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Optics Express

Controllable superbunching effect from four-wave mixing process in atomic vapor

Shuanghao Zhang, Huaibin Zheng, Gao Wang, Jianbin Liu, Sheng Luo, Yuchen He, Yu Zhou, Hui Chen, Zhuo Xu

Published Jun 25, 2020• 3 citations
Publisher

Abstract

Correlation property of light limits the performance in related applications such as the visibility of ghost imaging or intensity interferometry. To exceed these performance limits, we here manipulate the degree of second- and higher-order coherence of light by changing controllable variables in four-wave mixing (FWM) process. The measured degree of second- and third-order coherence of the output light beams considerably exceed those of the incident pseudothermal light. Namely superbunching effects, g(2)(0) value up to 7.47 and g(3)(0) value up to 58.34, are observed experimentally. In addition, strong second- and third-order cross-correlation exist between the output light beams. Further insights into the dependence of superbunching light on the temperature of Rb vapor, the laser detuning and the optical power of all the incident light beams show that it can serve as a light source with a tunable superbunching degree.

DOI
10.1364/oe.394211

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Correlation property of light limits the performance in related applications such as the visibility of ghost imaging or intensity interferometry. To exceed these performance limits, we here manipulate the degree of second- and higher-order coherence of light by changing controllable variables in four-wave mixing (FWM) process. The measured degree of second- and third-order coherence of the output light beams considerably exceed those of the incident pseudothermal light. Namely superbunching effects, g(2)(0) value up to 7.47 and g(3)(0) value up to 58.34, are observed experimentally. In addition, strong second- and third-order cross-correlation exist between the output light beams. Further insights into the dependence of superbunching light on the temperature of Rb vapor, the laser detuning and the optical power of all the incident light beams show that it can serve as a light source with a tunable superbunching degree.
Two-photon superbunching of classical light is observed with single-mode continuous-wave laser light in a linear optical system. By adding more two-photon paths via rotating ground glasses, pinholes, lens, etc., g(2)(0)=7.10±0.07 is experimentally observed. The second-order temporal coherence function of the superbunching pseudothermal light is theoretically and experimentally studied in detail. It is predicted that the degree of coherence can be increased dramatically by adding more multi-photon paths. For instance, the degree of the second- and third-order coherence of the superbunching pseudothermal light with five rotating ground glasses can reach 32 and 7776, respectively. The results are helpful to understanding the physics of superbunching and improving the visibility of thermal light ghost imaging.
Superposition of multiple indistinguishable two-photon paths is introduced by means of a digital wave front encoding technique to design a spatially phase-correlated wave front of a light field, which could result in a superbunching effect with a bunching peak much larger than 2, the theoretical bunching peak of thermal light. Experimentally, we demonstrated a bunching peak of $11.72\ifmmode\pm\else\textpm\fi{}0.05$ with the digitally designed phase-correlated wave front of classical light, which can be improved further on. A significant improvement of the visibility of the second-order interference fringes and ghost imaging was also experimentally demonstrated. Our method provides a convenient digitally controllable way to implement superposition of multiple different but indistinguishable two-photon paths, and therefore to modify the optical coherence properties of photons. Such a superbunching effect may have potential applications in improving the visibility of correlation interference and imaging, and enhancing the efficiency of two-photon nonlinear effects such as two-photon absorption effect.
Two-photon bunching and superbunching are important to understanding the physics of ghost imaging and second-order interference of light. With the help of the recently proposed superbunching pseudothermal light, the physics of bunching and superbunching in superbunching pseudothermal light is studied in detail. A special two-photon coincidence count detection system is designed to measure the required two-photon coincidence counts. It is concluded that the two-photon superbunching effect cannot be observed without taking the intensity changing process into account. A similar conclusion holds for two-photon bunching of thermal light. The conclusions are helpful for understanding of the physics of two-photon bunching and superbunching in intensity or photon number fluctuation correlation theory.
Three-photon superbunching is experimentally observed with the recently proposed superbunching pseudothermal light. To the best of our knowledge, it is the first time that three-photon superbunching is observed with classical light in a linear optical system. From the quantum optics point of view, three-photon superbunching is interpreted as the result of constructive-destructive three-photon interference. The key to observe three-photon superbunching with superbunching pseudothermal light is that all the different ways to trigger a three-photon coincidence count are in principle indistinguishable, which is experimentally guaranteed by putting a pinhole before each rotating ground glass to ensure that all the passed photons are within the same coherence area. The observed three-photon superbunching is helpful to increase the visibility of ghost imaging and understand the physics of third-order interference of light.
Multi-photon nonlinear processes in atoms have served as important tools for quantum metrology, quantum communications, and quantum sensing. In this thesis, we experimentally address the interplay of various multi-photon Raman processes in hot Rb vapor, with the four-wave mixing (FWM) process being a central theme. FWM is the nonlinear response of a medium to a strong optical pump field inelastically scattering off atomic resonances and resulting in the generation of additional photons in different modes. FWM is a detrimental, but inherent part of electromagnetically induced transparency (EIT) and Raman based quantum memories. However, we were able to weaken the four-photon resonance by utilizing two-photon absorption to remove the additional photons without interfering with the signal beam. We also demonstrate the ability to tailor FWM to generate new photons in a controlled fashion for mode conversion. With this, we showed the conversion of 795 nm light to 420 nm light. While FWM is a source of noise in quantum memories, it can also be used for the generation squeezed twin-beams. Such beams have relative intensity noise reduced below the classical shot noise limit and share mode dependence based on the phase-matching conditions. Using this, we demonstrated that twin-beams can be generated with largely different spatial structure (optical angular momentum) and still share strong correlations, so long as the phase-matching conditions are satisfied. We then constructed and demonstrated the operation of a polarization-based quantum interferometer using squeezed twin-beams and showed that our beams were entangled under the inseparability condition. Using this interferometer, we were also able to achieve squeezing at low detection frequencies, which is necessary for things like quantum imaging and gravitational wave detection. We also demonstrated that squeezed twin-beams can be utilized to enhance the sensitivity of two-photon absorption spectroscopy. This research has touched on many different subjects related to quantum information science and improved upon some of the tools needed for the implementation of such technologies.
Superbunching pseudothermal light has important applications in studying the second- and higher-order interference of light in quantum optics. Unlike the photon statistics of thermal or pseudothermal light is well understood, the photon statistics of superbunching pseudothermal light has not been studied yet. In this paper, we will employ single-photon detectors to measure the photon statistics of superbunching pseudothermal light and calculate the degree of second-order coherence. It is found that the larger the value of the degree of second-order coherence of superbunching pseudothermal light is, the more the measured photon distribution deviates from the one of thermal or pseudothermal light in the tail part. The results are helpful to understand the physics of two-photon superbunching with classical light. It is suggested that superbunching pseudothermal light can be employed to generate non-Rayleigh temporal speckles.