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OptSp

Optical nonlinearity of a two-level medium

V. E. Brazovskii

Published May 1, 1986• 0 citations
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We present a microscopic analysis and evaluation of the dielectric susceptibility of a dielectric medium consisting of vector-type two-energy-level atoms responding on a weak probe mode when the atoms are driven by a strong coherent field. Each atom, in an environment of others, exists as a quasiparticle further structuring a bulk medium. In a limit of dilute atomic gas, the dynamics of each atom follows the Mollow-type nonlinear excitation regime, and the medium susceptibility collectivizes the individual atomic responses to the probe mode. We outline how the collective dynamics can be interpolated up to a dense medium, and we argue from general positions that in such a medium the optical nonlinearity and, in particular, its parametric part could be significantly magnified by manipulating both the coherent pump and the sample density. That indicates certain limitations for potential capabilities of quantum communication protocols utilizing the entangled photons, created by a parametric process, as a main resource of quantum correlations.

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We investigate the propagation dynamics of nonlinear chirped optical laser pulses in a two-level medium.For certain chirp strength and chirp width, an incident 2π nonlinear chirped pulse will split into optical precursors and a stable self-induced transparency soliton.This is caused by the particular Fourier spectrum that includes not only central resonant frequency components but also high-frequency and low-frequency sidebands.Moreover, the effects of chirp parameters on the evolution of nonlinear chirped pulses are also discussed.
Summary form only given.Nonlinear optical effects are normally limited to high-intensity fields containing a large number of photons because the electric field associated with a single photon is usually very weak. Nonlinear phase shifts at the two-photon level previously have been observed using high-Q cavities and atomic beams. The authors recently predicted that nonlocal effects involving pairs of atoms in a medium could enhance the nonlinear interaction between two photons to the point that nonlinear phase shifts could be obtained in an ordinary medium without the use of resonant cavities.
We present a microscopic analysis and evaluation of the dielectric susceptibility of a dielectric medium consisting of vector-type two-energy-level atoms responding on a weak probe mode when the atoms are driven by a strong coherent field. Each atom, in an environment of others, exists as a quasiparticle further structuring a bulk medium. In a limit of dilute atomic gas, the dynamics of each atom follows the Mollow-type nonlinear excitation regime, and the medium susceptibility collectivizes the individual atomic responses to the probe mode. We outline how the collective dynamics can be interpolated up to a dense medium, and we argue from general positions that in such a medium the optical nonlinearity and, in particular, its parametric part could be significantly magnified by manipulating both the coherent pump and the sample density. That indicates certain limitations for potential capabilities of quantum communication protocols utilizing the entangled photons, created by a parametric process, as a main resource of quantum correlations.