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OptSp

Dispersion of light-induced anisotropy of dye solutions under conditions of inhomogeneous broadening of the resonance transition

Leonid I. Burov, Ганчеренок Игорь Иванович

Published Feb 1, 1988• 0 citations
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Physical Review A•Apr 1, 1993•9 citations
A novel transient three-pulse scattering technique for measuring ultrafast dephasing times in condensed matter is analyzed using a perturbative solution of the density matrix equation. The advantages of this technique include subpulsewidth resolution, a clear distinction between homogeneous and inhomogeneous broadening, and sensitivity to spectral cross-relaxation. Its application to the case of a multilevel resonance is also considered. We report results of femtosecond dephasing experiments with dye molecules in liquids and in a polymer host. The dephasing time is determined to be less than 20 fsec for dyes in solution at room temperature. At low temperatures in polymers, a transition from homogeneous to inhomogeneous broadening has been observed and studied as a function of temperature.
The self-induced transparency in the Kerr host medium has been studied beyond the slowly-varying-envelope approximation. An analytic solution is obtained. There exists a hyperbolic-secant soliton whose power, pulse width, group velocity, and propagation constant are uniquely determined for given parameters of the medium. The reductions of the group velocities of the solitons by the self-induced-transparency effect in the resonant medium with homogeneous and inhomogeneous broadening are also studied. It is found that there is negative dispersion induced by the self-induced transparency, which is not predicted by the theory with the slowly-varying-envelope approximation. The amount of the induced dispersion is determined by the total dispersion of the system required to be compensated by the Kerr effect. Numerical examples of the self-induced transparency in an erbium-doped fiber are shown. In a typical erbium-doped fiber, the soliton solution has not been found because the inhomogeneous-broadening linewidth of the medium is too large.