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Physical Review A

Atomic ionization driven by the quantized electromagnetic field in a Fock state

Igor A. Ivanov, Kyung Taec Kim

Published Aug 24, 2020• 4 citations
Publisher

Abstract

We consider ionization of an atom by the electromagnetic field in a Fock state $|N\ensuremath{\rangle}$: An eigenvector of the operator ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{N}}_{\mathbit{k},\ensuremath{\lambda}}={\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{a}}_{\mathbit{k},\ensuremath{\lambda}}^{\ifmmode\dagger\else\textdagger\fi{}}{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{a}}_{\mathbit{k},\ensuremath{\lambda}}$ of the number of photons in the mode $\mathbit{k},\ensuremath{\lambda}$. We treat the electromagnetic field in a quantized way, which allows us to obtain the photon picture of the strong field ionization. We obtain, in particular, probability distributions for the number of absorbed photons in the process of strong field ionization for atomic systems governed by short-range and Coulomb potentials.

DOI
10.1103/physreva.102.023117

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We consider ionization of an atom by the electromagnetic field in a Fock state ∣N\ensuremath⟩|N\ensuremath{\rangle}∣N\ensuremath⟩: An eigenvector of the operator N\ifmmode^\elseˆ\fi\mathbitk,\ensuremathλ=a\ifmmode^\elseˆ\fi\mathbitk,\ensuremathλ\ifmmode†\else\textdagger\fia\ifmmode^\elseˆ\fi\mathbitk,\ensuremathλ{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{N}}_{\mathbit{k},\ensuremath{\lambda}}={\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{a}}_{\mathbit{k},\ensuremath{\lambda}}^{\ifmmode\dagger\else\textdagger\fi{}}{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{a}}_{\mathbit{k},\ensuremath{\lambda}}N\ifmmode^\elseˆ\fi​\mathbitk,\ensuremathλ​=a\ifmmode^\elseˆ\fi\mathbitk,\ensuremathλ\ifmmode†\else\textdagger\fi​a\ifmmode^\elseˆ\fi\mathbitk,\ensuremathλ​ of the number of photons in the mode \mathbitk,\ensuremathλ\mathbit{k},\ensuremath{\lambda}\mathbitk,\ensuremathλ. We treat the electromagnetic field in a quantized way, which allows us to obtain the photon picture of the strong field ionization. We obtain, in particular, probability distributions for the number of absorbed photons in the process of strong field ionization for atomic systems governed by short-range and Coulomb potentials.
The ionization of atoms in a strong nonclassical unimodal electromagnetic field was considered. It was shown that the probability of ionization could substantially change depending on the quantum state of the field even at a constant mean number of quanta in the radiation mode. The difference of ionization rates was especially large for multiphoton ionization processes. It was, in particular, shown that a nonclassical field could be much more effective from the point of view of the ionization of atoms than a classical field of the same intensity. The characteristics of the decay of a bound atomic system state in a strong nonclassical field were studied without invoking perturbation theory.
The ionization of a model atom in a strong single-mode non-classical electromagnetic field is studied beyond the perturbation approach using the model of ``one discrete level + continuum'' for the atom. Explicit analytical expressions for the time-dependent probability of atomic ionization are obtained for different initial states of radiative field: Fock state, coherent wave packet, squeezed vacuum state. The results are compared to the ionization decay of discrete atomic level in a classical light field, and are analyzed for different mean number of radiative photons. The time-dependent distribution of the quantized field over photon number states is examined.
Using the analytically obtained solution of the Schrödinger equation for an electron in a quantized electromagnetic field, the ionization of an atom has been considered in the framework of a simple one-dimensional model. Expressions for the ionization rate and photoelectron spectrum have been derived and analyzed. We discuss a difference between the results obtained in the model in which the electromagnetic field is described classically and the results obtained in the model of quantized electromagnetic field. In particular, in the latter model the photoelectron spectrum can have a minimum at a certain number of absorbed photons. The minimum is a consequence of destructive interference between the contributions of two parts of the interaction operator.
The photoionization of atoms in a strong electromagnetic field leads to the effect of "above-threshold" ionization, displaying a number of peaks in the energy spectrum of the photoelectrons. In the case of a one-electron model atom in a circularly polarized field, we derive expressions that describe the position as well as the intensity of those peaks as a function of the field parameters by means of a nonperturbative method. It is immediately clear from our formulas that the lowest-energy peaks in general disappear with increasing field intensity, for Coulomb-like as well as shortrange potentials. For a zero-range potential, a numerical evaluation is easily performed, leading to results that are in every respect qualitatively similar to the experimental results obtained thus far on these kinds of processes.
Multiphoton ionization of hydrogen atoms by a strong multimode field when several final continuum states are populated is treated theoretically within a model based on the S-matrix formalism. The field is taken in dipole approximation, with zero bandwidth. Field-dressed Coulomb wave functions are used for the electron final states. Ionization rates are calculated for different numbers of photons absorbed in excess of the minimum number required to go into the continuum. In general, the calculated quantities are in good qualitative agreement with the corresponding experimental observations.
We describe a procedure that allows us to solve the three-dimensional time-dependent Schrödinger equation for an atom interacting with a quantized one-mode electromagnetic field. Atom-field interaction is treated in an ab initio way prescribed by quantum electrodynamics. We use the procedure to calculate probability distributions of absorbed photons in the regime of tunneling ionization. We analyze evolution of the reduced photon density matrix describing the state of the field. We show that non-diagonal density matrix elements decay quickly, as a result of the decoherence process. A stochastic model, viewing ionization as a Markovian birth-death process, reproduces the main features of the calculated photon distributions.