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Zhurnal Eksperimentalnoi i Teoreticheskoi Fiziki

Spectral distribution of the intensity and polarization of radiation in single-photon quantum transitions in a strong magnetic field.

Igor G. Mitrofanov, Alexei S. Pozanenko

Published Jan 1, 1991• 0 citations
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Spectral distributions of the intensity and polarization in single-photon quantum transitions in a strong electromagnetic field.

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We have studied the transition probabilities and the photofragment energy and angular distributions in a resonant two-photon transition to the continuum with an elliptically polarized radiation field. The general formalism applies both to ionization of atoms within the framework of a single-electron model and the dissociation of diatomic molecules with the involvement of \ensuremath{\Sigma} states only. Detailed calculations for an initial J=0 state give the observable quantities as functions of detuning, intensity, and the polarization parameter for several combinations of the system parameters such as bound-bound and bound-continuum couplings and the Fano q parameter. For sufficiently intense fields the Raman-like coupling between the two coherently excited magnetic sublevels of the resonant J=1 state (one of which can be decoupled from the ground state by a linear transformation) causes a significant enhancement of the transition probability near the Fano minimum obtained for linearly or circularly polarized fields. The evolution of the photofragment kinetic-energy distribution changes with the ellipticity parameter of the radiation. The angular distribution becomes intensity dependent for general ellipticity parameters; the shapes of the resultant distribution in different space-fixed planes are discussed.