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APS

The 4 ^3Σ^+ State of NaK: Potential Energy Curve and Hyperfine Structure

Angela D. Wilkins, P. Burns, L. Sibbach-Morgus, A. P. Hickman, John Huennekens, Li Li

Published May 1, 2003• 0 citations
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We establish a theoretical model to analyze the photoassociative spectroscopy of 85Rb 133Cs molecules in the (3)3Σ+ state. The vibrational energy, spin-spin coupling constant, and hyperfine interaction constant of the (3)3Σ+ state are determined based on nine observed vibrational levels. Consequently, the Rydberg-Klein-Rees potential energy curve of the (3)3Σ+ state is obtained and compared with the ab initial potential energy curve. Our model can be adopted to analyze the photoassociative spectroscopy of other heteronuclear alkali-metal diatomic molecules in the (3)3Σ+ state.