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OptSp

Photon echo based on optical nutation

Aleksey I. Alekseev, Ashat M. Basharov

Published May 1, 1979• 0 citations
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Physical Review Letters•Sep 6, 1971•338 citations
Photon echo and optical nutation have been easily observed in C13{\mathrm{C}}^{13}C13H3{\mathrm{H}}_{3}H3​F and NH2{\mathrm{H}}_{2}H2​D by applying Stark pulses which shift the molecular levels into resonance with cw laser radiation. Numerical computations of the nutation effect agree with observation, and echo characteristics closely follow predictions of existing theories. The $T_{2}^{}{}_{}{}^{\ensuremath{'}}$ pressure dependence, from infrared-echo measurements, indicates that C13{\mathrm{C}}^{13}C13H3{\mathrm{H}}_{3}H3​F relaxes primarily by rotational energy transfer.