Nonlinear Quantum Signal Processing in Nanoscale Exciton Systems

Huib J. Bakker, Karl Leo, Jagdeep Shah +1 more

We present an experimental and theoretical study of the dephasing of heavy-hole excitons in a 70-\AA{} GaAs/${\mathrm{Al}}_{\mathit{x}}$${\mathrm{Ga}}_{1\mathrm{\ensuremath{-}}\mathit{x}}$As multiple-quantum-well stucture. We measure the time-integrated three-pulse four-wave-mixing signal of heavy-hole excitons in the quantum-well sample. We model the third-order nonlinear optical response incorporating the effects of a stochastic modulation of the transition frequency. We find that the dephasing of the nonlinear polarization is mainly the result of a spectral-migration process of the excitons and, to a lesser extent, due to a homogeneous dephasing process. The time dependence of the four-wave-mixing signal is very well described by theory if the spectral-migration process is assumed to be energy dependent.

Brendon W. Lovett, John Henry Reina, Ahsan Nazir +2 more

Michel Alexis, Gevorg Mnatsakanyan, Christoph M. Thiele

Abstract Elucidating a connection with nonlinear Fourier analysis (NLFA), we extend a well known algorithm in quantum signal processing (QSP) to represent measurable signals by square summable sequences. Each coefficient of the sequence is Lipschitz continuous as a function of the signal.

T. Voss, Ilja Rückmann, J. Gutowski +2 more

By use of an optical coherent-control technique we demonstrate and analyze the control of transitions involved in the generation of four-wave-mixing signals in a semiconductor quantum well for the two different four-wave-mixing directions and for different sequences of the excitation pulses. Results are presented for frequency- as well as for time-resolved signals. A doubling of the coherent switching frequency is found which occurs if the laser pulses performing the control process contribute quadratically to the wave-mixing signal. A direct comparison between experiment and microscopic theory reveals how the coherent-control process acts on the coherent polarization of the exciton-biexciton system in all different configurations. An additional interpretation of the experimental results based on a simplified few-level model is able to provide an intuitive understanding of the relevant processes which govern the coherent control of the excitonic and biexcitonic wave-mixing polarizations.

T. Takagahara