Radiative Transitions

В. П. Крайнов, Howard R. Reiss, Борис М. Смирнов

Radiative transition of atomic electrons radiative transitions between discrete states in atomic systems atomic photoprocesses involving free particles coherent phenomena in radiative transitions atoms in strong fields.

Richard C. Powell

Richard J. Cook

. Each transition dipole in a single atom has a radiation reaction field which acts on itself and on the other transition dipoles of the atom. The self interaction on a given transition gives rise to spontaneous emission and radiative decay on that transition. Here we emphasize that the mutual radiative interaction of different transition dipoles can sometimes have important consequences. The mutual radiative interaction can substantially alter radiative decay rates and inhibit the radiative decay of certain expectation values. The hydrogen atom and the harmonic oscillator are cited as examples and a possible experimental test of mutual radiation reaction involving a single electron in a Penning trap is discussed. Introduction Modern quantum mechanics began with Heisenberg's picture of a bound charge as a “virtual orchestra” of transition dipoles oscillating at different frequencies. It is known from modern quantum theory that each of these dipoles generates a radiation reaction field which, acting on the dipole itself, gives rise to spontaneous emission and radiative relaxation (Milonni, 1976). In this paper we consider the mutual interaction of different transition dipoles within a single “atom”. We begin by considering some simple cases of mutual radiation reaction in classical electrodynamics and proceed to the quantum theory of mutual radiation reaction (MRR), citing the hydrogen atom and the charged harmonic oscillator as examples. We point out that the equations describing MRR are not at all new, but can be traced to the earliest treatments of the interaction of atoms with the quantized electromagnetic field.

B. K. Ridley FRS

Clemens Spinnler, Liang Zhai, Giang N. Nguyen +8 more

In a radiative Auger process, optical decay leaves other carriers in excited states, resulting in weak red-shifted satellite peaks in the emission spectrum. The appearance of radiative Auger in the emission directly leads to the question if the process can be inverted: simultaneous photon absorption and electronic demotion. However, excitation of the radiative Auger transition has not been shown, neither on atoms nor on solid-state quantum emitters. Here, we demonstrate the optical driving of the radiative Auger transition, linking few-body Coulomb interactions and quantum optics. We perform our experiments on a trion in a semiconductor quantum dot, where the radiative Auger and the fundamental transition form a Λ-system. On driving both transitions simultaneously, we observe a reduction of the fluorescence signal by up to 70%. Our results suggest the possibility of turning resonance fluorescence on and off using radiative Auger as well as THz spectroscopy with optics close to the visible regime.