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Chinese Physics Letters

High-Fidelity Manipulation of the Quantized Motion of a Single Atom via Stern–Gerlach Splitting*

Kunpeng Wang, Jun Zhuang, Xiaodong He, Ruijun Guo, Cheng Sheng, Peng Xu, Min Liu, Jin Wang, Mingsheng Zhan

Published Mar 1, 2020• 12 citations
Publisher

Abstract

We demonstrate high-fidelity manipulation of the quantized motion of a single 87 Rb atom in an optical tweezer via microwave couplings induced by Stern–Gerlach splitting. The Stern–Gerlach splitting is mediated by polarization gradient of a strongly focused tweezer beam that functions as fictitious magnetic field gradient. The spatial splitting removes the orthogonality of the atomic spatial wavefunctions, thus enables the microwave couplings between the motional states. We obtain coherent Rabi oscillations for up to third-order sideband transitions, in which a high fidelity of larger than 0.99 is obtained for the spin-flip transition on the first order sideband after subtraction of the state preparation and detection error. The Stern–Gerlach splitting is measured at a precision of better than 0.05 nm. This work paves the way for quantum engineering of motional states of single atoms, and may have wide applications in few body physics and ultracold chemistry.

DOI
10.1088/0256-307x/37/4/044209

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Quantum fine structure of the optical Stern-Gerlach effect

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In the optical Stern-Gerlach effect the interaction of a two-level atom with an optical-field gradient causes a state-selective deflection that leads to a splitting of the atomic trajectory. The semiclassical approach to this problem actually predicts a splitting of the atomic beam into two paths, similar to the well-known magnetic Stern-Gerlach effect for spin 1/2. Here we study a model in which the quantum nature of the field is taken into account and we show, in particular, that for an initial coherent state of the cavity light the optical Stern-Gerlach effect manifests itself as a splitting of the atomic beam into two groups containing, however, many spots. \textcopyright{} 1996 The American Physical Society.

Physical Review A•Oct 1, 1996•12 citations
We demonstrate high-fidelity manipulation of the quantized motion of a single 87 Rb atom in an optical tweezer via microwave couplings induced by Stern–Gerlach splitting. The Stern–Gerlach splitting is mediated by polarization gradient of a strongly focused tweezer beam that functions as fictitious magnetic field gradient. The spatial splitting removes the orthogonality of the atomic spatial wavefunctions, thus enables the microwave couplings between the motional states. We obtain coherent Rabi oscillations for up to third-order sideband transitions, in which a high fidelity of larger than 0.99 is obtained for the spin-flip transition on the first order sideband after subtraction of the state preparation and detection error. The Stern–Gerlach splitting is measured at a precision of better than 0.05 nm. This work paves the way for quantum engineering of motional states of single atoms, and may have wide applications in few body physics and ultracold chemistry.
Here we propose and demonstrate a new way of using SG type methods in order to split and recombine matter waves. We use Rabi oscillations and magnetic field gradients in order to split87Rb atoms into two momentum components while keeping the two outputs of the beam splitter (BS) in the same spin state (Zeeman sublevels). After recombining the two outputs of the BS a spatial fringe pattern is observed. The new BS may enable a wide range of applications, such as, fundamental studies of many-body entanglement and dephasing processes, probing classical and quantum properties of nearby solids, and metrology of rotation, acceleration and gravity on a chip scale.
The Stern-Gerlach (SG) effect, discovered almost a century ago, has become a paradigm of quantum mechanics. Surprisingly there is little evidence that the original scheme with freely propagating atoms exposed to gradients from macroscopic magnets is a fully coherent quantum process. Specifically, no high-visibility spatial interference pattern has been observed with such a scheme, and furthermore no full-loop SG interferometer has been realized with the scheme as envisioned decades ago. On the contrary, numerous theoretical studies explained why it is a near impossible endeavor. Here we demonstrate for the first time both a high-visibility spatial SG interference pattern and a full-loop SG interferometer, based on an accurate magnetic field, originating from an atom chip, that ensures coherent operation within strict constraints described by previous theoretical analyses. This also allows us to observe the gradual emergence of time-irreversibility as the splitting is increased. Finally, achieving this high level of control over magnetic gradients may facilitate technological applications such as large-momentum-transfer beam splitting for metrology with atom interferometry, ultra-sensitive probing of electron transport down to shot-noise and squeezed currents, as well as nuclear magnetic resonance and compact accelerators.
We study the birefringence of quantized polarized light in a magneto-optically manipulated atomic ensemble as a generalized Stern-Gerlach effect of light. To explain this engineered birefringence microscopically, we derive an effective Shr\"odinger equation for the spatial motion of two orthogonally polarized components, which behave as a spin with an effective magnetic moment leading to a Stern-Gerlach split in a nonuniform magnetic field. We show that the electromagnetically-induced-transparency mechanism can enhance the magneto-optical Stern-Gerlach effect of light in the presence of a control field with a transverse spatial profile and a nonuniform magnetic field.
Ultracold single molecules have wide-ranging potential applications, such as ultracold chemistry, precision measurements, quantum simulation, and quantum computation. However, given the difficulty of achieving full control of a complex atom-molecule system, the coherent formation of single molecules remains a challenge. Here, we report an alternative route to coherently bind two atoms into a weakly bound molecule at megahertz levels by coupling atomic spins to their two-body relative motion in a strongly focused laser with inherent polarization gradients. The coherent nature is demonstrated by long-lived atom-molecule Rabi oscillations. We further manipulate the motional levels of the molecules and measure the binding energy precisely. This work opens the door to full control of all degrees of freedom in atom-molecule systems.
The Stern-Gerlach experiment performed in 1922 is a seminal work of modern physics. It was the experiment that first showed the quantized nature of the spin of an atom. This dissertation returns to this early experiment and describes the design, construction, and characterization of a variation that produces a one-dimensional Stern-Gerlach effect, or 1D kick, on a beam of neutral lithium atoms. Our technique relies on the combination of a magnetic field gradient and a strong bias field to generate a one-dimensional force on lithium entrained in a supersonic helium beam. By adjusting the bias field via variable, pulsed currents, we demonstrate the transition from a purely dispersive kick to a one-dimensional kick where off-axis heating of the beam has been eliminated. Pure one-dimensional forces enable access to new atomic and molecular cooling methods that can replace or supplement existing techniques to produce larger samples of cold atoms currently limited by evaporative cooling. Simulations suggest that the proposed magneto-optical cooling utilizing one-dimensional kicks will increase the total number of atoms in cold atom traps by orders of magnitude thus opening applications such as high flux atom lasers and more sensitive atom interferometry.
In the optical Stern-Gerlach effect the interaction of a two-level atom with an optical-field gradient causes a state-selective deflection that leads to a splitting of the atomic trajectory. The semiclassical approach to this problem actually predicts a splitting of the atomic beam into two paths, similar to the well-known magnetic Stern-Gerlach effect for spin 1/2. Here we study a model in which the quantum nature of the field is taken into account and we show, in particular, that for an initial coherent state of the cavity light the optical Stern-Gerlach effect manifests itself as a splitting of the atomic beam into two groups containing, however, many spots. \textcopyright{} 1996 The American Physical Society.