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Annual Meeting Optical Society of America

Instabilities of counterpropagating waves in a two-level medium

Israel Bar-Joseph, Yaron R. Silberberg

Published Jan 1, 1986• 0 citations
Publisher

Abstract

We have previously shown that counterpropagating waves in a Kerrlike medium exhibit spontaneous oscillations above a certain threshold intensity. The period of these oscillations was related to the medium length and to its response time. These oscillations were explained as results of parametric gain and feedback supplied by the grating formed through the nonlinear interaction. In this paper we extend the theory to a two-level medium. The complexity of the parametric interaction in this medium provides a reach spectrum of behaviors. The power exchange due to this interaction, between waves of different frequencies, is usually maximized when the frequency difference is the Rabi frequency. However, another maximum, which is smaller in magnitude, occurs in certain limits when the frequency difference is T1. Our derivation is based on performing a linear stability analysis to the steady-state solutions of the Maxwell-Bloch equations. We assumed a small signal absorption and large detuning from resonance. The solutions were studied in the limit of pure radiative broadening (T2 = T1) and rapid collisional dephasing (T2 ≪ T1). It is found that for most cases Rabi frequency self-oscillations are dominant. However, for T2 ≪ T1 and for large interaction length, we found slower oscillations, with a period of T1. We show that the results can be understood by the gain feedback model. We also discuss the effect of inhomogeneous broadening and present experimental parameters required for observation of T1 oscillations.

DOI
10.1364/oam.1986.mf3

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Annual Meeting Optical Society of America•Jan 1, 1989•0 citations
We have previously shown that counterpropagating waves in a Kerrlike medium exhibit spontaneous oscillations above a certain threshold intensity. The period of these oscillations was related to the medium length and to its response time. These oscillations were explained as results of parametric gain and feedback supplied by the grating formed through the nonlinear interaction. In this paper we extend the theory to a two-level medium. The complexity of the parametric interaction in this medium provides a reach spectrum of behaviors. The power exchange due to this interaction, between waves of different frequencies, is usually maximized when the frequency difference is the Rabi frequency. However, another maximum, which is smaller in magnitude, occurs in certain limits when the frequency difference is T1. Our derivation is based on performing a linear stability analysis to the steady-state solutions of the Maxwell-Bloch equations. We assumed a small signal absorption and large detuning from resonance. The solutions were studied in the limit of pure radiative broadening (T2 = T1) and rapid collisional dephasing (T2 ≪ T1). It is found that for most cases Rabi frequency self-oscillations are dominant. However, for T2 ≪ T1 and for large interaction length, we found slower oscillations, with a period of T1. We show that the results can be understood by the gain feedback model. We also discuss the effect of inhomogeneous broadening and present experimental parameters required for observation of T1 oscillations.
The dynamical behavior of counterpropagating light waves interacting with a nonlinear medium is studied numerically. It is found that the wave and the medium form a system that becomes unstable under certain conditions and exhibits self-oscillation. Because the interacting medium is modeled by an ensemble of two-level systems, we recognize the self-oscillation frequency as the Rabi-frequency of the constituent systems. The physical mechanisms responsible for this self-oscillation are the gain and the distributed feedback of the combined lightwave-medium system. When the environment changes, in particular when the intensity is increased, this system becomes more unstable and we find that the oscillation exhibits more complex behavior, including quasi-periodic motion and chaos. We analyze the output fields by using Fourier spectra, phase portraits, and autocorrelation functions. In the chaotic regime, the Lyapunov exponents and dimensions are also calculated. A physical interpretation of the quasiperiodic motion is given by an exact calculation of the absorption spectrum of our two-level medium. The negative absorption (gain) peaks are found at the frequencies of the quasi-periodic motions, thus implying that the gain of the combined light-medium system is responsible at least in part for the observed complex behavior. In addition, we investigate the stability of the propagating plane wave when a transverse wave is added to the system as a perturbation. Instabilities are analyzed by linearizing the nonlinear equations which model the lightwave-medium system. The results show that the instability is highly-correlated with the four-wave mixing phase conjugation.
Two counterpropagating waves in a Kerr medium were shown to exhibit instabilities, which lead to self-oscillations, bifurcations, and chaos.1 These instabilities, as well as self-oscillation phenomena in bistable systems, can be explained by a gain-feedback mechanism.2 Fields at frequencies adjacent to the input pump-wave frequency can be amplified through four-wave-mixing interactions. If feedback is supplied, sidebands at these frequencies can be excited and beat with the pump wave to yield an oscillating output. In a counterpropagating-beam configuration, the feedback is distributed, and it originates from the grating that is formed by the interfering beams.
The threshold characteristics of the static and periodic instability of the single feedback mirror device are investigated for a homogeneously broadened two-level medium as a function of the input intensity, the detuning, the buffer-gas pressure, the atomic concentration, and the round-trip time d, and compared with experimental results. For a large range of parameters that agrees with the experiment, the self-oscillation process is shown to be mainly induced by the longitudinal grating, which ensures a large instability domain, and controlled by the buffer-gas pressure, which must be low enough in order that the threshold period of the oscillation is constant on a doughnutlike transverse profile and nearly equal to 2d. This oscillation, called the 2d oscillation, is neither a result of pure phase-conjugate-mirror operation of the atomic medium nor a result of a Rabi sideband gain process. It is shown to take place through a mixture of phase-conjugate-mirror and ordinary mirror operations, which are both allowed by the specific optical arrangement of the device.
We investigated the sideband instability by numerical integration of the Maxwell-Bloch equations for propagation of a nearly resonant pump laser and a weak probe laser in a system of two-level atoms. In an optically thick medium, the probe gain (absorption) spectrum becomes a function of propagation distance. We find that the well-known gain resonance at the generalized Rabi frequency Ω' is suppressed and a broad asymmetric gain region forms on each side of the laser frequency. For probe-pump detunings inside these gain regions, the field envelope breaks up into periodic traveling waves that are compared to the polycnoidal solutions of the sine-Gordon equation with periodic boundary conditions.
We have shown previously that two strong laser beams (with the same frequency) counterpropagating in a Kerr nonlinear medium with linear dispersion become un stable when their intensities exceed a certain threshold.1 We demonstrate here that the system exhibits large (theoretically unlimited) amplification of a probe beam when the two pumping beams have their intensities slightly below the threshold. This is in contrast to the conventional phase conjugation due to four-wave mixing in a nondispersive Kerr nonlinear medium. The mechanism of amplification in our system can be explained in terms of positive distributed feedback from the Kerr nonlinear index grating formed by two strong pumping laser beams in the presence of dispersion giving rise to a light-induced distributed-feedback resonator. This feedback is attributed to the fact that the weak beams with both signal frequency, ω + δ, and conjugate frequency, ω − δ, propagate with phase speed different (due to dispersion) from that of a pumping wave with frequency ω, which triggers the exponentially increasing energy exchange between weak and strong beams at the nonlinear index grating (this energy exchange is prohibited in nondispersive media). When the probe frequency approaches a frequency of one of the longitudinal modes of the light-induced distributed resonator, and the pumping intensity approaches the threshold of instability, the resonant amplification increases infinitely; for presently available laser intensity stabilities, amplification as large as 104 is feasible.