Spatial modes have attracted a lot of attention in the quantum optics community because of their possible application in high-dimensional quantum bits, i.e. qudits. One crucial task in quantum communication and computation applications, is the ability to perform unitary transformations on these qudits. However, arbitrary unitary transformations between full-field spatial modes have not been realized so far. Thus, in order to bring spatial modes closer to communication and computation applications, methods for performing these transformations need to be devised. \n \nIn this thesis, we introduce a method for generating these unitary transformations. The method is based on multi-plane light conversion (MPLC), where the spatial structure of light is transformed through multiple consecutive transverse-phase modulations. The method we use for generating these task specific phase-modulations is called wavefront matching (WFM). \n \nThis thesis consists of three main sections. First, we will introduce some necessary theory behind high-dimensional quantum-states and single photons. We will also explore some theory behind the generation of single photons and introduce light's spatial modes in more detail. Second, we will introduce WFM along with other methods we needed for testing the unitary transformations experimentally. Finally, we will experimentally test the mode transformations in a spatial mode filter and in multi-mode transformations. We apply the mode filter in quantum key distribution (QKD) and quantum state tomography (QST) measurements, and we implement different high-dimensional quantum gates using the multi-mode transformations. Additionally, we introduce a method of potentially observing two-photon interference with these unitary transformations. \n \nWith the mode filter, we achieved error rates below five percent and in the QKD application we measured a theoretical data transmission rate of 1.98 bits per measured photon. With the quantum gates, we achieved accuracies of up to 98\\% in all mutually unbiased bases (MUBs). The results shown in this thesis demonstrate the efficiency and unitarity of WFM in a broad set of different tasks. All the shown tasks are important in high-dimensional quantum communication and computation, and hence we believe that WFM will become an important tool in high-dimensional quantum information processing. We also give an outlook on how WFM could potentially be improved, and list some additional tasks, in which WFM could be useful. We believe that the broad applicability of WFM will enable some unexplored quantum information or photonics applications.
Spatial modes have attracted a lot of attention in the quantum optics community because of their possible application in high-dimensional quantum bits, i.e. qudits. One crucial task in quantum communication and computation applications, is the ability to perform unitary transformations on these qudits. However, arbitrary unitary transformations between full-field spatial modes have not been realized so far. Thus, in order to bring spatial modes closer to communication and computation applications, methods for performing these transformations need to be devised. \n \nIn this thesis, we introduce a method for generating these unitary transformations. The method is based on multi-plane light conversion (MPLC), where the spatial structure of light is transformed through multiple consecutive transverse-phase modulations. The method we use for generating these task specific phase-modulations is called wavefront matching (WFM). \n \nThis thesis consists of three main sections. First, we will introduce some necessary theory behind high-dimensional quantum-states and single photons. We will also explore some theory behind the generation of single photons and introduce light's spatial modes in more detail. Second, we will introduce WFM along with other methods we needed for testing the unitary transformations experimentally. Finally, we will experimentally test the mode transformations in a spatial mode filter and in multi-mode transformations. We apply the mode filter in quantum key distribution (QKD) and quantum state tomography (QST) measurements, and we implement different high-dimensional quantum gates using the multi-mode transformations. Additionally, we introduce a method of potentially observing two-photon interference with these unitary transformations. \n \nWith the mode filter, we achieved error rates below five percent and in the QKD application we measured a theoretical data transmission rate of 1.98 bits per measured photon. With the quantum gates, we achieved accuracies of up to 98\% in all mutually unbiased bases (MUBs). The results shown in this thesis demonstrate the efficiency and unitarity of WFM in a broad set of different tasks. All the shown tasks are important in high-dimensional quantum communication and computation, and hence we believe that WFM will become an important tool in high-dimensional quantum information processing. We also give an outlook on how WFM could potentially be improved, and list some additional tasks, in which WFM could be useful. We believe that the broad applicability of WFM will enable some unexplored quantum information or photonics applications.
Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing, allowing the complete manipulation of quantum systems in a coherent manner. In the case of photons, optical elements that can perform unitary transformations are readily available only for some degrees of freedom, e.g., wave plates for polarization. However, for high-dimensional states encoded in the transverse spatial modes of light, performing arbitrary unitary transformations remains a challenging task for both theoretical proposals and actual implementations. Following the idea of multi-plane light conversion, we show that it is possible to perform a broad variety of unitary operations at high quality by using only a few phase modulation planes. More importantly, we experimentally implement several high-dimensional quantum gates for up to five-dimensional states encoded in the full-field mode structure of photons. In particular, we realize cyclic and quantum Fourier transformations, known as Pauli X ^ -gates and Hadamard H ^ -gates, respectively, with an average visibility of more than 90%. In addition, we demonstrate near-perfect “unitarity” by means of quantum process tomography, unveiling a process purity of 99%. Last, we demonstrate the benefit of the two independent spatial degrees of freedom, i.e., azimuthal and radial, and implement a two-qubit controlled-NOT quantum operation on a single photon. Thus, our demonstrations open up new paths to implement high-dimensional quantum operations, which can be applied to various tasks in quantum communication, computation, and sensing schemes.
Structure photons invoke interesting fundamental properties and enable novel applications, e.g. their use as high-dimensional quantum states, which are known to be beneficial in various quantum information tasks. However, to use their full potential the ability to perform any unitary operations is indispensable. Here, we present a scheme to perform arbitrary unitary operation for all transverse spatial modes, i.e. a so-called multiport for high-dimensional quantum states. We realize it by using multiple consecutive phase modulations, which are designed by wave front matching techniques. At first, we perform near-perfect measurements of full-field modes, i.e. modes with an azimuthal and radial structure [1]. Our method only requires three consecutive phase modulations followed by a single mode fiber and is, in principle, error-free and lossless. We achieve an average error of 4.2% for a set of 9 different full-field Laguerre-Gauss and Hermite-Gauss modes with an efficiency of up to 70%. We further demon-strate its potential in a quantum cryptography protocol and in high-dimensional quantum state tomography. We then use the multiport to implement high-dimensional quantum gates [2], such as cyclic and quantum Fourier transformations, known as Pauli X-gates and Hadamard H-gates, respectively. We achieve an aver-age visibility of more than 90% for dimensions up to 5 and obtain a process purity of 99% by means of a full quantum process tomography. We also demonstrate the benefit of the two independent spatial degrees of freedom, i.e. azimuthal and radial, and implement a two-qubit controlled-NOT quantum operation on a single photon. Using more efficient phase modulations will pave the way to novel multi-particle high-dimensional quantum information experiments. [1] M. Hiekkamäki, S. Prabhakar, R. Fickler, Near-perfect measuring of full-field transverse-spatial modes of light, arXiv:1909.01685 [2] F. Brandt, M. Hiekkamäki, F. Bouchard, M. Huber, R. Fickler, High-dimensional quantum gates using full-field spatial modes of photons, arXiv:1907.13002
This thesis explores the development and application of multi-plane light conversion (MPLC) technol-ogy, focusing on its integration into experimental setups that push the boundaries of quantum opticsand spatial state tomography. Central to this study is a custom-built, research-grade MPLC devicedesigned around a programmable spatial light modulator (SLM), which facilitates two groundbreak-ing experiments: the manipulation of high-dimensional qudits for quantum gate operations, and thedevelopment of a high-dimensional Stokes-space spatial beam analyser for single-shot spatial statetomography.The first experiment involved implementing quantum gates — specifically the X-gate, Z-gate, andDFT-gate — for a 17-dimensional qudit, represented through the first 17 azimuthal Laguerre-Gaussianspatial modes on a MPLC device. This experiment not only demonstrated MPLC’s capability tohandle complex, high-dimensional quantum states but also underscored its potential to enhance thescalability and efficiency of quantum computing architectures. By leveraging the precise control overspatial modes afforded by MPLC and the programmability of SLM-based MPLC, the experimentdemonstrated high-dimensional gate operations, paving the way for more complex quantum computingoperations for qudits.The second project focused on using MPLC to develop a device capable of performing high-dimensional Stokes-space spatial beam analysis. This innovative instrument marks a significantbreakthrough in optical beam characterisation, providing a reference-free, single-shot technique forconducting spatial state tomography on beams characterisable by a six-mode or six-dimensional system.The device’s capacity to swiftly and precisely characterise the wavefront and coherence of opticalfields renders it an invaluable asset for advancing optical communication technologies and enhancingoptical sensing methodologies.Throughout this thesis, the theoretical foundations of MPLC technology are presented, with adetailed account of the MPLC device design and operational principles. Experimental results arepresented to validate the effectiveness of the MPLC device in both quantum gate operations andspatial state tomography. Comparisons with existing technologies highlight the MPLC’s enhancedperformance and versatility.This work not only expands the understanding and application of MPLC in quantum and opticalsciences but also sets the stage for future innovations in these fields. The continuous refinement andadaptation of MPLC technology promise to unlock new possibilities in both fundamental research andpractical applications.
Along with the growing interest in using the transverse-spatial modes of light in quantum and classical optics applications, developing an accurate and efficient measurement method has gained importance. Here, we present a technique relying on a unitary mode conversion for measuring any full-field transverse-spatial mode. Our method only requires three consecutive phase modulations followed by a single mode fiber and is, in principle, error-free and lossless. We experimentally test the technique using a single spatial light modulator and achieve an average error of 4.2 % for a set of 9 different full-field Laguerre-Gauss and Hermite-Gauss modes with an efficiency of up to 70%. Moreover, as the method can also be used to measure any complex superposition state, we demonstrate its potential for quantum cryptography applications and in high-dimensional quantum state tomography.
Photons can carry quantum information not only in two-level systems (qubits) but also in d-level systems known as qudits. A single photon distributed across d optical modes can encode up to log2(d) qubits of information, allowing for more efficient use of quantum resources and increased resilience to noise. This advantage, however, comes at a price: implementing quantum gates and performing measurements in high-dimensional Hilbert spaces is significantly more demanding than in the qubit case. To tackle these challenges, I will present our recent work developing new protocols and optical hardware that enable quantum communication and computation with high-dimensional qudits encoded in the temporal or spatial modes of single and entangled photons. I will discuss our experimental implementations of quantum key distribution using weak coherent pulses [Sulimany et al., NPJ Quantum Information 11, 16 (2025)], single photons from quantum dots [Halevi et al., Optica Quantum 2, 351 (2024)], and entangled photon pairs [Lib et al., Optica Quantum 3, 182 (2025)]. In the latter, we demonstrated projective measurements in two mutually unbiased bases for d=25 using a multi-plane light converter (MPLC). I will also show how the same MPLC platform can be used to perform elementary operations in measurement-based quantum computation with high-dimensional cluster states [Lib and Bromberg, Nat. Photonics 18, 1218 (2024)]. Throughout the talk, I will discuss the tradeoffs between qubit- and qudit-based approaches and highlight the regimes where high-dimensional systems offer a practical advantage.
High-dimensional quantum key distribution (QKD) offers higher information capacity and stronger resilience to noise compared with its binary counterpart. However, these advantages are often hindered by the difficulty of realizing the required high-dimensional measurements and transformations. Here, we implement a large-scale multi-plane light converter (MPLC) and program it as a high-dimensional mode sorter of spatial modes for QKD. Using the MPLC, we demonstrate five-dimensional QKD with six mutually unbiased bases and 25-dimensional QKD with two mutually unbiased bases in the same experimental setup. Furthermore, we propose a construction of pairs of mutually unbiased bases that are robust to experimental errors, with measurement complexity scaling only with the square root of the encoded dimension. This approach paves the way for QKD implementations in higher dimensions.