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Research

Spatial Wavefunction Characterization of Femtosecond Pulses at Single-Photon Level

Billy Lam, Mohamed ElKabbash, Jihua Zhang, Chunlei Guo

Published Jan 1, 2020• 6 citations
Publisher

Abstract

Reading quantum information of single photons is commonly realized by quantum tomography or the direct (weak) measurement approach. However, these methods are time-consuming and face enormous challenges in characterizing single photons from an ultrafast light source due to the stringent temporal mode matching requirements. Here, we retrieve the spatial wavefunction of indistinguishable single photons from both a continuous wave source and a femtosecond light source using a self-referencing interferometer. Our method only requires nine ensemble-averaged measurements. This technique simplifies the measurement procedure of single-photon wavefunction and automatically mode matches each self-interfering single photon temporally, which enables the measurement of the spatial wavefunction of single photons from an ultrafast light source.

DOI
10.34133/2020/2421017

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Reading quantum information of single photons is commonly realized by quantum tomography or the direct (weak) measurement approach. However, these methods are time-consuming and face enormous challenges in characterizing single photons from an ultrafast light source due to the stringent temporal mode matching requirements. Here, we retrieve the spatial wavefunction of indistinguishable single photons from both a continuous wave source and a femtosecond light source using a self-referencing interferometer. Our method only requires nine ensemble-averaged measurements. This technique simplifies the measurement procedure of single-photon wavefunction and automatically mode matches each self-interfering single photon temporally, which enables the measurement of the spatial wavefunction of single photons from an ultrafast light source.
The large capacity and robustness of information encoding in the temporal mode of photons is important in quantum information processing, in which characterizing temporal quantum states with high usability and time resolution is essential. We propose and demonstrate a direct measurement method of temporal complex wavefunctions for weak light at a single-photon level with subpicosecond time resolution. Our direct measurement is realized by ultrafast metrology of the interference between the light under test and self-generated monochromatic reference light; no external reference light or complicated post-processing algorithms are required. Hence, this method is versatile and potentially widely applicable for temporal state characterization.
Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.
Quantitative characterization of the spatial structure of single photons is essential for free-space quantum communication and quantum imaging. We introduce an interferometric technique that enables the complete characterization of a two-dimensional probability amplitude of a single photon. Importantly, in contrast to methods that use a reference photon for the phase measurement, our technique relies on a single photon interfering with itself. Our setup comprises of a heralded single-photon source with an unknown spatial phase and a modified Mach-Zehnder interferometer with a spatial filter in one of its arms. The spatial filter removes the unknown spatial phase and the filtered beam interferes with the unaltered beam passing through the other arm of the interferometer. We experimentally confirm the feasibility of our technique by reconstructing the spatial phase of heralded single photons using the lowest order interference fringes. This technique can be applied to the characterization of arbitrary pure spatial states of single photons.
The ability to characterize the complete quantum state of light is essential for both fundamental and applied science. For single photons the quantum state is provided by the mode that it occupies. The spectral temporal mode structure of light has recently emerged as an essential means for quantum information science. Here we experimentally demonstrate a self-referencing technique to completely determine the pulse-mode structure of single photons by means of spectral shearing interferometry. We detail the calibration and resolution of the measurement and discuss challenges and critical requirements for future advances of this method.
Energy-time entangled photons are critical in many quantum optical phenomena and have emerged as important elements in quantum information protocols. Entanglement in this degree of freedom often manifests itself on ultrafast time scales, making it very difficult to detect, whether one employs direct or interferometric techniques, as photon-counting detectors have insufficient time resolution. Here, we implement ultrafast photon counters based on nonlinear interactions and strong femtosecond laser pulses to probe energy-time entanglement in this important regime. Using this technique and single-photon spectrometers, we characterize all the spectral and temporal correlations of two entangled photons with femtosecond resolution. This enables the witnessing of energy-time entanglement using uncertainty relations and the direct observation of nonlocal dispersion cancellation on ultrafast time scales. These techniques are essential to understand and control the energy-time degree of freedom of light for ultrafast quantum optics.
Summary form only given. The spatial structure of a photon has proved to be indispensable resource allowing the experimental realization of free-space quantum cryptography or high dimensional entanglement. Although efficient methods for manipulating spatial characteristic of individual photons can be easily transferred from the field of classical optics, their spatial structure cannot be measured using the standard interferometric reference-based methods such as optical holography due to their completely undefined-global phase. Hence, the full recovery of a transverse photon wavefunction still remains a challenging task tackled so far exclusively using indirect methods such as the quantum tomography [1] and weak values measurements [2].Here we present and experimentally demonstrate a different approach based on spatially resolved detection of two-photon interference [3,4]. Although such measurements are usually perceived to be insensitive to the relative phase between two interfering photons we show that rarely considered local phase dependence can be still observed and utilized for direct recovery of a single photon quantum wavefunction. In particular we experimentally show that the complex transversal wavefunction of the unknown photon can be fully recovered from the 2D spatial coincidence pattern resulting from its two-photon interference with the reference photon [5].