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Журнал Экспериментальной и Теоретической Физики

Quasi-resonant Stark broadening of the optical spectra of quantum systems in a noisy Gaussian field

N. F. Perel'Man, Ilya Sh. Averbukh, Viktor A Kovarskii

Published Aug 1, 1987• 0 citations
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As an application of the nonlocal theory of radiation matter interaction, pump-probe spectra for ultrathin (<500 Å) platelets of CuCl have been calculated for the pumping condition between exciton and biexciton levels. Typical aspects such as (1) pump induced absorption to biexciton states, and (2) optical Stark shift and resonant broadening of size quantized exciton levels can be seen in the calculated response spectra. The spatial variation of the light field inside the samples depends sensitively on the frequency and slab thickness, which is clearly reflected in the response spectra as quasi k -selection rule. For thicker samples the k -selection rule becomes more strictly valid, as expected.
The review systematizes the experimental material and reports the fundamental theoretical results on the study of nonlinear resonance effects in spectra of atomic systems situated in the radiation field of lasers. The theoretical part explains the topics of greatest importance and significance for understanding of the experimental studies: the Stark effect in an optical field; the nonequilibrium velocity distribution of the atoms; the shape of the spectral line for a transition adjacent to a transition combining with a strong field; the simultaneous manifestation of the Stark effect and of Doppler broadening in the form of a very sharp structure on the line contour; a brief mention of the influence of collisions, recoil, and other factors on the sharp structure in spectra. The experimental part reports the results of experiments on the observation of the Stark effect in the optical region of the spectrum, the fine structure of the profile of a Doppler-broadened line and its properties, namely the dependence on the observation direction, the anisotropy in the field of a standing wave, the polarization properties, etc. in spectra of spontaneous or stimulated emission, absorption, and generation.