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Soviet physics. Doklady

Optical Absorption Spectra of Silver Atoms Stabilized in Various Matrices at 77°k

R. A. Zhitnikov, N. I. Melnikov

Published Aug 1, 1966• 0 citations
OpenAlex

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Optical properties of a concentric silver-atomic medium nanoshell are investigated based on the quasi-static and Maxwell-Garnett approximations. We consider the atomic medium as Λ-type three-level atoms driven simultaneously by a coupling field and a probe field. It is shown that the strong coupling between atoms and sphere plasmon of silver core emerges of multiple-mode and ultra narrow-band absorption spectra by controlling the permittivity of the atomic medium. In particular, coherent driving of the coupling field allows us to manipulate surface plasmon resonances, including frequency shift and bandwidth modification. Furthermore, we demonstrate that selective absorption enhancement of different modes can be achieved by tuning the radius of the core and the shell. These absorption properties yield potential applications of the nanoshells as ultracompact tunable nonlinear optical devices.
We present a quantitative study of laser absorption on the 52S1/2→52P3/25{^{2}}\mathrm{S}_{1/2} \rightarrow 5{^{2}}\mathrm{P}_{3/2}52S1/2​→52P3/2​ transition of silver in a hollow-cathode lamp. Spectra obtained using a weak probe are measured and compared to a simple theoretical model. We fit our results to extract an effective temperature and number density associated with the silver in the lamp and confirm that the spectra are dominated by Doppler broadening. We consider the broadening effect of collisions between silver and the neon buffer gas in the lamp, and establish that these effects are small but modify the optimum effective parameters for the model. Our work results in a simple, quantitative, and predictive model for laser absorption in the lamp.