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Journal of Experimental and Theoretical Physics

Theory of spontaneous and stimulated emission of electromagnetic waves in unidimensionally inhomogeneous media and resonators

V. S. Pekar

Published Aug 1, 1975• 1 citation
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In this paper, four different ways are described in which homogeneous, isotropic, nonferromagnetic, Maxwellian media at rest may exhibit absorption and stimulated emission. These four ways may be identified by a positive or negative conductivity, a sink or source-type electric field, a complex dielectric constant, and a complex permeability. The forms of the electromagnetic waves, the refractive index, and the positive or negative extinction coefficient are determined for each process for both absorbing and active media. Spontaneous emission is associated with source-type electric and magnetic fields which generate conduction or displacement currents in the medium with improper phases to contribute to the radiant flux in the incident electromagnetic wave. Stimulated emission is characterized by exponentially increasing incident electric and magnetic fields and an excess of the time average of the outflow of radiant flux over the surfaces of an arbitrary volume. Stimulated emission appears when the time average of the rate at which the source-type electric and magnetic fields do work in carrying certain conduction or displacement currents in directions opposite to the incident electric and magnetic fields is greater than the time average of the rate at which the incident electric and magnetic fields dissipate energy by doing work in carrying other conduction or displacement currents in directions parallel to the incident electric and magnetic fields.

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The rate of spontaneous emission is known to depend on the environment of a emitter, and the enhancement of one-photon emission in a resonant cavity is known as the Purcell effect. Here we develop a theory of spontaneous two-photon emission for a general electromagnetic environment including inhomogeneous dispersive and absorptive media. This theory is used to evaluate the two-photon Purcell enhancement in the vicinity of metallic nanoparticles and demonstrates that the surface-plasmon resonances supported by these particles can increase the emission rate by more than two orders of magnitude. The control over two-photon Purcell enhancement given by tailored nanostructured environments could provide an emitter with any desired spectral response and may serve as an ultimate route for designing light sources with novel properties.

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Possibility of multiline stimulated emission from spectrally inhomogeneous liquid media

L. P. Godenko, Vladimir S. Mashkevich

A theoretical investigation is made of the possibility of multiline stimulated emission from spectrally inhomogeneous liquid media. Numerical estimates are given.

Soviet Journal of Quantum Electronics•Jun 30, 1975•0 citations
In this paper, four different ways are described in which homogeneous, isotropic, nonferromagnetic, Maxwellian media at rest may exhibit absorption and stimulated emission. These four ways may be identified by a positive or negative conductivity, a sink or source-type electric field, a complex dielectric constant, and a complex permeability. The forms of the electromagnetic waves, the refractive index, and the positive or negative extinction coefficient are determined for each process for both absorbing and active media. Spontaneous emission is associated with source-type electric and magnetic fields which generate conduction or displacement currents in the medium with improper phases to contribute to the radiant flux in the incident electromagnetic wave. Stimulated emission is characterized by exponentially increasing incident electric and magnetic fields and an excess of the time average of the outflow of radiant flux over the surfaces of an arbitrary volume. Stimulated emission appears when the time average of the rate at which the source-type electric and magnetic fields do work in carrying certain conduction or displacement currents in directions opposite to the incident electric and magnetic fields is greater than the time average of the rate at which the incident electric and magnetic fields dissipate energy by doing work in carrying other conduction or displacement currents in directions parallel to the incident electric and magnetic fields.
The rate of spontaneous emission is known to depend on the environment of a emitter, and the enhancement of one-photon emission in a resonant cavity is known as the Purcell effect. Here we develop a theory of spontaneous two-photon emission for a general electromagnetic environment including inhomogeneous dispersive and absorptive media. This theory is used to evaluate the two-photon Purcell enhancement in the vicinity of metallic nanoparticles and demonstrates that the surface-plasmon resonances supported by these particles can increase the emission rate by more than two orders of magnitude. The control over two-photon Purcell enhancement given by tailored nanostructured environments could provide an emitter with any desired spectral response and may serve as an ultimate route for designing light sources with novel properties.