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Proceedings annual meeting Electron Microscopy Society of America

Interferometric (Fourier-Spectroscopic) Measurement of Electron Energy Distributions

FRANZ HASSELBACH, A. Schäfer

Published Aug 12, 1990• 5 citations
Publisher

Abstract

Möllenstedt and Wohland proposed in 1980 two methods for measuring the coherence lengths of electron wave packets interferometrically by observing interference fringe contrast in dependence on the longitudinal shift of the wave packets. In both cases an electron beam is split by an electron optical biprism into two coherent wave packets, and subsequently both packets travel part of their way to the interference plane in regions of different electric potential, either in a Faraday cage (Fig. 1a) or in a Wien filter (crossed electric and magnetic fields, Fig. 1b). In the Faraday cage the phase and group velocity of the upper beam (Fig.1a) is retarded or accelerated according to the cage potential. In the Wien filter the group velocity of both beams varies with its excitation while the phase velocity remains unchanged. The phase of the electron wave is not affected at all in the compensated state of the Wien filter since the electron optical index of refraction in this state equals 1 inside and outside of the Wien filter.

DOI
10.1017/s0424820100134144

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Möllenstedt and Wohland proposed in 1980 two methods for measuring the coherence lengths of electron wave packets interferometrically by observing interference fringe contrast in dependence on the longitudinal shift of the wave packets. In both cases an electron beam is split by an electron optical biprism into two coherent wave packets, and subsequently both packets travel part of their way to the interference plane in regions of different electric potential, either in a Faraday cage (Fig. 1a) or in a Wien filter (crossed electric and magnetic fields, Fig. 1b). In the Faraday cage the phase and group velocity of the upper beam (Fig.1a) is retarded or accelerated according to the cage potential. In the Wien filter the group velocity of both beams varies with its excitation while the phase velocity remains unchanged. The phase of the electron wave is not affected at all in the compensated state of the Wien filter since the electron optical index of refraction in this state equals 1 inside and outside of the Wien filter.
Longitudinal coherence in two-beam interferometers means that the two partial wave packets arrive in the plane of interference simultaneously. In charged-particle interferometers, this simultaneity can be lost due to a difference in the geometrical path lengths, a difference in the optical path length, or a difference in the group velocities for the two wave packets on parts of or all of the beam paths. Several of those influences can combine to yield a net relative spatial delay between the wave packets in the interference plane, thus causing a reduction of the interference fringe contrast. A Wien filter can be used in charged-matter-wave interferometry to compensate for this relative delay and thus to reestablish longitudinal coherence. A Wien filter consists of an electric and a magnetic field perpendicular both to each other and the beam path. In its matched state, i.e., when the electrostatic and the magnetic forces on the electrons exactly cancel each other, the Wien filter neither deflects the beams nor exerts any phase shift on the wave packets. However, wave packets traveling through the Wien filter on laterally separated paths propagate in regions of different electric potentials and in turn with different group velocities, which leads to a longitudinal shift of the wave packets relative to each other. Maximum longitudinal coherence (and thereby fringe contrast) can be restored by choosing the compensating delay caused by the Wien filter exactly opposite to the net relative delay caused by the influences mentioned.An experiment is presented that demonstrates this property of a Wien filter. The coherence-reviving action of a Wien filter is discussed in the context of the incoherent superposition in the registration plane of the plane waves corresponding to different wavelengths in the electron spectrum. It demonstrates that the quantum-mechanical coherence of the self-interacting plane-wave components of the wave packets describing the particle ensemble is more robust than the experimental loss of interference-fringe contrast often suggests. The availability of such a contrast-restoring device is especially important for very-low-energy (a few keV or less) electron interferometry. It is also likely to become important for future ion-beam interferometers.
Electron double-slit experiments, the essence of quantum mechanical “wave/particle duality”, have been extensively and continuously studied because their unrealistic interpretations have attracted many researchers. Here, we discuss recent sophisticated V-shaped double-slit experiments to elucidate electron-path information, i.e., which slit electrons pass through, which path they pursue, and where they arrive and interfere on the image plane. In a transmission electron microscope, an optically zero-propagation distance condition was realized, where the double-slit position was imaged just on the detector plane. Interference fringes composed of dot images were controlled by using two electron biprisms. Using a V-shaped double slit, we confirmed that it is possible to observe interference fringes only when the path information of individual electrons is not available. Furthermore, we studied how the interference fringes would shift their detected positions when electron wave phases were modulated before illumination to the double slit. Phase shifts were generated by tilting electron beams. We confirmed that each single electron as a wave changed its phase even when it traveled alone inside the microscope.
Electron double-slit experiments, the essence of quantum mechanical “wave/particle duality,” have been extensively and continuously studied because their unrealistic interpretations have attracted many researchers. Here, we discuss recent sophisticated V-shaped double-slit experiments to elucidate electron-path information, i.e., which slit electrons pass through, which path they pursue, and where they arrive and interfere on the image plane. In a transmission electron microscope, an optically zero-propagation distance condition was realized, where the double-slit position was imaged just on the detector plane. Interference fringes composed of dot images were controlled by using two electron biprisms. Using a V-shaped double slit, we confirmed that it is possible to observe interference fringes only when the path information of individual electrons is not available. Furthermore, we studied how the interference fringes would shift their detected positions when electron wave phases were modulated before illumination to the double slit. Phase shifts were generated by tilting electron beams. We confirmed that each single electron as a wave changed its phase even when it traveled alone inside the microscope.
The coherence length of a neutron wave packet depends on the spectral width of the distribution of wave vectors that make up the packet. The coherent overlap of the wave packets traversing the two beam paths in a perfect-silicon-crystal neutron interferometer (NI) is altered by placing a material with a neutron-nuclear optical potential in one of the beam paths in the NI. If the optical potential is positive, it causes a delay of the wave packet and a loss of fringe visibility. By use of an analyzer crystal, we narrow the spectral distribution after the mixing and interference has occurred in the last crystal slab of the NI. This increases the coherence length and restores some of the fringe visibility.
We propose a two-dimensional interferometry based on the electron wave-packet interference by using a cycle-shaped orthogonally polarized two-color laser field. With such a method, the subcycle and intercycle interferences can be disentangled into different directions in the measured photoelectron momentum spectra. The Coulomb influence can be minimized and the overlapping of interference fringes with the complicated low-energy structures can be avoided as well. The contributions of the excitation effect and the long-range Coulomb potential can be traced in the Fourier domain of the photoelectron distribution. Because of these advantages, precise information on valence electron dynamics of atoms or molecules with attosecond temporal resolution and additional spatial information with angstrom resolution can be obtained with the two-dimensional electron wave-packet interferometry.
An experiment is described which is an analog of Young's double-slit interferometer using an atomic electron instead of light. Two phase-coherent laser pulses are used to excite a single electron into a state of the form of a pair of Rydberg wave packets that are initially on opposite sides of the orbit. The two wave packets propagate and spread until they completely overlap, then a third phase-coherent laser pulse probes the resulting fringe pattern. The relative phase of the two wave packets is varied so that the interference produces a single localized electron wave packet on one side of the orbit or the other.