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APS

Tunneling Ionization Rates from Arbitrary 1-D Potential Wells

George N. Gibson, Gerald V. Dunne, K. J. Bergquist

Published May 1, 1998• 0 citations
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The comprehension of the tunnel effect, the passage of matter waves and particles across a high potential barrier, was the most astounding of all discoveries in quantum mechanics. Research on tunnelling in semiconductors and superconductors, as well as the development of scanning tunnelling microscopy, garnered five Nobel prizes in physics. In this study, the resonant tunnelling effect of electron tunnelling through a one-dimensional double-potential barrier was found and verified by solving the time-independent Schrödinger equation and calculating the transmittance rate of the electron tunnelling through the two potential barriers by using the transmission matrix technique performed by MATLAB. According to the analysis, the transmittance rate was one under certain specific conditions (under some specific incident energy values or some specific distance between two potential barriers), which was called as resonant tunnelling. However, in this study, square potential wells were analyzed, which can be considered merely as ideal models in real life, and therefore all results are idealized. For further investigations, researchers can use more realistic parameters to set up potential wells and analyze real-life problems.

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Probing Resonant Photoionization Time Delay by Self-Referenced Molecular Attoclock

Jihong Tong, Xiwang Liu, Wenhui Dong +9 more

Attosecond time-resolved electron tunneling dynamics have been investigated by using attosecond angular streaking spectroscopy, where a clock reference to the laser field vector is required in atomic strong-field ionization and the situation becomes complicated in molecules. Here we reveal a resonant ionization process via a transient state by developing an electron-tunneling-site-resolved molecular attoclock in Ar-Kr^{+}. Two distinct deflection angles are observed in the photoelectron angular distribution in the molecular frame, corresponding to the direct and resonant ionization pathways. We find the electron is temporally trapped in the Coulomb potential wells of the Ar-Kr^{+} before finally releasing into the continuum when the electron tunnels through the internal barrier. By utilizing the direct tunneling ionization as a self-referenced arm of the attoclock, the time delay of the electron trapped in the resonant state is revealed to be 3.50±0.04 fs. Our results give an impetus to exploring the ultrafast electron dynamics in complex systems and also endow a semiclassical presentation of the electron trapping dynamics in a quantum resonant state.

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Suppression and Enhancement of Collisions in Optical Lattices

John Lawall, Chad Orzel, S. L. Rolston

In a three-dimensional optical lattice for metastable xenon we observe the dynamical effects of the optical potential on Penning ionizing collisions between atoms. Enhancement of collisions over that for free atoms is observed at short times after the atoms are loaded into the lattice. After the atoms thermalize and localize into the potential wells, we observe a suppression of the collisions by as much as a factor of 2. From our measurements and a simple model we are able to extract an estimate of the rate at which atoms ``hop'' between wells.

Physical Review Letters•Jan 19, 1998•16 citations
The comprehension of the tunnel effect, the passage of matter waves and particles across a high potential barrier, was the most astounding of all discoveries in quantum mechanics. Research on tunnelling in semiconductors and superconductors, as well as the development of scanning tunnelling microscopy, garnered five Nobel prizes in physics. In this study, the resonant tunnelling effect of electron tunnelling through a one-dimensional double-potential barrier was found and verified by solving the time-independent Schrödinger equation and calculating the transmittance rate of the electron tunnelling through the two potential barriers by using the transmission matrix technique performed by MATLAB. According to the analysis, the transmittance rate was one under certain specific conditions (under some specific incident energy values or some specific distance between two potential barriers), which was called as resonant tunnelling. However, in this study, square potential wells were analyzed, which can be considered merely as ideal models in real life, and therefore all results are idealized. For further investigations, researchers can use more realistic parameters to set up potential wells and analyze real-life problems.
Attosecond time-resolved electron tunneling dynamics have been investigated by using attosecond angular streaking spectroscopy, where a clock reference to the laser field vector is required in atomic strong-field ionization and the situation becomes complicated in molecules. Here we reveal a resonant ionization process via a transient state by developing an electron-tunneling-site-resolved molecular attoclock in Ar-Kr^{+}. Two distinct deflection angles are observed in the photoelectron angular distribution in the molecular frame, corresponding to the direct and resonant ionization pathways. We find the electron is temporally trapped in the Coulomb potential wells of the Ar-Kr^{+} before finally releasing into the continuum when the electron tunnels through the internal barrier. By utilizing the direct tunneling ionization as a self-referenced arm of the attoclock, the time delay of the electron trapped in the resonant state is revealed to be 3.50±0.04 fs. Our results give an impetus to exploring the ultrafast electron dynamics in complex systems and also endow a semiclassical presentation of the electron trapping dynamics in a quantum resonant state.
In a three-dimensional optical lattice for metastable xenon we observe the dynamical effects of the optical potential on Penning ionizing collisions between atoms. Enhancement of collisions over that for free atoms is observed at short times after the atoms are loaded into the lattice. After the atoms thermalize and localize into the potential wells, we observe a suppression of the collisions by as much as a factor of 2. From our measurements and a simple model we are able to extract an estimate of the rate at which atoms ``hop'' between wells.