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Topological Order in Spin Liquids with Chirality

Burkhard Scharfenberger

Published Jan 1, 2011• 0 citations
Publisher

Abstract

We use the Kalmeyer-Laughlin Chiral Spin Liquid as building block to construct a hierarchy of higher-spin spin liquids and determine numerically their topological properties. We compute the entanglement spectra of some of these liquids as well as of ground states of critically frustrated quantum magnets. From the comparison, we find preliminary evidence for a topological phase transition in these systems.

DOI
10.5445/ir/1000023742

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We use the Kalmeyer-Laughlin Chiral Spin Liquid as building block to construct a hierarchy of higher-spin spin liquids and determine numerically their topological properties. We compute the entanglement spectra of some of these liquids as well as of ground states of critically frustrated quantum magnets. From the comparison, we find preliminary evidence for a topological phase transition in these systems.
We demonstrate the existence of a topological chiral spin liquid in the frustrated Shastry-Sutherland Heisenberg model with an additional spin chirality interaction, using numerically unbiased exact diagonalization and density matrix renormalization group methods. We establish a quantum phase diagram where conventional phases, including dimer singlet, plaquette singlet, N\'eel, and collinear phase, can be clearly identified by suitable local order parameters. Among them, an SU(2)1\text{SU}{(2)}_{1}SU(2)1​ chiral spin liquid emerges in the highly frustrated region, which is unambiguously identified by two topologically degenerate ground states, a modular matrix, and characteristic level counting in an entanglement spectrum, featuring the same topological order of the $\ensuremath{\nu}=1/2$ bosonic Laughlin state. The phase boundaries among the different orders are determined by the energy level crossing analysis and wave-function fidelity susceptibility.
The frustrated XY model on the honeycomb lattice has drawn lots of attention because of the potential emergence of chiral spin liquid (CSL) with the increasing of frustrations or competing interactions. In this paper, we study the extended spin-12\frac{1}{2}21​ XY model with nearest-neighbor (J1)({J}_{1})(J1​), and next-nearest-neighbor (J2)({J}_{2})(J2​) interactions in the presence of a three-spins chiral $({J}_{\ensuremath{\chi}})$ term using density matrix renormalization group methods. We obtain a quantum phase diagram with both conventionally ordered and topologically ordered phases. In particular, the long-sought Kalmeyer-Laughlin CSL is shown to emerge under a small ${J}_{\ensuremath{\chi}}$ perturbation due to the interplay of the magnetic frustration and chiral interactions. The CSL, which is a nonmagnetic phase, is identified by the scalar chiral order, the finite spin gap on a torus, and the chiral entanglement spectrum described by chiral SU(2)1SU{(2)}_{1}SU(2)1​ conformal field theory.
We describe a coupled-chain construction for chiral spin liquids in two-dimensional spin systems. Starting from a one-dimensional zigzag spin chain and imposing SU(2) symmetry in the framework of non-Abelian bosonization, we first show that our approach faithfully describes the low-energy physics of an exactly solvable model with a three-spin interaction. Generalizing the construction to the two-dimensional case, we obtain a theory that incorporates the universal properties of the chiral spin liquid predicted by Kalmeyer and Laughlin: charge-neutral edge states, gapped spin-1/2 bulk excitations, and ground-state degeneracy on the torus signaling the topological order of this quantum state. In addition, we show that the chiral spin liquid phase is more easily stabilized in frustrated lattices containing corner-sharing triangles, such as the extended kagome lattice, than in the triangular lattice. Our field-theoretical approach invites generalizations to more exotic chiral spin liquids and may be used to assess the existence of the chiral spin liquid as the ground state of specific lattice systems.
The Kalmeyer-Laughlin chiral spin liquids (CSL) and the Z2 spin liquids are two of the simplest topologically ordered states. Here I develop a theory of a direct quantum phase transition between them. Each CSL is characterized by an integer n and is topologically equivalent to the 1/2n Laughlin fractional quantum Hall (FQH) state. Depending on the parity of n, the transition from the CSL is either to a "twisted" version of the Z2 spin liquid, the "doubled semion" model, or the conventional Z_2 spin liquid ("toric code"). In the presence of SU(2) spin symmetry, the triplet gap remains open through the transition and only singlet operators acquire algebraic correlations. An essential observation is that the CSL/Laughlin FQH states can be understood in terms of bosonic integer quantum Hall (BIQH) states of Schwinger bosons or vortices, respectively. I propose several novel many-body wave functions that can interpolate through the transition.
We describe a coupled-chain construction for chiral spin liquids in two-dimensional spin systems. Starting from a one-dimensional zigzag spin chain and imposing SU(2) symmetry in the framework of non-Abelian bosonization, we first show that our approach faithfully describes the low-energy physics of an exactly solvable model with a three-spin interaction. Generalizing the construction to the two-dimensional case, we obtain a theory that incorporates the universal properties of the chiral spin liquid predicted by Kalmeyer and Laughlin: charge-neutral edge states, gapped spin-1/2 bulk excitations, and ground state degeneracy on the torus signalling the topological order of this quantum state. In addition, we show that the chiral spin liquid phase is more easily stabilized in frustrated lattices containing corner-sharing triangles, such as the extended kagome lattice, than in the triangular lattice. Our field theoretical approach invites generalizations to more exotic chiral spin liquids and may be used to assess the existence of the chiral spin liquid as the ground state of specific lattice systems.
Despite long-standing theoretical interest, the chiral spin liquid, a topologically ordered phase, has yet to be observed experimentally. Here we surprisingly find its emergence in an experimentally realized dipolar XY\text{XY}XY model when Rydberg atoms are arranged in a breathing kagome lattice. Using the infinite density matrix renormalization group, we numerically calculate the ground state's chiral order parameter, spin-spin correlations, Chern number, and entanglement spectrum. Our numerical results provide strong evidence for the chiral spin liquid phase. Furthermore, we identify a quantum phase transition from a Dirac spin liquid to a chiral spin liquid as the lattice geometry is tuned from the isotropic kagome to the breathing kagome lattice.