State University as follows: Exploration of methods to control the radiative gamma- processes in nuclei is currently one of the most promising investigation directions of the modern Quantum Nucleonics - a new realm of contemporary Physics which spreads the basic conceptual ideas and methods of optical Quantum Electronics of atoms and molecules to the gamma-ray range and atomic nuclei and even anti-particles. One of the most important problems in this field is the generation of coherent gamma-radiation by a Gamma-ray Lasing (GRL) process which makes use of excited nuclei as an amplifying medium. The most likely medium for gamma-ray lasers is an ensemble of metastable nuclear isomers, Direct excitation of these isomeric states by electrons or X-ray photons will also create a deeper understanding of nuclear structure and properties.

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•Apr 14, 2008•0 citations
This report results from a contract tasking Moscow State University as follows: Exploration of methods to control the radiative gamma- processes in nuclei is currently one of the most promising investigation directions of the modern Quantum Nucleonics - a new realm of contemporary Physics which spreads the basic conceptual ideas and methods of optical Quantum Electronics of atoms and molecules to the gamma-ray range and atomic nuclei and even anti-particles. One of the most important problems in this field is the generation of coherent gamma-radiation by a Gamma-ray Lasing (GRL) process which makes use of excited nuclei as an amplifying medium. The most likely medium for gamma-ray lasers is an ensemble of metastable nuclear isomers, Direct excitation of these isomeric states by electrons or X-ray photons will also create a deeper understanding of nuclear structure and properties.
The evolution of the foreign and native search for solving the problem of a nuclear gamma-ray laser (NGL), which has been attracting attention for almost half a century despite the absence at present of any convincing data about its experimental solution, is considered. It is shown that the key conflict inherent in any conception of the NGL is the antagonism between the necessity to accumulate a sufficient amount of excited nuclei and the requirement to narrow down the emission gamma-ray line to its natural radiative width. The critical analysis of different approaches for solving this conflict (Mössbauer scheme, deeply cooled ensembles of free nuclei with the hidden inversion, nuclear inversionless amplification, two-quantum gamma emission in counterpropagating photon beams, hypothetical amplifying medium of long-lived isomers in a Bose—Einstein condensate) shows that this search is important not only due to the expected result, which could stimulate the development of quantum nucleonics as a new branch in physics, but also is of interest due to a variety of physical disciplines and experimental approaches used in this search.
The direct interaction between nuclei and strong electromagnetic fields generated by novel coherent x-ray light sources such as the x-ray free electron laser is studied. We investigate the case of various stable or long-lived isotopes with energetically low-lying excited states, where the laser drives the nuclear transition from the ground to the first excited state. We therefore consider the nucleus as a two-level system including the corresponding hyperfine levels in our theoretical description. The performance of present and upcoming x-ray free electron laser facilities in coherently controlling the nuclear excited state population is analyzed for setups involving both solid state as well as accelerated nuclear targets to bridge the gap between photon and transition frequency. Current and predicted laser parameters are applied to calculate excited state populations and signal photon rates of nuclei after a radiation pulse, finding significant improvements compared to former calculations. Furthermore, we determine the parameters necessary to transfer substantial amounts of the nuclear ground state population to the excited state, and therefore to bring nuclear Rabi-oscillation within reach. Additionally, we take into account for the first time collective effects that take place in solid state targets and show that they may provide a significant effect in broadening natural linewidths of nuclear levels depending on the experimental setup. Our findings support the case of nuclear quantum optics for XFEL applications. Therefore, one hopes that eventually coherent control of nuclear transitions can be successfully applied in a number of areas in nuclear physics including preparation, control and detection methods.
There is a possibility that an isomer can be found which could be used to obtain a sufficient population inversion density to bring about nuclear lasing. If it can be realized, a gamma ray laser ("graser") will be a new source of radiation in the sim\\simsim 1A region of unexcelled spectral brightness and coherence, and can be expected to have revolutionary consequences for physics, biology, and chemistry. The result of our research is that the effects of crystallinity are of crucial importance in considerations regarding gamma-ray lasers, bringing in new elements to laser theory which could very well prove decisive in determining whether grasing can or cannot be achieved.\nCertain multi-beam Borrmann eigenmodes of the radiation field in a perfect crystal have much stronger coupling to the emitting nuclei, and much less photoabsorption, than modes in the amorphous case. These modes may be selectively fed by nuclear transitions of the proper multipolarity. A crystal containing such emitters would require orders of magnitude less population inversion density in order to lase than would an amorphous sample of similar material.\nMulti-beam Borrmann modes also have several applications to single-photon optics, particularly the problem of anomalous emission of a gamma\\gammagamma-ray by an internal source of multipolarity M1 or higher. While this effect can occur for a 2-beam Borrmann mode, even stronger anomalous emission is possible into multi-beam Borrmann modes. In addition, certain multi-beam Borrmann modes can anomalously transmit resonant radiation through a Mossbauer crystal. (This cannot occur for the 2-beam modes, except for the case of an E1 transition, since the Borrmann mode couples strongly to the nuclei and thus will be strongly absorbed at resonance.)
The project is focused on theoretical and experimental studies of the quantum coherence effects at the atomic and nuclear transitions in solids. The main results are the following. 1. Electromagnetically Induced Transparency (EIT) and all-optical writing and probing of quantum coherence in room temperature solids are demonstrated experimentally in the first time. 2. The method for coherent suppression of excited state absorption in laser crystals is suggested. It opens the prospects for realization of the variety tunable solid state lasers including UV and VUV ranges. 3. High-efficient THz generation by means of resonant three-level mixing based on EIT in solids is predicted. 4. EIT in gamma-ray range of frequencies at the nuclear transitions via the nuclear level crossing is demonstrated experimentally in the first time. 5. Slowing of the gamma-ray photons due to the absorption line doublet is demonstrated in the first time. 6. Modifications of the Mossbauer absorption spectra under the action of laser radiation demonstrated experimentally in the first time. 7. The method for suppression of the inhomogeneous line broadening of the Mossbauer spectra is suggested.