Ultradilute quantum droplets are intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in low-dimensional two-component Bose-Bose mixtures, by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the inter-species attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In one dimension, we find that the energy calculated by the pairing theory is in an excellent agreement with the latest diffusion Monte Carlo simulation {[}Phys. Rev. Lett. \textbf{122}, 105302 (2019){]}, for nearly all the interaction strengths at which quantum droplets exist. In two dimensions, we show that quantum droplets disappear and may turn into a soliton-like many-body bound state, when the inter-species attraction exceeds a critical value. Below the threshold, the pairing theory predicts more or less the same results as the Bogoliubov theory derived by Petrov and Astrakharchik {[}Phys. Rev. Lett. \textbf{117}, 100401 (2016){]}. The predicted energies from both theories are higher than the diffusion Monte Carlo results, due to the weak inter-species attraction and the increasingly important role played by the beyond-Bogoliubov-approximation effect in two dimensions. Our pairing theory provides an ideal starting point to understand interesting ground-state properties of quantum droplets, including their shape and collective oscillations.
Ultradilute quantum droplets are intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in low-dimensional two-component Bose-Bose mixtures, by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the inter-species attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In one dimension, we find that the energy calculated by the pairing theory is in an excellent agreement with the latest diffusion Monte Carlo simulation {[}Phys. Rev. Lett. \textbf{122}, 105302 (2019){]}, for nearly all the interaction strengths at which quantum droplets exist. In two dimensions, we show that quantum droplets disappear and may turn into a soliton-like many-body bound state, when the inter-species attraction exceeds a critical value. Below the threshold, the pairing theory predicts more or less the same results as the Bogoliubov theory derived by Petrov and Astrakharchik {[}Phys. Rev. Lett. \textbf{117}, 100401 (2016){]}. The predicted energies from both theories are higher than the diffusion Monte Carlo results, due to the weak inter-species attraction and the increasingly important role played by the beyond-Bogoliubov-approximation effect in two dimensions. Our pairing theory provides an ideal starting point to understand interesting ground-state properties of quantum droplets, including their shape and collective oscillations.
Ultradilute quantum droplets are an intriguing new state of matter, in which the attractive mean-field force can be balanced by the repulsive force from quantum fluctuations to avoid collapse. Here, we present a microscopic theory of ultradilute quantum droplets in three-, one-, and two-dimensional two-component Bose-Bose mixtures by generalizing the conventional Bogoliubov theory to include the bosonic pairing arising from the interspecies attraction. Our pairing theory is fully equivalent to a variational approach and hence gives an upper bound for the energy of quantum droplets. In three dimensions, we predict the existence of a strongly interacting Bose droplet at the crossover from Bose-Einstein condensates (BECs) to BCS superfluids and map out the bosonic BEC-BCS crossover phase diagram. In one dimension, we find that the energy of the one-dimensional Bose droplet calculated by the pairing theory is in excellent agreement with the latest diffusion Monte Carlo simulation [L. Parisi et al., Phys. Rev. Lett. 122, 105302 (2019)] for nearly all the interaction strengths at which quantum droplets exist. In two dimensions, we show that Bose droplets disappear and may turn into a solitonlike many-body bound state, when the interspecies attraction exceeds a critical value. Below the threshold, the pairing theory predicts more or less the same results as the Bogoliubov theory derived by D. S. Petrov and G. E. Astrakharchik [Phys. Rev. Lett. 117, 100401 (2016)]. The predicted energies from both theories are higher than the diffusion Monte Carlo results due to the weak interspecies attraction and the increasingly important role played by the beyond-Bogoliubov-approximation effect in two dimensions. Our pairing theory provides an ideal starting point to understand interesting ground-state properties of quantum droplets in various dimensions, including their shape and collective oscillations.
We revisit the Bogoliubov theory of quantum droplets proposed by Petrov [Phys. Rev. Lett. 115, 155302 (2015)PRLTAO0031-900710.1103/PhysRevLett.115.155302] for an ultracold Bose-Bose mixture, where the mean-field collapse is stabilized by the Lee-Huang-Yang quantum fluctuations. We show that a loophole in Petrov's theory, i.e., the ignorance of the softening complex Bogoliubov spectrum, can be naturally removed by the introduction of bosonic pairing. The pairing leads to weaker mean-field attractions, and also a stronger Lee-Huang-Yang term in the case of unequal intraspecies interactions. As a result, the equilibrium density for the formation of self-bound droplets significantly decreases in the deep droplet regime, in agreement with a recent observation from diffusion Monte Carlo simulations. Our construction of a consistent Bogoliubov theory paves the way to understand the puzzling low critical number of small quantum droplets observed in the experiment [C. Cabrera et al., Science 359, 301 (2018)SCIEAS0036-807510.1126/science.aao5686].
In his seminal proposal of quantum droplets in binary Bose mixtures [D. Petrov, Phys. Rev. Lett. 115, 155302 (2015)], Petrov suggested that the density ratio n2/n1 of the two bosonic components is locked to an optimal value, which is given by the square root of the ratio of the two intraspecies scattering lengths, i.e., a11/a22. Due to such density locking, quantum droplets can be efficiently described by using an extended Gross-Pitaevskii equation within the single-mode approximation. Here, we find that this single-mode description necessarily breaks down in the deep quantum droplet regime, when the attractive interspecies scattering length a12 significantly deviates away from the threshold of mean-field collapse (i.e., $\ensuremath{-}\sqrt{{a}_{11}{a}_{22}}$). By applying a bosonic pairing theory, we show that the density ratio is allowed to fluctuate in a sizable interval. Most importantly, the optimal density ratio would be very different from a11/a22, in the case of unequal intraspecies scattering lengths (${a}_{11}\ensuremath{\ne}{a}_{22}$). Our finding might provide a plausible microscopic explanation of the puzzling low critical particle number of quantum droplets, as experimentally observed. Our predicted interval of the density ratio, as a function of the interspecies scattering length, could also be experimentally examined in cold-atom laboratories in the near future.
An ultradilute quantum droplet is a self-bound liquidlike state recently observed in ultracold Bose-Einstein condensates. In most previous theoretical studies, it is described by a phenomenological low-energy effective theory, termed as the extended Gross-Pitaevskii equation. Here, we microscopically derive the Gross-Pitaevskii equation for the condensate and also for a pairing field in an inhomogeneous quantum droplet realized by Bose-Bose mixtures with attractive interspecies interaction. We show that the inclusion of the pairing field is essential, in order to have a consistent description of the droplet state. We clarify that the extended Gross-Pitaevskii equation used earlier should be understood as the equation of motion for the pairing field, rather than the condensate. The fluctuations of the pairing field give rise to low-energy collective excitations of the droplet. We also present the Bogoliubov equations for gapless phonon modes and gapped modes due to pairing in real space, which characterizes single-particle-like excitations of the droplet. The equations of motion derived in this work for the condensate and the pairing field serve as an ideal starting point to understand the structure and collective excitations of nonuniform ultradilute quantum droplets in ongoing cold-atom experiments.
Among settings which have recently been elaborated for the creation of stable multidimensional solitons, most advanced, as concerns the theory and experiment alike, is the work with quantum droplets (QDs) in atomic BEC. Important theoretical predictions for fundamental and topologically structured soliton-like (stably self-trapped) QDs have been published in many papers, starting from the pioneering work of Petrov [Phys. Rev. Lett. 115, 155302 (2015)]. Simultaneously, the experimental advancement in the making of QDs in binary BECs, as well as in single-component BECs of atoms carrying magnetic dipole moments, have been really remarkable and unique. Successful experiments followed the first theoretical prediction of the QDs very quickly, and the progress in the experimental work was much faster than in other areas of physics where stable multidimensional solitons were predicted. The basis of these works is a correction to the MF (mean-field) BEC dynamics produced by quantum fluctuations around MF states. The correction was first predicted in 1957 by Lee, Huang, and Yang (LHY). The breakthrough proposal made by Petrov [Phys. Rev. Lett. 115, 155302 (2015)] was to use the effective higher-order (quartic) self-repulsion, produced by the LHY effect in the atomic BEC, as a mechanism arresting the collapse driven by mutual attraction of two self-repulsive components in a binary quantum bosonic gas. The balance between the inter-species attraction and LHY-induced self-repulsion gives rise to stable 3D and quasi-2D (pancake-shaped) localized bound states in the form of the quantum droplets (QDs). In single-component condensates of magnetic atoms, the attraction is provided by the long-range dipole–dipole interaction (Chomaz et al., 2016; Schmitt et al., 2016). The competition between the MF attraction and LHY repulsion maintains a superfluid state whose density (taking very low values) cannot exceed a certain maximum, thus making it effectively incompressible. This is a reason why this quantum macroscopic state of matter is identified as a superfluid. Accordingly, localized states filled by this quantum fluid are called “droplets.” In addition to the 3D QDs, droplets in the effectively 2D setting, which may exist under the action of tight confinement in one direction, imposed by an external potential, were theoretically predicted [Petrov and Astrakharchik, Phys. Rev. Lett. 117, 100401 (2016)] and experimentally created [Cabrera et al., Science 359, 301-304 (2018)] too. This chapter provides a condensed review of basic theoretical results for stable QDs in binary BECs, maintained through the stable balance between the inter-species attraction and intra-species LHY repulsion. Both fundamental modes and ones with embedded vorticity are considered. The presentation is partly based on a review article by Luo et al. [Front. Phys. 16, 32501 (2021)]. In addition to 2D and 3D self-trapped QDs in free space, the present chapter addresses 2D fundamental and vortex modes trapped in a singular attractive potential, ∼−1/r2, which are stabilized by the LHY repulsion. Two subsequent chapters present a summary of experimental findings for QDs in binary BECs and for QDs in single-component BECs of magnetic atoms.