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Optica Acta International Journal of Optics

Quantum Statistics of Light after Two-photon Absorption and Emission Processes

Published Nov 1, 1980• 15 citations
Publisher
DOI
10.1080/713820173

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Two-photon absorption and emission for a collection of two level atoms from a single mode beam of light are considered and the statistical proper- ties of the field after the interaction are investigated without placing any restriction of the population of the atomic levels . The dynamical behaviour of the field is described by assuming the atomic levels maintained with a nearly fixed popula- tion distribution . By applying iteration methods the time development for the density operator of the field is written and an expression for the coherent component is obtained . This component appears to be present only when there is a coherent component in the field before the interaction . The statistical properties of the field after the interaction, when the mean photon number is large initially, are then discussed and explicit calculations are carried out for some special cases of initial fields . Finally, it is shown that two-photon spontaneous emission field can be expressed as a superposition of chaotic fields .

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The well-known photon correlations of thermal light are now understood to result from the random superposition of independently emitted photons from spontaneous emission. Through random interference the number of photons evolves as a Bose-Einstein distribution rather than the Poisson distribution as one might expect for independent emissions of classical particles. By identifying terms in the density-matrix (\ensuremath{\rho}) equation for a linear amplifier, those terms giving rise to spontaneous emission were earlier distinguished from those causing amplification and absorption. We investigate the role of interference in the evolution of the photon statistics by further identifying terms in the equation for \ensuremath{\rho}${\ifmmode \dot{}\else \.{}\fi{}}_{n}$ solely responsible for quantum interference phenomena. The effects of this random interference on the photon factorial moments are quantified, even for those cases where the final field statistics are not Bose-Einstein. From our analysis we conclude that stimulated emission should be viewed as analogous to time-reversed absorption, rather than either a cascade process or pure constructive interference.

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Exact solutions of the master equations which describe single-mode mmm-photon absorption and mmm-photon emission processes in a two-level atomic system are obtained using a density-matrix approach. Some aspects of the photon statistics, e.g., antibunching, are discussed.
Two-photon absorption and emission for a collection of two level atoms from a single mode beam of light are considered and the statistical proper- ties of the field after the interaction are investigated without placing any restriction of the population of the atomic levels . The dynamical behaviour of the field is described by assuming the atomic levels maintained with a nearly fixed popula- tion distribution . By applying iteration methods the time development for the density operator of the field is written and an expression for the coherent component is obtained . This component appears to be present only when there is a coherent component in the field before the interaction . The statistical properties of the field after the interaction, when the mean photon number is large initially, are then discussed and explicit calculations are carried out for some special cases of initial fields . Finally, it is shown that two-photon spontaneous emission field can be expressed as a superposition of chaotic fields .
The well-known photon correlations of thermal light are now understood to result from the random superposition of independently emitted photons from spontaneous emission. Through random interference the number of photons evolves as a Bose-Einstein distribution rather than the Poisson distribution as one might expect for independent emissions of classical particles. By identifying terms in the density-matrix (\ensuremath{\rho}) equation for a linear amplifier, those terms giving rise to spontaneous emission were earlier distinguished from those causing amplification and absorption. We investigate the role of interference in the evolution of the photon statistics by further identifying terms in the equation for \ensuremath{\rho}${\ifmmode \dot{}\else \.{}\fi{}}_{n}$ solely responsible for quantum interference phenomena. The effects of this random interference on the photon factorial moments are quantified, even for those cases where the final field statistics are not Bose-Einstein. From our analysis we conclude that stimulated emission should be viewed as analogous to time-reversed absorption, rather than either a cascade process or pure constructive interference.