We introduce the concept of designing new optical materials from “meta-atoms” comprised of matter ultra-strongly-coupled to an optical cavity. Such “strongly-coupled” materials can have surprising properties, such as metallic behavior at low frequencies.
Recent experiments have revealed ultrastrong coupling between light and matter as a promising avenue for modifying material properties, such as electrical transport, chemical reaction rates, and even superconductivity. Here, we explore (ultra)strong coupling as a means for manipulating the optical response of metamaterials based on ensembles of constituent units individually in the ultrastrong-coupling regime. We develop a framework based on linear response for quantum electrodynamical systems to study how light-matter coupling affects the optical response. We begin by applying this framework to find the optical response of a two-level emitter coupled to a single cavity mode, which could be seen as a ``meta-atom'' of a metamaterial built from repeated units of this system. We find optical behavior ranging from that of a simple two-level system (Lorentz-oscillator) to effectively transparent, as the coupling goes from the weak to deep strong-coupling regimes. We explore a one-dimensional chain of these meta-atoms, demonstrating the tunability of its optical behavior. Our scheme may ultimately provide a framework for designing metamaterials with low-loss, highly confined modes, as well as tunable (single-photon) nonlinearities.
Metamaterials are artificially designed materials to exhibit properties not available in natural materials by engineering the constituting elements at sub-wavelength scales, enabling unique interactions of matter with electromagnetic waves or coupling modes of electromagnetic waves. Examples of such novel optics phenomenons include negative index of refraction, cloaking, and super-resolution imaging. The study of superconducting metamaterials operating in the microwave frequency domain has recently generated significant interest in the framework of quantum technologies due to a wide range of direct applications, e.g., exploration of novel quantum optics phenomena, non-destructive quantum sensing, quantum-limited amplification, quantum information processing, and quantum illumination. In contrast to their normal metal and semiconducting counterparts, superconducting metamaterials offer some unique advantages. The most relevant of these for Josephson junction based metamaterials are low losses, flux quantization, and Josephson effects. The Josephson effect in a superconducting loop can also be exploited to exact more control over the nonlinearities of the meta-material.In this thesis, we present Josephson junction based metamaterials with in-situ tunability of second and third-order (Kerr) nonlinearities. We optimized the Josephson junction composites SNAILs, well-known in the superconducting circuits community, for the specific use case of building blocks for an impedance-matched nonlinear meta-material. In such devices, the strong third-order (Kerr) nonlinearity can be tuned from positive to negative values. To demonstrate the efficacy of this phenomenon, we have shown a use case of the meta-material as a TWPA with a new phase-matching mechanism: reversed Kerr phase matching, which utilizes the sign reversal of the Kerr nonlinearity to correct for the dispersion curvature of such devices arising due to its finite plasma. The meta-material operated as reversed Kerr TWPA exhibits up to 4 GHz wide combined amplification band with 8 GHz dynamic band tunability, -98 dBm saturation (1 dB compression point) around 20 dB gain, and amplifier added noise close to the standard quantum limit. The absence of any gaps in the transmission can provide a continuous amplification band with significantly lower gain ripples in contrast to the previously demonstrated TWPAs with dispersion engineering.We also present the generation of entanglement utilizing the metamaterials to demonstrate their versatility and further emphasize their potential in the general framework of nonlinear microwave quantum optics. Due to their large bandwidth, these devices have been identified as promising for generating two-mode squeezing and broadband entanglement. With a device optimized for the generation of broadband entanglement, we observed entanglement between two modes separated by up to 400 MHz. We measured logarithmic negativity between 0.27 and 0.51, and the collective quadrature squeezing below the vacuum limit between 1.5 and 2.1 dB. The presented proof-of-principle results can pave the way towards the implementation of Josephson junction based metamaterials in novel applications, including non-destructive single-photon detection, single-photon measurement and control in c-QED, photon-based quantum computing, precision sensing, the detection of dark matter, and quantum illumination.
Metamamterials are 1D, 2D or 3D arrays of articial atoms. The articial atoms, called "meta-atoms", can be any component with tailorable electromagnetic properties, such as resonators, LC circuits, nano particles, and so on. By designing the properties of individual meta-atoms and the interaction created by putting them in a lattice, one can create a metamaterial with intriguing properties not found in nature. My Ph. D. work examines the meta-atoms based on radio frequency superconducting quantum interference devices (rf-SQUIDs); their tunability with dc magnetic field, rf magnetic field, and temperature are studied. The rf-SQUIDs are superconducting split ring resonators in which the usual capacitance is supplemented with a Josephson junction, which introduces strong nonlinearity in the rf properties. At relatively low rf magnetic field, a magnetic field tunability of the resonant frequency of up to 80 THz/Gauss by dc magnetic field is observed, and a total frequency tunability of 100% is achieved. The macroscopic quantum superconducting metamaterial also shows manipulative self-induced broadband transparency due to a qualitatively novel nonlinear mechanism that is different from conventional electromagnetically induced transparency (EIT) or its classical analogs. A near complete disappearance of resonant absorption under a range of applied rf flux is observed experimentally and explained theoretically. The transparency comes from the intrinsic bi-stability and can be tuned on/ off easily by altering rf and dc magnetic fields, temperature and history. Hysteretic in situ 100% tunability of transparency paves the way for auto-cloaking metamaterials, intensity dependent filters, and fast-tunable power limiters. An rf-SQUID metamaterial is shown to have qualitatively the same behavior as a single rf-SQUID with regards to dc flux, rf flux and temperature tuning. The two-tone response of self-resonant rf-SQUID meta-atoms and metamaterials is then studied here via intermodulation (IM) measurement over a broad range of tone frequencies and tone powers. A sharp onset followed by a surprising strongly suppressed IM region near the resonance is observed. This behavior can be understood employing methods in nonlinear dynamics; the sharp onset, and the gap of IM, are due to sudden state jumps during a beat of the two-tone sum input signal. The theory predicts that the IM can be manipulated with tone power, center frequency, frequency difference between the two tones, and temperature. This quantitative understanding potentially allows for the design of rf-SQUID metamaterials with either very low or very high IM response.