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Accelerated adiabatic quantum control

Francesco Petiziol

Published Mar 1, 2020• 0 citations
OpenAlex

Abstract

The challenge to fully grasp and to harness the bizarre phenomena which take place in the quantum realm is crucially linked to the ability to engineer and manipulate quantum systems with high precision. The scientific progress in this direction is opening new routes for the investigation of fundamental quantum physics, and it is at the same time paving the way to the development of the first quantum technologies. \n\nThis thesis is dedicated to the search of strategies for high-fidelity and noise-tolerant quantum control.\nA versatile theoretical framework is set up for the design of optimized control protocols based on accelerated adiabatic processes. The benefits of the adiabatic dynamics, rooted in its intrinsic stability versus control imperfections, are released from the requirement of slow evolution: this is achieved thanks to the theoretical construction of accelerating control Hamiltonians which dynamically counteract deviations from the target dynamics. Our framework provides a methodical way to engineer these Hamiltonians by introducing fast modulations of the initially-available control parameters, and it results from the interplay between the theory of counterdiabatic fields and Floquet-Magnus average Hamiltonian theory. As compared to other shortcut-to-adiabaticity strategies, our control method keeps the system always close to the exact adiabatic path while not requiring the implementation of new Hamiltonian couplings. Moreover, the flexibility in the construction of the accelerating Hamiltonians offers a fertile ground for the hybridization with optimal control techniques.\n\nThe general setup is applied to exemplary control problems of relevance in quantum optics and quantum information processing. First, a protocol is designed for the generation of entanglement between effective two-level systems coupled through a transmission line, in the experimental context of circuit quantum electrodynamics. Second, an accelerated version of the widespread technique of stimulated Raman adiabatic passage is presented, which dramatically enlarges its range of applicability for implementations both in the optical and in the microwave regime.\n\nThe results strongly support the potential of the quantum control framework developed in this thesis. In particular, our methodology offers the opportunity to flank high fidelities and small error sensitivity with on-demand adaptability to experimental constraints and the flexibility for integrations with other control techniques. This makes it a valuable resource for applications in many branches of quantum science, with a natural outlet in quantum computation and simulation.

Related papers

Shortcuts to adiabaticity for open systems in circuit quantum electrodynamics

Zelong Yin, Chunzhen Li, Jonathan Allcock +5 more

Shortcuts to adiabaticity are powerful quantum control methods, allowing quick evolution into target states of otherwise slow adiabatic dynamics. Such methods have widespread applications in quantum technologies, and various shortcuts to adiabaticity protocols have been demonstrated in closed systems. However, realizing shortcuts to adiabaticity for open quantum systems has presented a challenge due to the complex controls in existing proposals. Here, we present the experimental demonstration of shortcuts to adiabaticity for open quantum systems, using a superconducting circuit quantum electrodynamics system. By applying a counterdiabatic driving pulse, we reduce the adiabatic evolution time of a single lossy mode from 800 ns to 100 ns. In addition, we propose and implement an optimal control protocol to achieve fast and qubit-unconditional equilibrium of multiple lossy modes. Our results pave the way for precise time-domain control of open quantum systems and have potential applications in designing fast open-system protocols of physical and interdisciplinary interest, such as accelerating bioengineering and chemical reaction dynamics.

arXiv:2107.08417•Nature Communications•Jan 10, 2022•35 citations

Optimized three-level quantum transfers based on frequency-modulated optical excitations

Francesco Petiziol, E. Arimondo, Luigi Giannelli +2 more

The difficulty in combining high fidelity with fast operation times and robustness against sources of noise is the central challenge of most quantum control problems, with immediate implications for the realization of quantum devices. We theoretically propose a protocol, based on the widespread stimulated Raman adiabatic passage technique, which achieves these objectives for quantum state transfers in generic three-level systems. Our protocol realizes accelerated adiabatic following through the application of additional control fields on the optical excitations. These act along frequency sidebands of the principal adiabatic pulses, dynamically counteracting undesired transitions. The scheme facilitates experimental control, not requiring new hardly-accessible resources. We show numerically that the method is efficient in a very wide set of control parameters, bringing the timescales closer to the quantum speed limit, also in the presence of environmental disturbance. These results hold for complete population transfers and for many applications, e.g., for realizing quantum gates, both for optical and microwave implementations. Furthermore, extensions to adiabatic passage problems in more-level systems are straightforward.

Scientific Reports•Feb 10, 2020•27 citations

Adiabatic control in circuit quantum electrodynamics

Antti P. Vepsäläinen

In circuit quantum electrodynamics the coherence of Cooper pairs in superconductors is employed to create macroscopic electric circuits with quantized energy levels. Such circuits can be coupled with each other and exploited as building blocks of a quantum computer. Accurate and robust control of the quantum state in the circuits is a central condition for the operation of the quantum computer and one of the prerequisites for the implementation of complex algorithms used in quantum information processing, such as quantum error correction. In this thesis adiabatic control in circuit quantum electrodynamics is investigated with the focus on manipulating three-level systems. \n \nIn adiabatic control the eigenstates of the system are slowly modified by changing the external control parameters, which govern the evolution of the system. If the changes in the parameters are slow enough, the state of the system follows the eigenstates in the adiabatic basis, thereby realizing the intended operation. The advantage of adiabatic control is its inherent robustness to small errors or noise in the control parameters; the result of the state manipulation only depends on the asymptotic values of the control parameters, but not on their exact values during the process. \n \nShortcuts to adiabaticity can be used to speed up the otherwise slow adiabatic control by introducing a correction pulse that compensates the diabatic losses during the state manipulation. This allows one to overcome the limitation on the speed of the protocol but simultaneously reduces the method's robustness to the variations in the control parameters. If the level of noise in the control parameters is known, using the shortcut it is possible to find the optimal level of robustness which is required to mitigate the noise. \n \nCircuit quantum electrodynamics offers a perfect experimental platform for investigating quantum control due to the possibility of realizing complicated control schemes using microwave electronics. With commercially available digital-to-analog converters the control signals can be digitally created, which enables accurate and coherent control of the quantum circuit. \n \nIn this thesis both theoretical and experimental results on adiabatic control applied to superconducting transmon circuits are presented. It is shown that stimulated Raman adiabatic passage can be used for population transfer in a three-level transmon, which can be further improved using shortcuts to adiabaticity. Furthermore, a scheme for implementing robust superadiabatic rotation gates in transmon is proposed. Finally, it is demonstrated that superconducting qubit can be used as an ultra-sensitive detector of magnetic flux.

•Jan 1, 2018•0 citations

Shortcuts To Adiabaticity: Theory and Application

Xi Chen

By definition, quantum adiabatic process means a slow process which allows the state to follow the instantaneous eigenstates of time-dependent Hamiltonian. For some reasons, for example, to avoid the decoherence effects, or to implement large-scale quantum information processing, we may want to speed up the adiabatic process, that is, to achieve the adiabatic-like control but in very short time. In this talk, we present new methods to speeded-up expansion and transport of cold atoms in a harmonic trap. Such shortcuts to adiabaticity provide the fast expansion or transport, in which the final atomic state is the same as in the adiabatic process, but in arbitrarily short time, keeping the same populations of vibrational levels in the initial and final trap. These methods can also be generalized to Bose-Einstein Condensates. Moreover, we present shortcuts to adiabatic passage from one internal atomic state to another in twoor three-level atoms. In detail, we can apply Berry’s transitionless quantum driving method and invariant-based inverse engineering method to accelerate the Rapid Adiabatic Passage (RAP) and Stimulated Raman Adiabatic Passage (STIRAP) in twoand three-level atomic systems, respectively. We also examine and compare the stability of different schemes concerning different types of noise and system errors. Finally, we show that the technique of shortcuts to adiabaticity in two-level system can be applied in fast and robust spin flip in a quantum dot, to avoid the decoherent effects.

•Jan 1, 2012•0 citations

Numerical Engineering of Adiabatic Quantum Operations

Seyed Sahand Tabatabaei

Adiabatic quantum operations are ubiquitous in fields such as quantum information processing, quantum control, and magnetic resonance, where their high fidelity and general robustness renders them an essential tool for various applications. This inherent robustness due to adiabaticity can, however, be impaired in cases where the experimental conditions strictly require very fast evolution times. In this thesis, we provide a gradient-based numerical optimization protocol for efficiently engineering adiabatic operations, allowing for the systematic inclusion of robustness criteria against various experimental non-idealities, including inhomogeneities and uncertainties in system parameters, as well as perturbations in the Hamiltonian such as spin-spin interactions. \nThe protocol is implemented in the context of adiabatic passages for magnetic resonance, and \nit is shown that in addition to conventional adiabatic pulses, it can also generate exceptionally fast operations that although slightly deviate from adiabaticity in limited instances, still lead to a high fidelity. \nThe effectiveness of our method for addressing perturbations is also demonstrated by designing a fast adiabatic passage for dipolar-coupled electrons, and numerically comparing its performance with a pulse without such considerations.

•Jan 23, 2020•0 citations

Quantum control theory for coherence and information dynamics

Lorenza Viola, David J. Tannor

Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.

Journal of Physics B Atomic Molecular and Optical Physics•Jul 25, 2011•6 citations
The challenge to fully grasp and to harness the bizarre phenomena which take place in the quantum realm is crucially linked to the ability to engineer and manipulate quantum systems with high precision. The scientific progress in this direction is opening new routes for the investigation of fundamental quantum physics, and it is at the same time paving the way to the development of the first quantum technologies. \n\nThis thesis is dedicated to the search of strategies for high-fidelity and noise-tolerant quantum control.\nA versatile theoretical framework is set up for the design of optimized control protocols based on accelerated adiabatic processes. The benefits of the adiabatic dynamics, rooted in its intrinsic stability versus control imperfections, are released from the requirement of slow evolution: this is achieved thanks to the theoretical construction of accelerating control Hamiltonians which dynamically counteract deviations from the target dynamics. Our framework provides a methodical way to engineer these Hamiltonians by introducing fast modulations of the initially-available control parameters, and it results from the interplay between the theory of counterdiabatic fields and Floquet-Magnus average Hamiltonian theory. As compared to other shortcut-to-adiabaticity strategies, our control method keeps the system always close to the exact adiabatic path while not requiring the implementation of new Hamiltonian couplings. Moreover, the flexibility in the construction of the accelerating Hamiltonians offers a fertile ground for the hybridization with optimal control techniques.\n\nThe general setup is applied to exemplary control problems of relevance in quantum optics and quantum information processing. First, a protocol is designed for the generation of entanglement between effective two-level systems coupled through a transmission line, in the experimental context of circuit quantum electrodynamics. Second, an accelerated version of the widespread technique of stimulated Raman adiabatic passage is presented, which dramatically enlarges its range of applicability for implementations both in the optical and in the microwave regime.\n\nThe results strongly support the potential of the quantum control framework developed in this thesis. In particular, our methodology offers the opportunity to flank high fidelities and small error sensitivity with on-demand adaptability to experimental constraints and the flexibility for integrations with other control techniques. This makes it a valuable resource for applications in many branches of quantum science, with a natural outlet in quantum computation and simulation.
Shortcuts to adiabaticity are powerful quantum control methods, allowing quick evolution into target states of otherwise slow adiabatic dynamics. Such methods have widespread applications in quantum technologies, and various shortcuts to adiabaticity protocols have been demonstrated in closed systems. However, realizing shortcuts to adiabaticity for open quantum systems has presented a challenge due to the complex controls in existing proposals. Here, we present the experimental demonstration of shortcuts to adiabaticity for open quantum systems, using a superconducting circuit quantum electrodynamics system. By applying a counterdiabatic driving pulse, we reduce the adiabatic evolution time of a single lossy mode from 800 ns to 100 ns. In addition, we propose and implement an optimal control protocol to achieve fast and qubit-unconditional equilibrium of multiple lossy modes. Our results pave the way for precise time-domain control of open quantum systems and have potential applications in designing fast open-system protocols of physical and interdisciplinary interest, such as accelerating bioengineering and chemical reaction dynamics.
The difficulty in combining high fidelity with fast operation times and robustness against sources of noise is the central challenge of most quantum control problems, with immediate implications for the realization of quantum devices. We theoretically propose a protocol, based on the widespread stimulated Raman adiabatic passage technique, which achieves these objectives for quantum state transfers in generic three-level systems. Our protocol realizes accelerated adiabatic following through the application of additional control fields on the optical excitations. These act along frequency sidebands of the principal adiabatic pulses, dynamically counteracting undesired transitions. The scheme facilitates experimental control, not requiring new hardly-accessible resources. We show numerically that the method is efficient in a very wide set of control parameters, bringing the timescales closer to the quantum speed limit, also in the presence of environmental disturbance. These results hold for complete population transfers and for many applications, e.g., for realizing quantum gates, both for optical and microwave implementations. Furthermore, extensions to adiabatic passage problems in more-level systems are straightforward.
In circuit quantum electrodynamics the coherence of Cooper pairs in superconductors is employed to create macroscopic electric circuits with quantized energy levels. Such circuits can be coupled with each other and exploited as building blocks of a quantum computer. Accurate and robust control of the quantum state in the circuits is a central condition for the operation of the quantum computer and one of the prerequisites for the implementation of complex algorithms used in quantum information processing, such as quantum error correction. In this thesis adiabatic control in circuit quantum electrodynamics is investigated with the focus on manipulating three-level systems. \n \nIn adiabatic control the eigenstates of the system are slowly modified by changing the external control parameters, which govern the evolution of the system. If the changes in the parameters are slow enough, the state of the system follows the eigenstates in the adiabatic basis, thereby realizing the intended operation. The advantage of adiabatic control is its inherent robustness to small errors or noise in the control parameters; the result of the state manipulation only depends on the asymptotic values of the control parameters, but not on their exact values during the process. \n \nShortcuts to adiabaticity can be used to speed up the otherwise slow adiabatic control by introducing a correction pulse that compensates the diabatic losses during the state manipulation. This allows one to overcome the limitation on the speed of the protocol but simultaneously reduces the method's robustness to the variations in the control parameters. If the level of noise in the control parameters is known, using the shortcut it is possible to find the optimal level of robustness which is required to mitigate the noise. \n \nCircuit quantum electrodynamics offers a perfect experimental platform for investigating quantum control due to the possibility of realizing complicated control schemes using microwave electronics. With commercially available digital-to-analog converters the control signals can be digitally created, which enables accurate and coherent control of the quantum circuit. \n \nIn this thesis both theoretical and experimental results on adiabatic control applied to superconducting transmon circuits are presented. It is shown that stimulated Raman adiabatic passage can be used for population transfer in a three-level transmon, which can be further improved using shortcuts to adiabaticity. Furthermore, a scheme for implementing robust superadiabatic rotation gates in transmon is proposed. Finally, it is demonstrated that superconducting qubit can be used as an ultra-sensitive detector of magnetic flux.
By definition, quantum adiabatic process means a slow process which allows the state to follow the instantaneous eigenstates of time-dependent Hamiltonian. For some reasons, for example, to avoid the decoherence effects, or to implement large-scale quantum information processing, we may want to speed up the adiabatic process, that is, to achieve the adiabatic-like control but in very short time. In this talk, we present new methods to speeded-up expansion and transport of cold atoms in a harmonic trap. Such shortcuts to adiabaticity provide the fast expansion or transport, in which the final atomic state is the same as in the adiabatic process, but in arbitrarily short time, keeping the same populations of vibrational levels in the initial and final trap. These methods can also be generalized to Bose-Einstein Condensates. Moreover, we present shortcuts to adiabatic passage from one internal atomic state to another in twoor three-level atoms. In detail, we can apply Berry’s transitionless quantum driving method and invariant-based inverse engineering method to accelerate the Rapid Adiabatic Passage (RAP) and Stimulated Raman Adiabatic Passage (STIRAP) in twoand three-level atomic systems, respectively. We also examine and compare the stability of different schemes concerning different types of noise and system errors. Finally, we show that the technique of shortcuts to adiabaticity in two-level system can be applied in fast and robust spin flip in a quantum dot, to avoid the decoherent effects.
Adiabatic quantum operations are ubiquitous in fields such as quantum information processing, quantum control, and magnetic resonance, where their high fidelity and general robustness renders them an essential tool for various applications. This inherent robustness due to adiabaticity can, however, be impaired in cases where the experimental conditions strictly require very fast evolution times. In this thesis, we provide a gradient-based numerical optimization protocol for efficiently engineering adiabatic operations, allowing for the systematic inclusion of robustness criteria against various experimental non-idealities, including inhomogeneities and uncertainties in system parameters, as well as perturbations in the Hamiltonian such as spin-spin interactions. \nThe protocol is implemented in the context of adiabatic passages for magnetic resonance, and \nit is shown that in addition to conventional adiabatic pulses, it can also generate exceptionally fast operations that although slightly deviate from adiabaticity in limited instances, still lead to a high fidelity. \nThe effectiveness of our method for addressing perturbations is also demonstrated by designing a fast adiabatic passage for dipolar-coupled electrons, and numerically comparing its performance with a pulse without such considerations.
Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.