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Science

Metalens-array–based high-dimensional and multiphoton quantum source

Lin Li, Zexuan Liu, Xi‐Feng Ren, Shuming Wang, Vin‐Cent Su, Mu Ku Chen, Cheng Hung Chu, Hsin Yu Kuo, Bi‐Heng Liu, Wenbo Zang, Guang‐Can Guo, Lijian Zhang, Zhenlin Wang, Shining N. Zhu, Din Ping Tsai

Published Jun 25, 2020• 463 citations
Publisher

Abstract

The development of two-dimensional metasurfaces has shown great potential in quantum-optical technologies because of the excellent flexibility in light-field manipulation. By integrating a metalens array with a nonlinear crystal, we demonstrate a 100-path spontaneous parametric down-conversion photon-pair source in a 10 × 10 array, which shows promise for high-dimensional entanglement and multiphoton-state generation. We demonstrate two-, three- and four-dimensional two-photon path entanglement with different phases encoded by metalenses with fidelities of 98.4, 96.6, and 95.0%, respectively. Furthermore, four-photon and six-photon generation is observed with high indistinguishability of photons generated from different metalenses. Our metalens-array-based quantum photon source is compact, stable, and controllable, indicating a new platform for integrated quantum devices.

DOI
10.1126/science.aba9779

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The development of two-dimensional metasurfaces has shown great potential in quantum-optical technologies because of the excellent flexibility in light-field manipulation. By integrating a metalens array with a nonlinear crystal, we demonstrate a 100-path spontaneous parametric down-conversion photon-pair source in a 10 × 10 array, which shows promise for high-dimensional entanglement and multiphoton-state generation. We demonstrate two-, three- and four-dimensional two-photon path entanglement with different phases encoded by metalenses with fidelities of 98.4, 96.6, and 95.0%, respectively. Furthermore, four-photon and six-photon generation is observed with high indistinguishability of photons generated from different metalenses. Our metalens-array-based quantum photon source is compact, stable, and controllable, indicating a new platform for integrated quantum devices.
Photon pairs generated by spontaneous parametric down-conversion (SPDC) are playing a pivotal role in many quantum applications such as quantum computing, quantum imaging and quantum communication. Metasurfaces, which are two-dimensional arrays of nanostructures, have been studied intensively to enhance SPDC and provide additional functionalities over the bulky optical systems [1]. Van der Waals (vdWs) layered materials have emerged as promising platform for quantum light sources, owing to their unique properties [2], [3]. For example, vdWs materials offer high refractive index, a high nonlinear susceptibility, and compatibility with on-chip integration.
Harnessing high-dimensional entangled states of light presents a frontier for advancing quantum information technologies, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the spatial degree of freedom stands out as particularly suited for on-chip integration. But while traditional demonstrations produce and manipulate path-entangled states sequentially with discrete optical elements, continuously-coupled nonlinear waveguide systems offer a promising alternative where photons can be generated and interfere along the entire propagation length, unveiling novel capabilities within a reduced footprint. Here we exploit this concept to implement a compact and reconfigurable source of path-entangled photon pairs based on parametric down-conversion in semiconductor AlGaAs nonlinear waveguides arrays.
All-dielectric optical metasurfaces are a workhorse in nano-optics, because of both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to 2 orders of magnitude, compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons-a new promising platform for quantum optics experiments.
Most modern quantum light sources are based on spontaneous parametric down-conversion (SPDC) in bulk non-linear crystals, with strict phase-matching requirements that limit their design flexibility and the range of two-photon states produced. Recent research has focused on generating quantum light via SPDC with metasurfaces [1], i.e. array of nanoresonators with sub-wavelength dimensions. At this scale, SPDC becomes independent of phase matching, allowing the use of materials with greater nonlinear susceptibility and enabling efficient photon generation with tailored properties for the angular and spectral distribution and polarization.
Entangled photon-pairs generated through spontaneous parametric down-conversion (SPDC) have evolved into an indispensable resource for various quantum communication, imaging, sensing and computing schemes. While photon-pair sources are so far mostly based on bulk-optical nonlinear components, resonant nonlinear metasurfaces with sub-wavelength thickness have recently been demonstrated as a new platform for photon-pair generation [1]–[3]. Contrary to bulk and integrated nonlinear structures where phase matching steers the pair generation efficiency in different directions and wavelengths, nanostructures can control these properties via their optical resonances. However, the tunability of spatial photon emission in multiple directions remained an open challenge.