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Physical Review A

Experimental violations of Leggett-Garg inequalities up to the algebraic maximum for a photonic qubit

Kunkun Wang, Mengyan Xu, Lei Xiao, Peng Xue

Published Aug 17, 2020• 7 citations
Publisher

Abstract

Leggett and Garg defined macrorealism by positing that a macroscopic system will exist in a well-defined state at all times, and that this state can be measured without disturbing it. They also formulated a class of inequalities which hold under macrorealism but can be violated by quantum mechanics. The degree to which quantum systems can violate these inequalities is restricted by the temporal Tsirelson bounds. Recently variants of Leggett-Garg inequalities which can be violated to the algebraic maximum 3 for a sufficient large number of measurement times have been proposed. In this work we report an experimental test of quantum violation of the variants of Leggett-Garg inequalities beyond the temporal Tsirelson bounds, up to $2.248\ifmmode\pm\else\textpm\fi{}0.039$ in five-time measurement scenarios for a photonic qubit. Our results clearly show the advantages of the modified measurement scenarios.

DOI
10.1103/physreva.102.022214

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Leggett and Garg defined macrorealism by positing that a macroscopic system will exist in a well-defined state at all times, and that this state can be measured without disturbing it. They also formulated a class of inequalities which hold under macrorealism but can be violated by quantum mechanics. The degree to which quantum systems can violate these inequalities is restricted by the temporal Tsirelson bounds. Recently variants of Leggett-Garg inequalities which can be violated to the algebraic maximum 3 for a sufficient large number of measurement times have been proposed. In this work we report an experimental test of quantum violation of the variants of Leggett-Garg inequalities beyond the temporal Tsirelson bounds, up to 2.248\ifmmode±\else\textpm\fi0.0392.248\ifmmode\pm\else\textpm\fi{}0.0392.248\ifmmode±\else\textpm\fi0.039 in five-time measurement scenarios for a photonic qubit. Our results clearly show the advantages of the modified measurement scenarios.
In 1985, Leggett and Garg formulated a class of inequalities for testing the compatibility between macrorealism and quantum mechanics. In this paper, we point out that, based on the same assumptions of macrorealism that are used to derive Leggett-Garg inequalities (LGIs), there is a scope of formulating another class of inequalities different from the standard LGIs. By considering the three-time measurement scenario in a dichotomic system, we first propose an interesting variant of the standard LGIs and show that its quantum violation is larger than the standard LGIs. By extending this formulation to the nnn-time measurement scenario, we found that the quantum violations of variants of the LGIs for a qubit system increase with nnn, and, for a sufficiently large nnn, an algebraic maximum can be reached. We then compare the violations of the standard and variants of the LGIs in an unsharp measurement scenario and show that, for any arbitrary nnn, the violation of the latter is more robust to unsharpness than the former. Furthermore, we examine the relation between the quantum violations of the variants of the LGIs and an another formulation macrorealism, known as no-signaling in time conditions.
Macrorealistic description governing the classical realm is known to get uprooted in the quantum domain. The Leggett-Garg inequality [A. J. Leggett and A. Garg, Phys. Rev. Lett. 54, 857 (1985)] proposes to probe the macrorealistic limit emerging from the quantum scenario. It places a bound on the linear combinations of temporal correlations of observables measured sequentially at different time intervals. Violation of the Leggett-Garg inequality, up to the so-called temporal Tsirelson bound (TTB), has been realized in the quantum domain. It is important to understand whether quantum theory permits larger violation beyond the TTB and up to the algebraic maximum value of the Leggett-Garg inequality. To this end, it has been shown [C. Budroni and C. Emary, Phys. Rev. Lett. 113, 050401 (2014)] that a three-term Leggett-Garg inequality can be violated beyond the TTB 3/23/23/2 in the time evolution of N>2N>2N>2 level quantum systems by choosing suitable measurement schemes and state-update rules. Furthermore, it is revealed that the algebraic maximum value 3 can be realized in the limit $N\ensuremath{\rightarrow}\ensuremath{\infty}$. Their measurement scheme rules out violation of the Leggett-Garg inequality beyond the TTB by a qubit. Being genuinely quantum in nature, we ask whether such enhanced violation of the Leggett-Garg inequality could be witnessed in a qubit itself. Here, we show that a qubit undergoing time evolution generated by a non-Hermitian PT\mathcal{P}\mathcal{T}PT-symmetric Hamiltonian indeed violates the three-term Leggett-Garg inequality beyond the TTB and up to its algebraic maximum value 3.
Leggett-Garg inequalities are tests of macroscopic realism that can be violated by quantum mechanics. In this letter, we realise photonic Leggett-Garg tests on a three-level system and implement measurements that admit three distinct measurement outcomes, rather than the usual two. In this way we obtain violations of three- and four-time Leggett-Garg inequalities that are significantly in excess of those obtainable in standard Leggett-Garg tests. We also report violations the quantum-witness equality up to the maximum permitted for a three-outcome measurement. Our results highlight differences between spatial and temporal correlations in quantum mechanics.
Leggett-Garg inequalities are tests of macroscopic realism that can be violated by quantum mechanics. In this letter, we realise photonic Leggett-Garg tests on a three-level system and implement measurements that admit three distinct measurement outcomes, rather than the usual two. In this way we obtain violations of three- and four-time Leggett-Garg inequalities that are significantly in excess of those obtainable in standard Leggett-Garg tests. We also report violations the quantum-witness equality up to the maximum permitted for a three-outcome measurement. Our results highlight differences between spatial and temporal correlations in quantum mechanics.
Quantum theory contravenes classical macrorealism by allowing a system to be in a superposition of two or more physically distinct states, producing physical consequences radically different from that of classical physics. We show that a system, upon subjecting to transform under superposition of unitary operators, exhibits enhanced non-macrorealistic feature - as quantified by violation of the Leggett-Garg inequality (LGI) beyond the temporal Tsirelson bound. Moreover, this superposition of unitaries also provides robustness against decoherence by allowing the system to violate LGI and thereby retain its non-macrorealistic behavior for a strikingly longer duration. Using an NMR register, we experimentally demonstrate the superposition of unitaries with the help of an ancillary qubit and verify these theoretical predictions.
According to the world view of macrorealism, the properties of a given system exist prior to and independent of measurement, which is incompatible with quantum mechanics. Leggett and Garg put forward a practical criterion capable of identifying violations of macrorealism, and so far experiments performed on microscopic and mesoscopic systems have always agreed with quantum mechanics. However, a macrorealist can always assign the cause of such violations to the perturbation that measurements effect on such small systems, and hence a definitive test would require using noninvasive measurements, preferably on macroscopic objects, where such measurements seem more plausible. However, the generation of truly macroscopic quantum superposition states capable of violating macrorealism remains a big challenge. In this work we propose a setup that makes use of measurements on the polarization of light, a property that has been extensively manipulated both in classical and quantum contexts, hence establishing the perfect link between the microscopic and macroscopic worlds. In particular, we use Leggett-Garg inequalities and the criterion of no signaling in time to study the macrorealistic character of light polarization for different kinds of measurements, in particular with different degrees of coarse graining. Our proposal is noninvasive for coherent input states by construction. We show for states with well-defined photon number in two orthogonal polarization modes, that there always exists a way of making the measurement sufficiently coarse grained so that a violation of macrorealism becomes arbitrarily small, while sufficiently sharp measurements can always lead to a significant violation.