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Many Body Localization with Rydberg Atoms

Alicia Handian

Published Jan 1, 2020• 0 citations

Abstract

Systems are known to thermalize, or reach equilibrium, with the passing of time. However, when this does not occur, the quantum states of the system may be localized. Localized states carry information of the system’s initial state that is typically lost during the process of thermalization. We aim to study thermalization and localization in systems of rubidium Rydberg atoms, and to further understand these phenomena via simulation while we are developing a more refined experiment. These atoms exchange energy via tuned resonances while contained within a magneto optical trap. This process can be categorized as either a two, three, or four body interaction; localization is only expected to occur in the latter two. As the atoms transfer energy via dipole-dipole interactions, the population of atoms occupying different states shifts. Some atoms are shifted to a measurable state, and each trial of the experiment lasts for only several microseconds as data is collected. The energy transport within the system is simulated on a supercomputer in order to produce a model for the experimental data, while also allowing us to closely analyze parameters that are not accessible through experiment. From the model, we hope to learn whether the system thermalizes or localizes. We present initial simulation results exploring the energy exchange dynamics in a Rubidium many-body system.

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Systems are known to thermalize, or reach equilibrium, with the passing of time. However, when this does not occur, the quantum states of the system may be localized. Localized states carry information of the system’s initial state that is typically lost during the process of thermalization. We aim to study thermalization and localization in systems of rubidium Rydberg atoms, and to further understand these phenomena via simulation while we are developing a more refined experiment. These atoms exchange energy via tuned resonances while contained within a magneto optical trap. This process can be categorized as either a two, three, or four body interaction; localization is only expected to occur in the latter two. As the atoms transfer energy via dipole-dipole interactions, the population of atoms occupying different states shifts. Some atoms are shifted to a measurable state, and each trial of the experiment lasts for only several microseconds as data is collected. The energy transport within the system is simulated on a supercomputer in order to produce a model for the experimental data, while also allowing us to closely analyze parameters that are not accessible through experiment. From the model, we hope to learn whether the system thermalizes or localizes. We present initial simulation results exploring the energy exchange dynamics in a Rubidium many-body system.

Isolated quantum systems are anticipated to obey the eigenstate thermalization hypothesis by coming to thermal equilibrium. In our experiments, ultracold Rydberg atoms thermalize when they exchange energy via two-body interactions, but not three-body interactions. We believe this to be the result of a specially tuned initial state that maps onto quantum many body scar states. We propose an experiment in which we modify the initial state and measure the degree to which the system thermalizes. We present experimental and simulation data to support this.

We simulate the dynamics of Rydberg atoms resonantly exchanging energy via two-, three-, and four-body dipole-dipole interactions in a one-dimensional array. Using simplified models of a realistic experimental system, we study the initial-state survival probability, mean level spacing, spread of entanglement, and properties of the energy eigenstates. By exploring a range of disorders and interaction strengths, we find regions in parameter space where the three- and four-body dynamics either fail to thermalize or do so slowly. The interplay between the stronger hopping and weaker field-tuned interactions gives rise to quantum many-body scar states, which play a critical role in slowing the dynamics of the three- and four-body interactions. Published by the American Physical Society 2024

We measure the transport of energy among the internal states of ultracold rubidium Rydberg atoms coupled by dipole-dipole exchange. In a magneto-optical trap, a static electric field of a few V/cm shifts the energy levels of the atoms. For a particular principal quantum number,

n

, the angular momentum eigenstates

\ell > 4

are nearly degenerate at zero electric field. At nonzero field, a manifold of equally spaced clusters form a ladder with each rung consisting of a set of closely spaced

m

energy eigenstates. We excite Rydberg atoms to energy levels near the center of the manifold and allow them to exchange energy via resonant dipole-dipole interactions. We measure the time evolution as energy spreads away from the center of the manifold, which reveals that the system may fail to thermalize for long interaction times. A computational model that includes only a few essential features of the system qualitatively agrees with this result.

An isolated system of ultracold Rydberg atoms can come to equilibrium by exchanging energy through dipole-dipole interactions. In our experiment, a static electric field of a few V/cm shifts the energy levels of the atoms, so that the energy levels are nearly degenerate at zero field and fan out with increasing field to form a manifold. We excite atoms to energy levels near the center of the manifold, where the spacing is nearly harmonic. We allow them to interact for a few microseconds, by which time the population of each energy level has reached a steady state. The population is then measured at various densities and compared to simulation results. We use the notion of dynamical typicality to predict the equilibrium configuration and show that the system fails to thermalize.

The dipole-dipole interaction strongly couples ultracold highly excited atoms, known as Rydberg atoms, and is the dominant mechanism for energy exchange among such atoms on microsecond time scales. I present the results of experiments that investigate this interaction using rubidium atoms excited to Rydberg states with an all-diode laser system. In the first of these, high resolution dipole-dipole interaction spectra for different magnetic sublevels of the 32d5/2 state are collected and analyzed. In the second experiment, ultracold rubidium atoms are implusively excited to coherent superpositions of three closely spaced |mj|sublevels of the 32d5/2 state in a weak electric field. The magnitude of the field sets the energy level spacing between these states, and hence the frequency of the phase dependent oscillations resulting from interference in resonant energy exchange processes. In the third experiment, the dipole-dipole interaction induced resonant energy exchange between columns of ultracold rubidium Rydberg atoms is imaged using a new technique involving selective field ionization with a spatially sensitive ion detector.

Rubidium Rydberg atoms in either |m_{j}| sublevel of the 36p_{3/2} state can exchange energy via Stark-tuned Förster resonances, including two-, three-, and four-body dipole-dipole interactions. Three-body interactions of this type were first reported and categorized by Faoro et al. [Nat. Commun. 6, 8173 (2015)NCAOBW2041-172310.1038/ncomms9173] and their Borromean nature was confirmed by Tretyakov et al. [Phys. Rev. Lett. 119, 173402 (2017)PRLTAO0031-900710.1103/PhysRevLett.119.173402]. We report the time dependence of the N-body Förster resonance N×36p_{3/2,|m_{j}|=1/2}→36s_{1/2}+37s_{1/2}+(N-2)×36p_{3/2,|m_{j}|=3/2}, for N=2, 3, and 4, by measuring the fraction of initially excited atoms that end up in the 37s_{1/2} state as a function of time. The essential features of these interactions are captured in an analytical model that includes only the many-body matrix elements and neighboring atom distribution. A more sophisticated simulation reveals the importance of beyond-nearest-neighbor interactions and of always-resonant interactions.