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Applied Optics

Nonlinear Optics of Free Atoms and Molecules. By D. C. Hanna, M. A. Yuratich, and D. Cotter

Lorenzo M. Narducci

Published Mar 1, 1981• 0 citations
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Some quantum effects in nonlinear optics

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Introduction We have already encountered situations in which light of one frequency falling on an atomic system gives rise to light of different frequencies (cf. Section 15.6). The atom may here be considered to play the role of a (noisy) nonlinear transducer for the incident field. Even stronger nonlinear effects arise when one is dealing with a large number of atoms, or a nonlinear medium . Under these circumstances it is sometimes permissible to ignore the atomic structure and to treat the medium as a continuum, as in Maxwell's electromagnetic theory. The subject of the interaction of the incident field with the nonlinear medium is usually known as nonlinear optics. The subject had its beginnings in an experiment in which a strong beam of red light (wavelength 6943 Å) from a ruby laser was allowed to fall on a quartz crystal, and a faint beam of blue light at a wavelength of 3472 Å, the first harmonic of the red, was produced (Franken, Hill, Peters and Weinreich, 1961). The development of the subject of nonlinear optics into a mature field is due largely to the work of Bloembergen and his collaborators. In the following we shall consider only a few simple illustrative examples of phenomena in nonlinear optics. More topics and more detail can be found in the books by Bloembergen and others (Bloembergen, 1965; Yariv, 1967, Chap. 21; Shen, 1984; Schubert and Wilhelmi, 1986; Butcher and Cotter, 1990; Boyd, 1992).

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Introduction We have already encountered situations in which light of one frequency falling on an atomic system gives rise to light of different frequencies (cf. Section 15.6). The atom may here be considered to play the role of a (noisy) nonlinear transducer for the incident field. Even stronger nonlinear effects arise when one is dealing with a large number of atoms, or a nonlinear medium . Under these circumstances it is sometimes permissible to ignore the atomic structure and to treat the medium as a continuum, as in Maxwell's electromagnetic theory. The subject of the interaction of the incident field with the nonlinear medium is usually known as nonlinear optics. The subject had its beginnings in an experiment in which a strong beam of red light (wavelength 6943 Å) from a ruby laser was allowed to fall on a quartz crystal, and a faint beam of blue light at a wavelength of 3472 Å, the first harmonic of the red, was produced (Franken, Hill, Peters and Weinreich, 1961). The development of the subject of nonlinear optics into a mature field is due largely to the work of Bloembergen and his collaborators. In the following we shall consider only a few simple illustrative examples of phenomena in nonlinear optics. More topics and more detail can be found in the books by Bloembergen and others (Bloembergen, 1965; Yariv, 1967, Chap. 21; Shen, 1984; Schubert and Wilhelmi, 1986; Butcher and Cotter, 1990; Boyd, 1992).