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APS

Quantum Control in Atom Optics

Dan Steck

Published Apr 1, 2005• 0 citations
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Advances of quantum control technology have led to nearly perfect single-qubit control of nuclear spins and atomic hyperfine ground states. In contrast, quantum control of strong optical transitions, even for free atoms, are far from being perfect. Developments of such quantum control appears to be limited by available laser technology for generating isolated, sub-nanosecond optical waveforms with 10's of GHz programming bandwidth. Here we propose a simple and robust method for the desired pulse shaping, based on precisely stacking multiple delayed picosecond pulses. Our proof-of-principal demonstration leads to arbitrarily shapeable optical waveforms with 30 GHz bandwidth and 100 ps duration. We confirm the stability of the waveforms by interfacing the pulses with laser-cooled atoms, resulting in "super-resolved" spectroscopic signals. This pulse shaping method may open exciting perspectives in quantum optics, and for fast laser cooling and atom interferometry with mode-locked lasers.

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GAINING CONTROL IN QUANTUM OPTICS

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John Hall Symposium•Mar 28, 2006•0 citations
Advances of quantum control technology have led to nearly perfect single-qubit control of nuclear spins and atomic hyperfine ground states. In contrast, quantum control of strong optical transitions, even for free atoms, are far from being perfect. Developments of such quantum control appears to be limited by available laser technology for generating isolated, sub-nanosecond optical waveforms with 10's of GHz programming bandwidth. Here we propose a simple and robust method for the desired pulse shaping, based on precisely stacking multiple delayed picosecond pulses. Our proof-of-principal demonstration leads to arbitrarily shapeable optical waveforms with 30 GHz bandwidth and 100 ps duration. We confirm the stability of the waveforms by interfacing the pulses with laser-cooled atoms, resulting in "super-resolved" spectroscopic signals. This pulse shaping method may open exciting perspectives in quantum optics, and for fast laser cooling and atom interferometry with mode-locked lasers.
Molecules, with their rich spectrum of internal states as well as strong and tunable dipolar interactions, are promising candidates for a broad range of experiments including quantum information, quantum chemistry, precision measurement and probing physics beyond the Standard Model, and quantum simulation of interacting many-body systems. At the same time, the complexity that made them attractive also poses a significant challenge to achieve a high level of quantum control that is required in many of their potential applications. Multiple approaches are being pursued for full quantum control of molecules including association of atomic gases and direct cooling of molecules, yet it remains challenging to control molecules at single particle level due to the difficulty in tuning the atom-atom interaction and laser cooling of molecules. In this thesis, we achieved full control on a single weakly bound ground state molecule created by coherent optical association from single atoms. We first discuss the trapping and imaging of the atoms in the optical tweezer and the cooling into a single quantum state in order to achieve the quantum control of atoms. Combining this control with the resolution and flexibility of tweezers. we developed a versatile platform to study interactions between single atoms and properties of single molecules, using precise optical spectroscopy on pairs of atoms in the tweezer. Based on these studies, we proposed a promising pathway for coherent all-optical creation of molecules and experimentally demonstrated full control on the molecule including all degrees of freedom.
We explore the emergence and active control of optical bistability in a two-level atom near a graphene sheet. Our theory incorporates self-interaction of the optically driven atom and its coupling to electromagnetic vacuum modes, both of which are sensitive to the electrically tunable interband transition threshold in graphene. We show that electro-optical bistability and hysteresis can manifest in the intensity, spectrum, and quantum statistics of the light emitted by the atom, which undergoes critical slow-down to steady state. The optically driven atom-graphene interaction constitutes a platform for active control of driven atomic systems in coherent quantum control and atomic physics.