Quantum degenerate gases have proven to be an ideal platform for the simulation of complex quantum systems. Due to their high level of control it is possible to readily design and implement systems with effective Hamiltonians in the laboratory. This thesis presents new tools for the characterization and control of engineered quantum systems and describes their application in the realization of a topological system with Rashba-type spin-orbit coupling. The underlying properties of these engineered systems depend on their underlying energies. I describe a Fourier transform spectroscopy technique for characterizing the single particle spectrum of a quantum system. We tested Fourier spectroscopy by measuring the dispersion relation of a spin-1 spin-orbit coupled Bose-Einstein condensate (BEC) and found good agreement with our predictions. Decoherence due to uncontrolled fluctuations of the environment presents fundamental obstacles in quantum science. I describe an implementation of continuous dynamical decoupling (CDD) in a spin-1 BEC. We applied a strong radio-frequency (RF) magnetic field to the ground state hyperfine manifold of Rubidium-87 atoms, generating a dynamically protected dressed system that was first-order insensitive to changes in magnetic field. The CDD states constitute effective clock states and we observed a reduction in sensitivity to magnetic field of up to four orders of magnitude. We additionally show that the CDD states can be coupled in a fully connected geometry and thus enable the implementation of new models not possible using the bare atomic states. Finally, I describe a new realization of Rashba-type SOC using Raman coupled CDD states. Our system had non-trivial topology but no underlying crystalline structure that yields integer valued Chern numbers in conventional materials. We validated our procedure using Fourier transform spectroscopy to measure the full dispersion relation containing only a single Dirac point. We measured the quantum geometry underlying the dispersion relation and obtained the topological index using matter-wave interferometry. In contrast to crystalline materials, where topological indices take on integer values, our continuum system reveals an unconventional half-integer Chern number.
Quantum degenerate gases have proven to be an ideal platform for the simulation of complex quantum systems. Due to their high level of control it is possible to readily design and implement systems with effective Hamiltonians in the laboratory. This thesis presents new tools for the characterization and control of engineered quantum systems and describes their application in the realization of a topological system with Rashba-type spin-orbit coupling. The underlying properties of these engineered systems depend on their underlying energies. I describe a Fourier transform spectroscopy technique for characterizing the single particle spectrum of a quantum system. We tested Fourier spectroscopy by measuring the dispersion relation of a spin-1 spin-orbit coupled Bose-Einstein condensate (BEC) and found good agreement with our predictions. Decoherence due to uncontrolled fluctuations of the environment presents fundamental obstacles in quantum science. I describe an implementation of continuous dynamical decoupling (CDD) in a spin-1 BEC. We applied a strong radio-frequency (RF) magnetic field to the ground state hyperfine manifold of Rubidium-87 atoms, generating a dynamically protected dressed system that was first-order insensitive to changes in magnetic field. The CDD states constitute effective clock states and we observed a reduction in sensitivity to magnetic field of up to four orders of magnitude. We additionally show that the CDD states can be coupled in a fully connected geometry and thus enable the implementation of new models not possible using the bare atomic states. Finally, I describe a new realization of Rashba-type SOC using Raman coupled CDD states. Our system had non-trivial topology but no underlying crystalline structure that yields integer valued Chern numbers in conventional materials. We validated our procedure using Fourier transform spectroscopy to measure the full dispersion relation containing only a single Dirac point. We measured the quantum geometry underlying the dispersion relation and obtained the topological index using matter-wave interferometry. In contrast to crystalline materials, where topological indices take on integer values, our continuum system reveals an unconventional half-integer Chern number.
AbstractTopological order can be found in a wide range of physical systems, from crystalline solids, photonic meta-materials and even atmospheric waves to optomechanic, acoustic and atomic systems. Topological systems are a robust foundation for creating quantized channels for transporting electrical current, light, and atmospheric disturbances. These topological effects are quantified in terms of integer-valued ‘invariants’, such as the Chern number, applicable to the quantum Hall effect, or the Z2 invariant suitable for topological insulators. Here, we report the engineering of Rashba spin-orbit coupling for a cold atomic gas giving non-trivial topology, without the underlying crystalline structure that conventionally yields integer Chern numbers. We validated our procedure by spectroscopically measuring both branches of the Rashba dispersion relation which touch at a single Dirac point. We then measured the quantum geometry underlying the dispersion relation using matter-wave interferometry to implement a form of quantum state tomography, giving a Berry’s phase with magnitude π. This implies that opening a gap at the Dirac point would give two dispersions (bands) each with half-integer Chern number, potentially implying new forms of topological transport.
Topological order can be found in a wide range of physical systems, from crystalline solids, photonic meta-materials and even atmospheric waves to optomechanic, acoustic and atomic systems. Topological systems are a robust foundation for creating quantized channels for transporting electrical current, light, and atmospheric disturbances. These topological effects are quantified in terms of integer-valued 'invariants', such as the Chern number, applicable to the quantum Hall effect, or the [Formula: see text] invariant suitable for topological insulators. Here, we report the engineering of Rashba spin-orbit coupling for a cold atomic gas giving non-trivial topology, without the underlying crystalline structure that conventionally yields integer Chern numbers. We validated our procedure by spectroscopically measuring both branches of the Rashba dispersion relation which touch at a single Dirac point. We then measured the quantum geometry underlying the dispersion relation using matter-wave interferometry to implement a form of quantum state tomography, giving a Berry's phase with magnitude π. This implies that opening a gap at the Dirac point would give two dispersions (bands) each with half-integer Chern number, potentially implying new forms of topological transport.
The dissertation explores the effects of synthetic spin-orbit coupling on the behaviour of quantum gases in several different contexts. We first study realistic methods to create vortices in spin-orbit-coupled (SOC) Bose-Einstein condensates (BEC). We propose two different methods to induce thermodynamically stable static vortex configurations: (1) to rotate both the Raman lasers and the anisotropic trap; and (2) to impose a synthetic Abelian field on top of synthetic spin-orbit interactions. We solve the Gross-Pitaevskii equation for several experimentally relevant regimes and find new interesting effects such as spatial separation of left- and right-moving spin-orbit-coupled condensates, and the appearance of unusual vortex arrangements. Next we consider cold atoms in an optical lattice with synthetic SOC in the Mott-insulator regime. We calculate the parameters of the corresponding tight-binding model and derive the low-energy spin Hamiltonian which is a combination of Heisenberg model, quantum compass model and Dzyaloshinskii-Moriya interaction. We find that the Hamiltonian supports a rich classical phase diagram with collinear, spiral and vortex phases. Next we study the time evolution of the magnetization in a Rashba spin-orbit-coupled Fermi gas, starting from a fully-polarized initial state. We model the dynamics using a Boltzmann equation, which we solve in the Hartree-Fock approximation. The resulting non-linear system of equations gives rise to three distinct dynamical regimes controlled by the ratio of interaction and spin-orbit-coupling strength λ: for small λ, the magnetization decays to zero. For intermediate λ, it displays undamped oscillations about zero and for large λ, a partially magnetized state is dynamically stabilized. Motivated by an interesting stripe phase which appears in BEC with SOC [Li et al., Phys. Rev. Lett. 108, 225301 (2011)], we study the finite-temperature phase diagram of a pseudospin-1/2 Bose gas with contact interactions. We show that strong inter-spin interactions can lead to the appearance of magnetically ordered phases at temperatures above the superfluid transition. For the case of inter-spin attraction, we also discuss the possibility of a bosonic analogue of the Cooper-paired phase, however this state is not energetically favourable. We extend our calculations to a spin-orbit-coupled Bose gas to investigate the possibility of stripe ordering in the normal phase. However, within our approximations, we do not find an instability towards stripe formation. Finally, we consider a two-dimensional Bose gas at zero temperature with an underlying quartic single-particle dispersion in one spatial direction. This Hamiltonian can be realized using the NIST scheme of spin-orbit coupling [Y.-J. Lin, K. Jimenez-Garcia, and I. B. Spielman, Nature 471, 83 (2011)], or using the shaken lattice scheme of Parker et al. [C. V. Parker, L.-C. Ha and C. Chin, Nature Physics 9, 769 (2013)]. By numerically comparing energies of various trial wave-functions, we show that, at low densities, the ground state is strongly correlated, in contrast to a typical mean-field BEC. The trial wave-function with the lowest energy is of Jastrow-type and it describes a state with finite, but strongly reduced, condensate fraction.
We review our recent experimental realization and investigation of a spin-orbit (SO) coupled Bose-Einstein condensate (BEC) and quantum degenerate Fermi gas. By using two counter-propagating Raman lasers and controlling the different frequency of two Raman lasers to engineer the atom-light interaction, we first study the SO coupling in BEC. Then we study SO coupling in Fermi gas. We observe the spin dephasing in spin dynamics and momentum distribution asymmetry of the equilibrium state as hallmarks of SO coupling in a Fermi gas. To clearly reveal the property of SO coupling Fermi gas, we also study the momentum-resolved radio-frequency spectroscopy which characterizes the energy-momentum dispersion and spin composition of the quantum states. We observe the change of fermion surfaces in different helicity branches with different atomic density, which indicates that a Lifshitz transition of the Fermi surface topology change can be found by further cooling the system. At last, we study the momentum-resolved Raman spectroscopy of an ultracold Fermi gas.
We describe a Fourier transform spectroscopy technique for directly measuring band structures, and apply it to a spin-1 spin-orbit coupled Bose-Einstein condensate. In our technique, we suddenly change the Hamiltonian of the system by adding a spin-orbit coupling interaction and measure populations in different spin states during the subsequent unitary evolution. We then reconstruct the spin and momentum resolved spectrum from the peak frequencies of the Fourier transformed populations. In addition, by periodically modulating the Hamiltonian, we tune the spin-orbit coupling strength and use our spectroscopy technique to probe the resulting dispersion relation. The frequency resolution of our method is limited only by the coherent evolution timescale of the Hamiltonian and can otherwise be applied to any system, for example, to measure the band structure of atoms in optical lattice potentials.
Atomic-molecular Bose-Einstein condensates (BECs) offer brand new opportunities to revolutionize quantum gases and probe the variation of fundamental constants with unprecedented sensitivity. The recent realization of spin-orbit coupling (SOC) in BECs provides a new platform for exploring completely new phenomena unrealizable elsewhere. In this study, we find a way of creating a Rashba-Dresselhaus SOC in atomic-molecular BECs by combining the spin-dependent photoassociation and Raman coupling, which can control the formation and distribution of a different type of topological excitation---carbon-dioxide-like skyrmion. This skyrmion is formed by two half-skyrmions of molecular BECs coupling with one skyrmion of atomic BECs, where the two half-skyrmions locate at both sides of one skyrmion. Carbon-dioxide-like skyrmion can be detected by measuring the vortices structures using the time-of-flight absorption imaging technique in real experiments. Furthermore, we find that SOC can effectively change the occurrence of the Chern number in k space, which causes the creation of topological spin textures from some separated carbon-dioxide-like monomers each with topological charge $\ensuremath{-}2$ to a polymer chain of the skyrmions. This work helps in creating dual SOC atomic-molecular BECs and opens avenues to manipulate topological excitations.