Stark mixing under full interaction in ion-Rydberg atom cold collisions

M. Raymond Flannery, D. Vrinceanu

Dean M. Homan

David M. Feldbaum

We have studied the development of gases of ultra-cold Rydberg atoms in Magneto Optic Traps, and discovered that such gases exhibit a range of density-dependent phenomena. In particular, we have found that at the densities of ∼ 10 7 cm -3 the Rydberg atoms spontaneously evolve into long-lived high angular momentum states. These states slowly decay due to microwave background radiation over tens of milliseconds. We have numerically simulated the effects leading to such behavior, and investigated numerically the l- and n-mixing collisions of Rydberg atoms with electrons in the range of 10 meV. These calculations show that the l- and n-mixing cross-sections follow the n 5 scaling law, expected from simple Stark map considerations, but also depend on the velocities of the colliding electrons, reflecting the adiabaticity of the atom-electron interactions. We have developed a novel technique of measuring the electric fields inside plasmas by using Rydberg excitation spectroscopy of embedded atoms, based on the disappearance of regions of zero oscillator strength in the presence of such fields. We have applied this technique to study the evolution of ultra-cold non-neutral plasmas excited from the MOT, and have found that it expands over 1 mus. We have simulated such an expansion by considering only Coulomb repulsion between the constituent ions, and have found that such a model is consistent with the experimental observations.

Moritz Berngruber, Daniel J. Bosworth, O. A. Herrera-Sancho +8 more

The onset of collision dynamics between an ion and a Rydberg atom is studied in a regime characterized by a multitude of collision channels. These channels arise from coupling between a nonpolar Rydberg state and numerous highly polar Stark states. The interaction potentials formed by the polar Stark states show a substantial difference in spatial gradient compared to the nonpolar state leading to a separation of collisional timescales, which is observed in situ. For collision energies in the range of k_{B}μK to k_{B}K, the dynamics exhibit a counterintuitive dependence on temperature, resulting in faster collision dynamics for cold-initially "slow"-systems. Dipole selection rules enable us to prepare the collision pair on the nonpolar potential in a highly controlled manner, which determines occupation of the collision channels. The experimental observations are supported by semiclassical simulations, which model the pair state evolution and provide evidence for tunable nonadiabatic dynamics.

Robert R. Lewis, Araceli Góngora

André Luiz de Oliveira, M. Mancini, Vanderlei Salvador Bagnato +1 more