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Conference on Lasers and Electro-Optics

Higher-Order Interference in Quantum Mechanics Induced by Optical Nonlinearities

Lee A. Rozema, Peter Namdar, Irati Alonso Calafell, Alessandro Trenti, Borivoje Dakić, Philip John Walther

Published Jan 1, 2020• 0 citations
Publisher

Abstract

It has been proven theoretically and confirmed experimentally that quantum mechanics exhibits only second-order interference. However, this makes several implicit assumptions. Here we highlight these assumptions experimentally, showing that optical nonlinearities can induce higher-order interference.
DOI
10.1364/cleo_at.2020.jtu2a.22

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The double-slit experiment is a direct demonstration of interference between quantum objects. Of course, interference is also observed in experiments using multiple slits. However, according to quantum theory, the interference patterns produced using such multi-slits can all be explained in terms of interference between pairs of slits [1] , [2] . Interestingly, there are proposed versions of quantum theory—so-called higher-order theories—wherein this is not possible [3] . In such theories the "third-order" interference (with three or more slits open) is genuinely different from second-order interference. Here we show that standard quantum mechanics actually allows for apparent high-order interference, if one considers nonlinear effects. Note, that another mechanism for this has also recently been shown based on so-called looped trajectories [4] – [6] .
Interference between two waves is a well-known concept in physics, and its generalization to more than two waves is straightforward. The order of interference is defined as the number of paths that interfere in a manner that cannot be reduced to patterns of a lower order. In practice, second-order interference means that in, say, a triple-slit experiment, the interference pattern when all three slits are open can be predicted from the interference patterns between all possible pairs of slits. Quantum mechanics is often said to only exhibit second-order interference. However, this is only true under specific assumptions, typically single particles undergoing linear evolution. Here we experimentally show that nonlinear evolution can in fact lead to higher-order interference. The higher-order interference in our experiment can be understood using a simple classical or quantum description, namely optical coherent states interacting in a nonlinear medium. Our work shows that nonlinear evolution could open a loophole for experiments attempting to verify Born's rule by ruling out higher-order interference.
The double-slit experiment is the most direct demonstration of interference between individual quantum objects. Since similar experiments with more slits produce interference fringes reducible to a combination of double-slit patterns it is usually argued that quantum interference occurs between pairs of trajectories, compactly denoted as second-order interference. Here we show that quantum mechanics in fact allows for interference of arbitrarily high order. This occurs naturally when one considers multiple quantum objects interacting in the presence of a nonlinearity. We make this clear by treating a generalised M-slit interferometer using second-quantisation. We then present explicit experimentally-relevant examples both with photons interacting in nonlinear media and an interfering Bose-Einstein condensate with particle-particle interactions. These examples are all perfectly described by quantum theory, and yet exhibit higher-order interference.
The double-slit experiment is the most direct demonstration of interference between individual quantum objects. Since similar experiments with single particles and more slits produce interference fringes reducible to a combination of double-slit patterns, it is usually argued that quantum interference occurs between pairs of trajectories, compactly denoted as second-order interference. Here we show that quantum mechanics in fact allows for interference of arbitrarily high order. This occurs naturally when one considers multiple quantum objects interacting in the presence of a nonlinearity, both of which are required to observe higher-order interference. We make this clear by treating a generalized multislit interferometer using second quantization. We then present explicit experimentally relevant examples both with photons interacting in nonlinear media and an interfering Bose-Einstein condensate with particle-particle interactions. These examples are all perfectly described by quantum theory, and yet exhibit higher-order interference based on multiple particles interacting nonlinearly.
The existence of higher than pairwise quantum interference in the set-up, in which there are more than two slits, is currently under experimental investigation. However, it is still unclear what the confirmation of existence of such interference would mean for quantum theory -- whether that usual quantum mechanics is merely a limiting case of some more general theory or whether that some assumption of quantum theory taken as a fundamental one does not actually hold true. The present paper tries to understand why quantum theory is limited only to a certain kind of interference.
Quantum theory permits interference between indistinguishable paths but, at the same time, restricts its order. Single-particle interference, for instance, is limited to the second order, that is, to pairs of single-particle paths. To date, all experimental efforts to search for higher-order interferences beyond those compatible with quantum mechanics have been based on such single-particle schemes. However, quantum physics is not bound to single-particle interference. We here experimentally study many-particle higher-order interference using a two-photon-five-slit setup. We observe nonzero two-particle interference up to fourth order, corresponding to the interference of two distinct two-particle paths. We further show that fifth-order interference is restricted to 10^{-3} in the intensity-correlation regime and to 10^{-2} in the photon-correlation regime, thus providing novel bounds on higher-order quantum interference.